journal article·2021-11-12

Evolution of the metallic state in LaNiO3/LaAlO3 superlattices measured by Li8β -detected NMR

Victoria L. Karner, Aris Chatzichristos, David L. Cortie, Derek Fujimoto, Robert F. Kiefl, C. D. Philip Levy, Ruohong Li, Ryan M. L. McFadden, Gerald D. Morris, Matthew R. Pearson, Eva Benckiser, Alexander V. Boris, Georg Cristiani, Gennady Logvenov, Bernhard Keimer, W. Andrew MacFarlane

Physical Review B· Volume 104· Issue 20
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Abstract

Using ion-implanted $8\mathrm{Li} \ensuremath{\beta}$-detected NMR, we study the evolution of the correlated metallic state of ${\mathrm{LaNiO}}3$ in a series of ${\mathrm{LaNiO}}3/{\mathrm{LaAlO}}3$ superlattices as a function of bilayer thickness. Spin-lattice relaxation measurements in an applied field of $6.55\phantom{\rule{0.16em}{0ex}}\mathrm{T}$ reveal two equal amplitude components: one with metallic ($T$ linear) $1/{T}1$ and a second with a more complex $T$ dependence. The metallic character of the slow relaxing component is only weakly affected by the ${\mathrm{LaNiO}}3$ thickness, while the fast component is much more sensitive, exhibiting the opposite temperature dependence (increasing toward low $T$) in the thinnest, most magnetic samples. The origin of this bipartite relaxation is discussed in terms of electronic phase separation.
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Research context

OpenAlex topics: Magnetic and transport properties of perovskites and related materials · Advanced Condensed Matter Physics · Rare-earth and actinide compounds

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

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