journal article·2021-07-21Open access

Absorption properties of graphene quantum dots under ultrashort optical pulses

S. Azar Oliaei Motlagh, Vadym Apalkov

Physical Review B· Volume 104· Issue 4

Abstract

We study the interaction of graphene quantum dots (GQDs) with ultrashort and strong optical pulses theoretically. An important characteristic of such interaction is the energy accumulated by GQDs after the pulse. We show that the GQD absorbance has a highly nonlinear dependence on the field amplitude. At small-field amplitudes, the absorbance strongly depends on the frequency of the pulse and the band gap of a QD, i.e., its size. At large-field amplitudes, $\ensuremath{\sim}1$ V/\AA{}, the absorbance has a weak nonmonotonic dependence on the size of the dot with its maximum value of $\ensuremath{\approx}4.5$% realized for GQD consisting of $\ensuremath{\approx}60$ atoms. As a function of the field amplitude, the absorbance also has a maximum, the position of which depends on the size of the dot.
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Research context

OpenAlex topics: Quantum optics and atomic interactions · Graphene research and applications · Quantum and electron transport phenomena

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Affiliations

Center for Nano-Optics (CeNO) and Department of Physics and Astronomy, Georgia State University, Atlanta, Georgia 30303, USA

Funding

U.S. Department of Energy · Basic Energy Sciences · Division of Materials Sciences and Engineering

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