journal article·2019-12-06Open access

Circular dichroism of second harmonic generation response

S. W. Lovesey, G. van der Laan

Physical Review B· Volume 100· Issue 24

Abstract

Polarization-dependent photon spectroscopy (dichroism) of the second-harmonic generation response is shown to reveal chiral and magnetic properties of a sample. Two dichroic signals are allowed with electric-dipole and electric-quadrupole scattering events, and both require circular polarization in the primary beam. Explicit expressions for the signals are derived using theoretical techniques from atomic physics.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Spectroscopy and Quantum Chemical Studies · Advanced Chemical Physics Studies · Molecular spectroscopy and chirality

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