journal article·2024-03-11Open access

Probing quantum criticality in ferromagnetic CeRh6Ge4

S. M. Thomas, S. Seo, T. Asaba, F. Ronning, P. F. S. Rosa, E. D. Bauer, J. D. Thompson

Physical Review B· Volume 109· Issue 12

Abstract

${\mathrm{CeRh}}6{\mathrm{Ge}}4$ is unusual in that its ferromagnetic transition can be suppressed continuously to zero temperature, i.e., to a ferromagnetic quantum-critical point (QCP), through the application of modest hydrostatic pressure. This discovery has raised the possibility that the ferromagnetic QCP may be of the Kondo-breakdown type characterized by a jump in Fermi volume, to which thermopower $S$ measurements should be sensitive. Though $S/T$ changes both sign and magnitude around the critical pressure ${\mathrm{P}}c\ensuremath{\approx}0.8$ GPa, these changes are not abrupt but extend over a pressure interval from within the ferromagnetic state up to ${\mathrm{P}}c$. Together with temperature and pressure variations in electrical resistivity and previously reported heat capacity, thermopower results point to the near coincidence of two sequential effects near ${\mathrm{P}}c$, delocalization of $4f$ degrees of freedom through orbital-selective hybridization followed by quantum criticality of itinerant ferromagnetism.
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Research context

OpenAlex topics: Rare-earth and actinide compounds · Iron-based superconductors research · Advanced Chemical Physics Studies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

MPA-Quantum, Los Alamos National Laboratory, Los Alamos, New Mexico 87544, USA

Department of Physics, Changwon National University, Changwon 51140, South Korea

Funding

U.S. Department of Energy · National Research Foundation of Korea

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