Frustrated magnetic cycloidal structure and emergent Potts nematicity in CaMn2P2
Source abstract
Abstract
We report neutron-diffraction results on single-crystal ${\mathrm{CaMn}}2{\mathrm{P}}2$ containing corrugated Mn honeycomb layers, and we determine its ground-state magnetic structure. The diffraction patterns consist of prominent (1/6,1/6,$L$) reciprocal-lattice unit (r.l.u.; $L$ = integer) magnetic Bragg reflections, whose temperature-dependent intensities are consistent with a first-order antiferromagnetic phase transition at the N\'eel temperature ${T}_{\mathrm{N}}=70(1)$ K. Our analysis of the diffraction patterns reveals an in-plane $6\ifmmode\times\else\texttimes\fi{}6$ magnetic unit cell with ordered spins that in the principal-axis directions rotate by ${60}^{\ensuremath{\circ}}$ steps between nearest neighbors on each sublattice that forms the honeycomb structure, consistent with the ${P}Ac$ magnetic space group. We find that a few other magnetic subgroup symmetries (${P}A2/c$, ${P}C2/m$, ${P}S\overline{1},{P}C2,{P}Cm,{P}S1$) of the paramagnetic $P\overline{3}m{11}^{\ensuremath{'}}$ crystal symmetry are consistent with the observed diffraction pattern. We relate our findings to frustrated ${J}1\text{\ensuremath{-}}{J}2\text{\ensuremath{-}}{J}3$ Heisenberg honeycomb antiferromagnets with single-ion anisotropy and the emergence of Potts nematicity.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Advanced Condensed Matter Physics · Physics of Superconductivity and Magnetism · Iron-based superconductors research
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Ames National Laboratory, Iowa State University, Ames, Iowa 50011, USA
Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011, USA
The Missouri Research Reactor and Department of Physics and Astronomy, University of Missouri, Columbia, Missouri 65211, USA
Funding
U.S. Department of Energy · Basic Energy Sciences · Division of Materials Sciences and Engineering · Ames Laboratory · Iowa State University
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