journal article·2022-03-30Open access

Doping-driven resistive collapse of the Mott insulator in a minimal model for VO2

L. Fratino, S. Bag, A. Camjayi, M. Civelli, M. Rozenberg

Physical Review B· Volume 105· Issue 12

Abstract

We study the resistive collapse of the Mott insulator state in the dimer Hubbard model. This minimal model has been used to describe the physics of ${\mathrm{VO}}2$, and should be relevant to other strongly correlated materials. It incorporates the physics of correlated dimers and the explicit competition between on-site Coulomb repulsion and magnetic exchange interactions. Our results unveil that between the Mott insulator at half filling and the Fermi liquid metal at high doping there is an intermediate bad metallic phase with exotic features such as a pseudogap, orbital selectivity, and a first-order metal-metal transition. The model is solved within dynamical mean field theory by means of quantum Monte Carlo, which provides the numerically exact solution of the model in the limit of large lattice dimensionality. This model can be considered as a minimal one that captures exotic phenomena associated to the physics of a doped Mott insulator, shading light on their basic physical mechanism.
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Research context

OpenAlex topics: Transition Metal Oxide Nanomaterials · Advanced Condensed Matter Physics · Magnetic and transport properties of perovskites and related materials

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Affiliations

Université Paris-Saclay, Centre National de la Recherche Scientifique Laboratoire de Physique des Solides, 91405 Orsay, France

Universidad de Buenos Aires, Ciclo Básico Común and CONICET, Universidad de Buenos Aires, Instituto de Física de Buenos Aires, Pabellón 1, Ciudad Universitaria, 1428, CABA, Argentina

Funding

Agence Nationale de la Recherche · U.S. Department of Energy · Consejo Nacional de Investigaciones Científicas y Técnicas · Secretaría de Ciencia y Técnica, Universidad de Buenos Aires

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