Direct observation of coexisting Kondo hybridization and antiferromagnetic state in UAs2
Source abstract
Abstract
In $f$-electron heavy fermion systems, a wide variety of fascinating magnetic and electronic properties arise, and they are often thought to be related to a crossover behavior between localized and itinerant regimes for $f$ electrons. Uranium-based compounds with partially occupied $5f$ orbitals provide an ideal platform to elucidate the outstanding issue of the competition between magnetic order and Kondo entanglement. Using angle-resolved photoemission spectroscopy, complemented by density functional theory simulations, we probe the temperature-dependent evolution of the low-energy electronic structure of ${\mathrm{UAs}}2$ and observe two nearly flat bands of different origin in the antiferromagnetic (AFM) state. A nearly flat band which behaves with quasi-two-dimensional character has been observed and contributed to the heavy spectral weight at the \cyrchar\CYRG{} point around ${E}_{\mathrm{F}}$. This flat band reveals typical Kondo hybridization. Another flat band around the $M$ point is closely related to paramagnetic (PM)-AFM phase transition, which opens an energy gap below the transition temperature \ensuremath{\sim}273 K. Our results provide direct spectral demonstration of the electronic structure evolution across the $f\text{\ensuremath{-}}c$ hybridization and PM-AFM transition in ${\mathrm{UAs}}2$.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Rare-earth and actinide compounds · Iron-based superconductors research · Physics of Superconductivity and Magnetism
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
References (40)
Show source-provided references
1. 10.1103/RevModPhys.56.75510.1103/RevModPhys.56.755 ↗
2. 10.1103/PhysRevLett.43.189210.1103/PhysRevLett.43.1892 ↗
3. 10.1016/0378-4363(84)90153-010.1016/0378-4363(84)90153-0 ↗
4. 10.1103/PhysRevLett.55.272710.1103/PhysRevLett.55.2727 ↗
5. 10.1007/BF0145375010.1007/BF01453750 ↗
6. 10.1126/science.109164810.1126/science.1091648 ↗
7. 10.1038/nmat239510.1038/nmat2395 ↗
8. 10.1051/jphys:0198000410301930010.1051/jphys:01980004103019300 ↗
9. 10.1088/0034-4885/79/7/074501/meta10.1088/0034-4885/79/7/074501/meta ↗
10. 10.1103/PhysRevLett.90.24720410.1103/PhysRevLett.90.247204 ↗
11. 10.1038/3510150710.1038/35101507 ↗
12. 10.1088/0953-8984/13/35/20210.1088/0953-8984/13/35/202 ↗
13. 10.1103/PhysRevB.14.116510.1103/PhysRevB.14.1165 ↗
14. 10.1103/PhysRevB.48.718310.1103/PhysRevB.48.7183 ↗
15. 10.1038/nphys137410.1038/nphys1374 ↗
16. 10.1038/nphys129910.1038/nphys1299 ↗
17. 10.1016/j.jmmm.2015.09.00810.1016/j.jmmm.2015.09.008 ↗
18. 10.1126/sciadv.aat715810.1126/sciadv.aat7158 ↗
19. 10.1103/PhysRevLett.123.10640210.1103/PhysRevLett.123.106402 ↗
20. 10.1016/S0921-4526(99)00918-710.1016/S0921-4526(99)00918-7 ↗
21. 10.1088/0953-8984/12/9/30210.1088/0953-8984/12/9/302 ↗
22. 10.1103/PhysRevLett.118.04680210.1103/PhysRevLett.118.046802 ↗
23. 10.1016/0927-0256(96)00008-010.1016/0927-0256(96)00008-0 ↗
24. 10.1103/PhysRevB.54.1116910.1103/PhysRevB.54.11169 ↗
25. 10.1103/PhysRevB.49.1425110.1103/PhysRevB.49.14251 ↗
26. 10.1103/PhysRevB.47.55810.1103/PhysRevB.47.558 ↗
27. 10.1103/PhysRevLett.77.386510.1103/PhysRevLett.77.3865 ↗
28. 10.1016/0304-8853(84)90291-910.1016/0304-8853(84)90291-9 ↗
29. 10.1103/PhysRevB.104.23510310.1103/PhysRevB.104.235103 ↗
30. 10.1103/PhysRevLett.100.09640410.1103/PhysRevLett.100.096404 ↗
31. 10.1103/PhysRevLett.92.01640110.1103/PhysRevLett.92.016401 ↗
32. 10.1103/PhysRevB.96.04510710.1103/PhysRevB.96.045107 ↗
33. 10.7566/JPSJ.85.06200110.7566/JPSJ.85.062001 ↗
34. 10.1103/PhysRevLett.100.17640210.1103/PhysRevLett.100.176402 ↗
35. 10.1103/PhysRevB.46.582610.1103/PhysRevB.46.5826 ↗
36. 10.1103/PhysRevB.49.1527110.1103/PhysRevB.49.15271 ↗
37. 10.1103/PhysRevB.31.729610.1103/PhysRevB.31.7296 ↗
38. 10.1016/S0081-1947(08)60378-110.1016/S0081-1947(08)60378-1 ↗
39. 10.1103/RevModPhys.79.101510.1103/RevModPhys.79.1015 ↗
40. 10.1016/S0368-2048(01)00257-210.1016/S0368-2048(01)00257-2 ↗