journal article·2022-09-14

Direct observation of coexisting Kondo hybridization and antiferromagnetic state in UAs2

Xingyu Ji, Xuebing Luo, Qiuyun Chen, Wei Feng, Qunqing Hao, Qin Liu, Yun Zhang, Yi Liu, Xiyang Wang, Shiyong Tan, Xinchun Lai

Physical Review B· Volume 106· Issue 12
Publisher page

Abstract

In $f$-electron heavy fermion systems, a wide variety of fascinating magnetic and electronic properties arise, and they are often thought to be related to a crossover behavior between localized and itinerant regimes for $f$ electrons. Uranium-based compounds with partially occupied $5f$ orbitals provide an ideal platform to elucidate the outstanding issue of the competition between magnetic order and Kondo entanglement. Using angle-resolved photoemission spectroscopy, complemented by density functional theory simulations, we probe the temperature-dependent evolution of the low-energy electronic structure of ${\mathrm{UAs}}2$ and observe two nearly flat bands of different origin in the antiferromagnetic (AFM) state. A nearly flat band which behaves with quasi-two-dimensional character has been observed and contributed to the heavy spectral weight at the \cyrchar\CYRG{} point around ${E}_{\mathrm{F}}$. This flat band reveals typical Kondo hybridization. Another flat band around the $M$ point is closely related to paramagnetic (PM)-AFM phase transition, which opens an energy gap below the transition temperature \ensuremath{\sim}273 K. Our results provide direct spectral demonstration of the electronic structure evolution across the $f\text{\ensuremath{-}}c$ hybridization and PM-AFM transition in ${\mathrm{UAs}}2$.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Rare-earth and actinide compounds · Iron-based superconductors research · Physics of Superconductivity and Magnetism

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (40)

Show source-provided references
1. 10.1103/RevModPhys.56.75510.1103/RevModPhys.56.755 ↗
2. 10.1103/PhysRevLett.43.189210.1103/PhysRevLett.43.1892 ↗
3. 10.1016/0378-4363(84)90153-010.1016/0378-4363(84)90153-0 ↗
4. 10.1103/PhysRevLett.55.272710.1103/PhysRevLett.55.2727 ↗
5. 10.1007/BF0145375010.1007/BF01453750 ↗
6. 10.1126/science.109164810.1126/science.1091648 ↗
7. 10.1038/nmat239510.1038/nmat2395 ↗
8. 10.1051/jphys:0198000410301930010.1051/jphys:01980004103019300 ↗
9. 10.1088/0034-4885/79/7/074501/meta10.1088/0034-4885/79/7/074501/meta ↗
10. 10.1103/PhysRevLett.90.24720410.1103/PhysRevLett.90.247204 ↗
11. 10.1038/3510150710.1038/35101507 ↗
12. 10.1088/0953-8984/13/35/20210.1088/0953-8984/13/35/202 ↗
13. 10.1103/PhysRevB.14.116510.1103/PhysRevB.14.1165 ↗
14. 10.1103/PhysRevB.48.718310.1103/PhysRevB.48.7183 ↗
15. 10.1038/nphys137410.1038/nphys1374 ↗
16. 10.1038/nphys129910.1038/nphys1299 ↗
17. 10.1016/j.jmmm.2015.09.00810.1016/j.jmmm.2015.09.008 ↗
18. 10.1126/sciadv.aat715810.1126/sciadv.aat7158 ↗
19. 10.1103/PhysRevLett.123.10640210.1103/PhysRevLett.123.106402 ↗
20. 10.1016/S0921-4526(99)00918-710.1016/S0921-4526(99)00918-7 ↗
21. 10.1088/0953-8984/12/9/30210.1088/0953-8984/12/9/302 ↗
22. 10.1103/PhysRevLett.118.04680210.1103/PhysRevLett.118.046802 ↗
23. 10.1016/0927-0256(96)00008-010.1016/0927-0256(96)00008-0 ↗
24. 10.1103/PhysRevB.54.1116910.1103/PhysRevB.54.11169 ↗
25. 10.1103/PhysRevB.49.1425110.1103/PhysRevB.49.14251 ↗
26. 10.1103/PhysRevB.47.55810.1103/PhysRevB.47.558 ↗
27. 10.1103/PhysRevLett.77.386510.1103/PhysRevLett.77.3865 ↗
28. 10.1016/0304-8853(84)90291-910.1016/0304-8853(84)90291-9 ↗
29. 10.1103/PhysRevB.104.23510310.1103/PhysRevB.104.235103 ↗
30. 10.1103/PhysRevLett.100.09640410.1103/PhysRevLett.100.096404 ↗
31. 10.1103/PhysRevLett.92.01640110.1103/PhysRevLett.92.016401 ↗
32. 10.1103/PhysRevB.96.04510710.1103/PhysRevB.96.045107 ↗
33. 10.7566/JPSJ.85.06200110.7566/JPSJ.85.062001 ↗
34. 10.1103/PhysRevLett.100.17640210.1103/PhysRevLett.100.176402 ↗
35. 10.1103/PhysRevB.46.582610.1103/PhysRevB.46.5826 ↗
36. 10.1103/PhysRevB.49.1527110.1103/PhysRevB.49.15271 ↗
37. 10.1103/PhysRevB.31.729610.1103/PhysRevB.31.7296 ↗
38. 10.1016/S0081-1947(08)60378-110.1016/S0081-1947(08)60378-1 ↗
39. 10.1103/RevModPhys.79.101510.1103/RevModPhys.79.1015 ↗
40. 10.1016/S0368-2048(01)00257-210.1016/S0368-2048(01)00257-2 ↗