Effect of intersystem crossing rates and optical illumination on the polarization of nuclear spins close to nitrogen-vacancy centers

H. Duarte; H. T. Dinani; V. Jacques; J. R. Maze

doi:10.1103/physrevb.103.195443

journal article·2021-05-27Open access

Effect of intersystem crossing rates and optical illumination on the polarization of nuclear spins close to nitrogen-vacancy centers

H. Duarte, H. T. Dinani, V. Jacques, J. R. Maze

Physical Review B· Volume 103· Issue 19

Publisher page Open full text

Source abstract

Abstract

Several methods to polarize nuclear spins nearby nitrogen-vacancy centers rely on electron spin polarization and therefore on the intersystem crossing rates. Here, the authors consider the effect of these rates on nuclear polarization methods based on the level anticrossing, and precession of the nuclear population while the electronic spin is on the ground state for different nuclear spins. These results are relevant for validating the models for intersystem crossing rates and achieving a higher nuclear polarization.

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Research context

OpenAlex topics: Diamond and Carbon-based Materials Research · Atomic and Subatomic Physics Research · High-pressure geophysics and materials

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Facultad de Física, Pontificia Universidad Católica de Chile, Santiago 7820436, Chile

Faculty of Physics, Universidad Técnica Federico Santa María, Avda. Vicuña Mackenna 3939, Santiago, Chile

Centro de Investigación DAiTA Lab, Facultad de Estudios Interdisciplinarios, Universidad Mayor, Santiago 7560908, Chile

L2C, Laboratoire Charles Coulomb, Université de Montpellier and CNRS, Montpellier 34095, France

Research Centre for Nanotechnology and Advanced Materials, Pontificia Universidad Católica de Chile, Santiago 7820436, Chile

Funding

Comisión Nacional de Investigación Científica y Tecnológica · Fondo Nacional de Desarrollo Científico y Tecnológico · Office of Naval Research · Air Force

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