journal article·2017-04-18Open access

Field-induced phase diagram of the XY pyrochlore antiferromagnetEr2Ti2O7

E. Lhotel, J. Robert, E. Ressouche, F. Damay, I. Mirebeau, J. Ollivier, H. Mutka, P. Dalmas de Réotier, A. Yaouanc, C. Marin, C. Decorse, S. Petit

Physical Review B· Volume 95· Issue 13

Abstract

We explore the field-temperature phase diagram of the XY pyrochlore antiferromagnet ${\mathrm{Er}}2{\mathrm{Ti}}2{\mathrm{O}}7$ by means of magnetization and neutron diffraction experiments. Depending on the field strength and direction relative to the high symmetry cubic directions $[001],[1\overline{1}0]$, and $[111]$, the refined field-induced magnetic structures are derived from the zero field ${\ensuremath{\psi}}2$ and ${\ensuremath{\psi}}3$ states of the ${\mathrm{\ensuremath{\Gamma}}}5$ irreducible representation which describes the ground state of XY pyrochlore antiferromagnets. At low field, domain selection effects are systematically at play. In addition, for $[001]$, a phase transition is reported towards a ${\ensuremath{\psi}}3$ structure at a characteristic field ${H}c001=43$ mT. For $[1\overline{1}0]$ and $[111]$, the spins are continuously tilted by the field from the ${\ensuremath{\psi}}2$ state, and no phase transition is found while domain selection gives rise to sharp anomalies in the field dependence of the Bragg peaks intensity. For $[1\overline{1}0]$, these results are confirmed by high resolution inelastic neutron scattering experiments, which in addition allow us to determine the field dependence of the spin gap. This study agrees qualitatively with the scenario proposed theoretically by Maryasin et al. [Phys. Rev. B 93, 100406(R) (2016)], yet the strength of the field-induced anisotropies is significantly different from theory.
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OpenAlex topics: Advanced Condensed Matter Physics · Multiferroics and related materials · Nuclear materials and radiation effects

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