journal article·2016-05-23

Kinetic narrowing of size distribution

V. G. Dubrovskii

Physical Review B· Volume 93· Issue 17
Publisher page

Abstract

We present a model that reveals an interesting possibility for narrowing the size distribution of nanostructures when the deterministic growth rate changes its sign from positive to negative at a certain stationary size. Such a behavior occurs in self-catalyzed one-dimensional III-V nanowires and more generally whenever a negative ``adsorption-desorption'' term in the growth rate is compensated by a positive ``diffusion flux.'' By asymptotically solving the Fokker-Planck equation, we derive an explicit representation for the size distribution that describes either Poissonian broadening or self-regulated narrowing depending on the parameters. We show how the fluctuation-induced spreading of the size distribution can be completely suppressed in systems with size self-stabilization. These results can be used for obtaining size-uniform ensembles of different nanostructures.
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Research context

OpenAlex topics: Semiconductor Quantum Structures and Devices · Advancements in Semiconductor Devices and Circuit Design · Nanowire Synthesis and Applications

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