Fractional electromagnetic response in a three-dimensional chiral anomalous semimetal

The magnetoelectric coupling of electrons in a three-dimensional solid can be effectively described by axion electrodynamics. Here we report the discovery of the fractional magnetoelectric effect in chiral anomalous semimetals of the three-dimensional massless Wilson fermions, which have linear dispersions at the energy crossing point and break the chiral symmetry at generic momenta. In the presence of electric and magnetic fields, the time-reversal and parity symmetry breaking give rise to the quarter-quantized topological magnetoelectric effect, which is directly related to the winding number 1/2 of the band structure and is only one-half of that for topological insulators. The fractional electromagnetic response can be revealed by the surface Hall conductance and extracted from the measurement of the topological Kerr and Faraday rotation. The transition-metal pentatelluride ${\mathrm{ZrTe}}₅$ with a strain-tunable band gap provides a potential platform to test the effect experimentally.