Magnetic terahertz resonances above the Néel temperature in the frustrated kagome antiferromagnet averievite
Source abstract
Abstract
Time-domain magneto-THz spectroscopy is utilized to study the frustrated magnet averievite ${\mathrm{Cu}}_{5\ensuremath{-}x}{\mathrm{Zn}}x{\mathrm{V}}2{\mathrm{O}}10$(CsCl). Pronounced THz resonances are observed in unsubstituted samples ($x=0$) when cooling below the onset of short-range magnetic correlations. The influence of external magnetic effects confirms the magnetic origin of these resonances. Increasing Zn substitution suppresses the resonances, as frustration effects dominate, reflecting the nonmagnetic phases for $x>0.25$ compounds. The temperature evolution of the THz spectra is complemented with electron spin resonance spectroscopy. This comparison allows a direct probe of the different contributions from magnetic order, frustration, and structural properties in the phase diagram of averievite. Our results illustrate the effect of magnetic interactions in THz spectra of frustrated magnets.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Advanced Condensed Matter Physics · Physics of Superconductivity and Magnetism · Multiferroics and related materials
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
1. Physikalisches Institut, Universität Stuttgart, Pfaffenwaldring 57, 70550 Stuttgart, Germany
Institute of Solid State Physics, TU Wien, 1040 Vienna, Austria
Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439, USA
Funding
Deutsche Forschungsgemeinschaft · Argonne National Laboratory · U.S. Department of Energy · Office of Science · Basic Energy Sciences
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