Anomalous rotation of the linearly polarized emission of bright excitons in strained WSe2 monolayers under high magnetic fields
Source abstract
Abstract
Linearly polarized microphotoluminescence ($\ensuremath{\mu}$-PL) measurements of strained ${\mathrm{WSe}}2$ monolayers in out-of-plane high magnetic fields are presented. At low temperature, a splitting of the bright exciton emission into two exciton components is observed, which is attributed to an in-plane uniaxial strain based on the full polarization dependence of the photoluminescence spectrum. High magnetic field measurements directly reveal a distinct evolution of the linear polarization and allows us to extract the valley coherence time constants (${T}s2*$) for both exciton components. For the high-energy transition of the exciton, the valley coherence time $\ensuremath{\simeq}0.45$ ps, closely matching ${T}s2*$ of an unstrained monolayer ($\ensuremath{\simeq}0.34$ ps). For the low-energy exciton, however, ${T}s2*$ is four times larger, $\ensuremath{\simeq}1.97$ ps. This valley coherence time observed here may be explored for future valleytronic applications.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: 2D Materials and Applications · Perovskite Materials and Applications · MXene and MAX Phase Materials
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
References (32)
Show source-provided references
1. 10.1038/nphys294210.1038/nphys2942 ↗
2. 10.1038/nphoton.2015.28210.1038/nphoton.2015.282 ↗
3. 10.1038/natrevmats.2016.5510.1038/natrevmats.2016.55 ↗
4. 10.1103/PhysRevLett.105.13680510.1103/PhysRevLett.105.136805 ↗
5. 10.1021/nl903868w10.1021/nl903868w ↗
6. 10.1103/PhysRevLett.108.19680210.1103/PhysRevLett.108.196802 ↗
7. 10.1093/nsr/nwu07810.1093/nsr/nwu078 ↗
8. 10.1515/nanoph-2016-016510.1515/nanoph-2016-0165 ↗
9. 10.1038/nnano.2012.9610.1038/nnano.2012.96 ↗
10. 10.1038/ncomms188210.1038/ncomms1882 ↗
11. 10.1038/nnano.2013.15110.1038/nnano.2013.151 ↗
12. 10.1038/nphys389110.1038/nphys3891 ↗
13. 10.1038/nphys320110.1038/nphys3201 ↗
14. 10.1103/PhysRevLett.117.07740210.1103/PhysRevLett.117.077402 ↗
15. 10.1103/PhysRevLett.117.18740110.1103/PhysRevLett.117.187401 ↗
16. 10.1038/nature0753010.1038/nature07530 ↗
17. 10.1063/1.360147910.1063/1.3601479 ↗
18. 10.1016/j.cap.2018.04.00310.1016/j.cap.2018.04.003 ↗
19. 10.1021/acs.nanolett.7b0486810.1021/acs.nanolett.7b04868 ↗
20. 10.1103/PhysRevB.98.11530810.1103/PhysRevB.98.115308 ↗
21. 10.1103/PhysRevB.98.23542910.1103/PhysRevB.98.235429 ↗
22. 10.1038/nphys320310.1038/nphys3203 ↗
23. 10.1038/nphys360410.1038/nphys3604 ↗
24. 10.1038/ncomms487610.1038/ncomms4876 ↗
25. 10.1038/ncomms1271510.1038/ncomms12715 ↗
26. 10.1103/PhysRevB.88.12130110.1103/PhysRevB.88.121301 ↗
27. M. Dyakonov · 200810.1007/978-3-540-78820-1 ↗
28. 10.1103/PhysRevB.90.07541310.1103/PhysRevB.90.075413 ↗
29. 10.1038/ncomms931510.1038/ncomms9315 ↗
30. 10.1103/PhysRevB.93.20542310.1103/PhysRevB.93.205423 ↗
31. 10.1021/nl503799t10.1021/nl503799t ↗
32. 10.1088/2053-1583/2/3/03400210.1088/2053-1583/2/3/034002 ↗