journal article·2019-04-16Open access

Anomalous rotation of the linearly polarized emission of bright excitons in strained WSe2 monolayers under high magnetic fields

A. Mitioglu, S. Anghel, M. V. Ballottin, K. Sushkevich, L. Kulyuk, P. C. M. Christianen

Physical Review B· Volume 99· Issue 15

Abstract

Linearly polarized microphotoluminescence ($\ensuremath{\mu}$-PL) measurements of strained ${\mathrm{WSe}}2$ monolayers in out-of-plane high magnetic fields are presented. At low temperature, a splitting of the bright exciton emission into two exciton components is observed, which is attributed to an in-plane uniaxial strain based on the full polarization dependence of the photoluminescence spectrum. High magnetic field measurements directly reveal a distinct evolution of the linear polarization and allows us to extract the valley coherence time constants (${T}s2*$) for both exciton components. For the high-energy transition of the exciton, the valley coherence time $\ensuremath{\simeq}0.45$ ps, closely matching ${T}s2*$ of an unstrained monolayer ($\ensuremath{\simeq}0.34$ ps). For the low-energy exciton, however, ${T}s2*$ is four times larger, $\ensuremath{\simeq}1.97$ ps. This valley coherence time observed here may be explored for future valleytronic applications.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: 2D Materials and Applications · Perovskite Materials and Applications · MXene and MAX Phase Materials

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (32)

Show source-provided references
1. 10.1038/nphys294210.1038/nphys2942 ↗
2. 10.1038/nphoton.2015.28210.1038/nphoton.2015.282 ↗
3. 10.1038/natrevmats.2016.5510.1038/natrevmats.2016.55 ↗
4. 10.1103/PhysRevLett.105.13680510.1103/PhysRevLett.105.136805 ↗
5. 10.1021/nl903868w10.1021/nl903868w ↗
6. 10.1103/PhysRevLett.108.19680210.1103/PhysRevLett.108.196802 ↗
7. 10.1093/nsr/nwu07810.1093/nsr/nwu078 ↗
8. 10.1515/nanoph-2016-016510.1515/nanoph-2016-0165 ↗
9. 10.1038/nnano.2012.9610.1038/nnano.2012.96 ↗
10. 10.1038/ncomms188210.1038/ncomms1882 ↗
11. 10.1038/nnano.2013.15110.1038/nnano.2013.151 ↗
12. 10.1038/nphys389110.1038/nphys3891 ↗
13. 10.1038/nphys320110.1038/nphys3201 ↗
14. 10.1103/PhysRevLett.117.07740210.1103/PhysRevLett.117.077402 ↗
15. 10.1103/PhysRevLett.117.18740110.1103/PhysRevLett.117.187401 ↗
16. 10.1038/nature0753010.1038/nature07530 ↗
17. 10.1063/1.360147910.1063/1.3601479 ↗
18. 10.1016/j.cap.2018.04.00310.1016/j.cap.2018.04.003 ↗
19. 10.1021/acs.nanolett.7b0486810.1021/acs.nanolett.7b04868 ↗
20. 10.1103/PhysRevB.98.11530810.1103/PhysRevB.98.115308 ↗
21. 10.1103/PhysRevB.98.23542910.1103/PhysRevB.98.235429 ↗
22. 10.1038/nphys320310.1038/nphys3203 ↗
23. 10.1038/nphys360410.1038/nphys3604 ↗
24. 10.1038/ncomms487610.1038/ncomms4876 ↗
25. 10.1038/ncomms1271510.1038/ncomms12715 ↗
26. 10.1103/PhysRevB.88.12130110.1103/PhysRevB.88.121301 ↗
27. M. Dyakonov · 200810.1007/978-3-540-78820-1 ↗
28. 10.1103/PhysRevB.90.07541310.1103/PhysRevB.90.075413 ↗
29. 10.1038/ncomms931510.1038/ncomms9315 ↗
30. 10.1103/PhysRevB.93.20542310.1103/PhysRevB.93.205423 ↗
31. 10.1021/nl503799t10.1021/nl503799t ↗
32. 10.1088/2053-1583/2/3/03400210.1088/2053-1583/2/3/034002 ↗