journal article·2021-03-15Open access

Quantum geometric exciton drift velocity

Jinlyu Cao, H. A. Fertig, Luis Brey

Physical Review B· Volume 103· Issue 11

Abstract

In many situations, excitons---bound particle-hole pairs above an insulating ground state---carry an electric dipole moment, allowing them to be manipulated via coupling to an electric field. For two-dimensional systems, we demonstrate that this property of an exciton is uniquely determined by the quantum geometry of its eigenstates, and demonstrate its intimate connection with a quantity which we call the quantum geometric dipole. We demonstrate that this quantity arises naturally in the semiclassical equations of motion of an exciton in an electric field, adding a term additional to the anomalous velocity coming from Berry's curvature. In a uniform electric field, this contributes a drift velocity to the exciton akin to that expected for excitons in crossed electric and magnetic fields, even in the absence of a real magnetic field. We compute the quantities relevant to semiclassical exciton dynamics for several interesting examples of bilayer systems with weak interlayer tunneling and Fermi energy in a gap, where the exciton may be sensibly described as a two-body problem. These quantities include the exciton dispersion, its quantum geometric dipole, and its Berry's curvature. For a simple example of two gapped-graphene layers in a vanishing magnetic field, we demonstrate that there is a nonvanishing quantum geometric dipole when the layers are different, e.g., have different gaps, but vanishes when the layers are identical. We further analyze examples in the presence of magnetic fields, allowing us to examine cases involving graphene, in which a gap is opened by Landau level splitting. Heterostructures involving transition metal dichalcogenides materials are also considered. In each case, the quantum geometric dipole and Berry's curvatures play out in different ways. In some cases, the lowest energy exciton state is found to reside at finite momentum, with interesting possible consequences for Bose condensation in these systems. Additionally, we find situations in which the quantum geometric dipole increases monotonically with exciton momentum, suggesting that the quantum geometry can be exploited to produce photocurrents from initially bound excitons with electric fields, without the need to overcome an effective barrier via tunneling or thermal excitation. We speculate on further possible effects of the semiclassical dynamics in geometries where the constituent layers are subject to the same or different electric fields.
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Research context

OpenAlex topics: Graphene research and applications · 2D Materials and Applications · Strong Light-Matter Interactions

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Physics, Indiana University, Bloomington, Indiana 47405, USA

Quantum Science and Engineering Center, Indiana University, Bloomington, Indiana 47408, USA

Instituto de Ciencia de Materiales de Madrid, (CSIC), Cantoblanco, 28049 Madrid, Spain

Funding

Ministerio de Ciencia e Innovación · Agencia Estatal de Investigación · Federación Española de Enfermedades Raras · National Science Foundation · Aspen Center for Physics · United States - Israel Binational Science Foundation · Research Corporation for Science Advancement · Indiana University

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