journal article·2017-12-08Open access

Rb-NMR study of the quasi-one-dimensional competing spin-chain compound Rb2Cu2Mo3O12

Kazuki Matsui, Ayato Yagi, Yukihiro Hoshino, Sochiro Atarashi, Masashi Hase, Takahiko Sasaki, Takayuki Goto

Physical Review B· Volume 96· Issue 22

Abstract

A Rb-NMR study has been performed on the quasi-one-dimensional competing spin chain $\mathrm{R}{\mathrm{b}}2\mathrm{C}{\mathrm{u}}2\mathrm{M}{\mathrm{o}}3{\mathrm{O}}12$ with ferromagnetic and antiferromagnetic exchange interactions on nearest-neighboring and next-nearest neighboring spins, respectively. The system changes from a gapped ground state at zero field to a gapless state at ${H}_{\mathrm{C}}\ensuremath{\simeq}2\phantom{\rule{0.16em}{0ex}}\mathrm{T}$, where the existence of magnetic order below 1 K was demonstrated by a broadening of the NMR spectrum, associated with a critical divergence of $1/{T}1$. In the higher-temperature region, ${T}1^{\ensuremath{-}1}$ showed a power-law-type temperature dependence, from which the field dependence of the Luttinger parameter $K$ was obtained and compared with theoretical calculations based on the spin nematic Tomonaga-Luttinger liquid (TLL) state.
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Research context

OpenAlex topics: Physics of Superconductivity and Magnetism · Advanced Condensed Matter Physics · Magnetic and transport properties of perovskites and related materials

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