journal article·2017-05-09Open access

Fast recovery of the stripe magnetic order by Mn/Fe substitution in F-doped LaFeAsO superconductors

M. Moroni, P. Carretta, G. Allodi, R. De Renzi, M. N. Gastiasoro, B. M. Andersen, P. Materne, H.-H. Klauss, Y. Kobayashi, M. Sato, S. Sanna

Physical Review B· Volume 95· Issue 18

Abstract

$75\mathrm{As}$ nuclear magnetic (NMR) and quadrupolar (NQR) resonance were used, together with M\"ossbauer spectroscopy, to investigate the magnetic state induced by Mn for Fe substitutions in F-doped ${\mathrm{LaFe}}_{1\ensuremath{-}x}{\mathrm{Mn}}x\mathrm{AsO}$ superconductors. The results show that 0.5% of Mn doping is enough to suppress the superconducting transition temperature ${T}c$ from 27 K to zero and to recover the magnetic structure observed in the parent undoped LaFeAsO. Also the tetragonal to orthorhombic transition of the parent compound is recovered by introducing Mn, as evidenced by a sharp drop of the NQR frequency. The NQR spectra also show that a charge localization process is at play in the system. Theoretical calculations using a realistic five-band model show that correlation-enhanced RKKY exchange interactions between nearby Mn ions stabilize the observed stripe magnetic order. These results give compelling evidence that F-doped LaFeAsO is a strongly correlated electron system at the verge of an electronic instability.
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OpenAlex topics: Iron-based superconductors research · Rare-earth and actinide compounds · Corporate Taxation and Avoidance

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