Valley-contrasting orbital magnetic moment induced negative magnetoresistance

The valley-contrasting orbital magnetic moment of Bloch electrons allows the lifting of valley degeneracy by an out-of-plane magnetic field. We demonstrate that this leads to negative magnetoresistance, utilizing a gapped two-dimensional multivalley model as an example. An intuitive physical picture in terms of the increased carrier density from a magnetic gating effect is proposed for this negative magnetoresistance. In particular, giant negative magnetoresistance is achieved after one of the two valleys is depleted by the magnetic field. This mechanism of negative magnetoresistance is argued to be relevant in ionic-liquid gated gapped graphene with a small effective mass.