journal article·2020-01-10Open access

Dynamical screening effects of substrate phonons on two-dimensional excitons

Alexander Steinhoff, Matthias Florian, Frank Jahnke

Physical Review B· Volume 101· Issue 4

Abstract

Atomically thin materials are exceedingly susceptible to their dielectric environment. For transition metal dichalcogenides, sample placement on a substrate or encapsulation in hexagonal boron nitride (hBN) are frequently used. In this paper we show that the dielectric response due to optical phonons of adjacent materials influences excitons in two-dimensional (2D) crystals. We provide an analytic model for the coupling of 2D charge carriers to optical substrate phonons, which causes polaron effects similar to that of intrinsic 2D phonons. We apply the model to hBN-encapsulated ${\mathrm{WSe}}2$, finding a significant reduction of the exciton binding energies due to dynamical screening effects.
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Research context

OpenAlex topics: 2D Materials and Applications · Perovskite Materials and Applications · Graphene research and applications

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