journal article·2021-10-11Open access

Electronic structure and topology across Tc in the magnetic Weyl semimetal Co3Sn2S2

Antonio Rossi, Vsevolod Ivanov, Sudheer Sreedhar, Adam L. Gross, Zihao Shen, Eli Rotenberg, Aaron Bostwick, Chris Jozwiak, Valentin Taufour, Sergey Y. Savrasov, Inna M. Vishik

Physical Review B· Volume 104· Issue 15

Abstract

${\mathrm{Co}}3{\mathrm{Sn}}2{\mathrm{S}}2$ is a magnetic Weyl semimetal, in which ferromagnetic ordering at 177 K is predicted to stabilize Weyl points. We perform temperature and spatial dependent angle-resolved photoemission spectroscopy measurements through the Curie temperature (${T}c$), which show large band shifts and renormalization concomitant with the onset of magnetism. We argue that ${\mathrm{Co}}3{\mathrm{Sn}}2{\mathrm{S}}2$ evolves from a Mott ferromagnet below ${T}c$ to a correlated metallic state above ${T}c$. To understand the magnetism, we derive a tight-binding model of Co-$3{d}_{{x}2\ensuremath{-}{y}2}$ orbitals on the kagome lattice. At the filling obtained by first-principles calculations, this model reproduces the ferromagnetic ground state, and results in the reduction of Coulomb interactions due to cluster effects. Using a disordered local moment simulation, we show how this reduced Hubbard $U$ leads to a collapse of the bands across the magnetic transition, resulting in a correlated state, which carries associated characteristic photoemission signatures that are distinct from those of a simple lifting of exchange splitting. The behavior of topology across ${T}c$ is discussed in the context of this description of the magnetism.
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Research context

OpenAlex topics: Topological Materials and Phenomena · Advanced Condensed Matter Physics · Electronic and Structural Properties of Oxides

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