Electronic structure and topology across Tc in the magnetic Weyl semimetal Co3Sn2S2
Source abstract
Abstract
${\mathrm{Co}}3{\mathrm{Sn}}2{\mathrm{S}}2$ is a magnetic Weyl semimetal, in which ferromagnetic ordering at 177 K is predicted to stabilize Weyl points. We perform temperature and spatial dependent angle-resolved photoemission spectroscopy measurements through the Curie temperature (${T}c$), which show large band shifts and renormalization concomitant with the onset of magnetism. We argue that ${\mathrm{Co}}3{\mathrm{Sn}}2{\mathrm{S}}2$ evolves from a Mott ferromagnet below ${T}c$ to a correlated metallic state above ${T}c$. To understand the magnetism, we derive a tight-binding model of Co-$3{d}_{{x}2\ensuremath{-}{y}2}$ orbitals on the kagome lattice. At the filling obtained by first-principles calculations, this model reproduces the ferromagnetic ground state, and results in the reduction of Coulomb interactions due to cluster effects. Using a disordered local moment simulation, we show how this reduced Hubbard $U$ leads to a collapse of the bands across the magnetic transition, resulting in a correlated state, which carries associated characteristic photoemission signatures that are distinct from those of a simple lifting of exchange splitting. The behavior of topology across ${T}c$ is discussed in the context of this description of the magnetism.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Topological Materials and Phenomena · Advanced Condensed Matter Physics · Electronic and Structural Properties of Oxides
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
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