Thermally Cross-Linkable Blended Hole Transport Layer for Solution-Processed Quantum Dot Light-Emitting Diodes
Source abstract
Abstract
Solution-processed quantum-dot light-emitting diodes (QLEDs) are promising for next-generation display technology. However, the solution process challenges multilayer fabrication due to solvent-induced damage to underlying layers. We propose a robust and highly efficient hole transport layer (HTL) based on a cross-linked blend of N 4, N 4′-Di(naphthalen-1-yl)- N 4, N 4′-bis(4-vinylphenyl) biphenyl-4,4′-Diamin (VNPB) and poly[bis(4-phenyl) (2,4,6-trimethylphenyl) amine] (PTAA). A precise control of the blend ratio allows a cross-linked structure with solvent resistance and tunable hole mobility and energy levels. The blended HTL, optimized at a 2:1 VNPB/PTAA ratio, outperforms nonblended VNPB or PTAA HTLs in QLEDs. This cross-linked blending strategy offers a promising approach for high-performance QLEDs by addressing electrical properties and solvent issues.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Quantum Dots Synthesis And Properties · Chalcogenide Semiconductor Thin Films · Semiconductor Quantum Structures and Devices
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Department of Semiconductor Engineering, Gyeongsang National University, 501 Jinju-daero, Jinju, Gyeongnam 52828, Republic of Korea
Department of Energy Science, Centre for Artificial Atoms, Sungkyunkwan University (SKKU), 2066 Seobu-ro, Jangan-gu, Suwon 16419, Republic of Korea
Department of Advanced Materials, Hannam University, 1646 Yuseong-daero, Yuseong gu, Daejeon 34054, Republic of Korea
SKKU Institute of Energy Science and Technology (SIEST), Sungkyunkwan University (SKKU), 2066 Seobu-ro, Jangan-gu, Suwon 16419, Republic of Korea
Funding
Gyeongsang National University · Hannam University
References (45)
Show source-provided references
1. 10.1038/370354a010.1038/370354a0 ↗
2. 10.1021/acs.nanolett.2c0313810.1021/acs.nanolett.2c03138 ↗
3. 10.1021/acs.nanolett.3c0390410.1021/acs.nanolett.3c03904 ↗
4. 10.1002/smtd.20230122410.1002/smtd.202301224 ↗
5. 10.1002/adma.20221222010.1002/adma.202212220 ↗
6. 10.1038/s41578-020-00274-910.1038/s41578-020-00274-9 ↗
7. 10.1002/smll.20240332510.1002/smll.202403325 ↗
8. 10.1002/smll.20230729810.1002/smll.202307298 ↗
9. 10.1002/adma.20230395010.1002/adma.202303950 ↗
10. 10.1002/adma.20241397810.1002/adma.202413978 ↗
11. 10.1038/s41566-024-01496-x10.1038/s41566-024-01496-x ↗
12. 10.1038/ncomms366110.1038/ncomms3661 ↗
13. 10.1021/nl300325410.1021/nl3003254 ↗
14. 10.1021/nn403594j10.1021/nn403594j ↗
15. 10.1002/adom.20220196510.1002/adom.202201965 ↗
16. 10.1021/acsaelm.0c0009110.1021/acsaelm.0c00091 ↗
17. 10.1002/admt.20220210510.1002/admt.202202105 ↗
18. 10.1021/acsapm.0c0042710.1021/acsapm.0c00427 ↗
19. 10.1002/adma.20210779810.1002/adma.202107798 ↗
20. 10.1016/j.esci.2023.10022710.1016/j.esci.2023.100227 ↗
21. 10.1002/adom.20220093510.1002/adom.202200935 ↗
22. 10.1021/nl052417e10.1021/nl052417e ↗
23. 10.1002/adma.20060237310.1002/adma.200602373 ↗
24. 10.1021/acsami.7b0061510.1021/acsami.7b00615 ↗
25. 10.1002/sdtp.1505910.1002/sdtp.15059 ↗
26. 10.1016/j.orgel.2019.05.03010.1016/j.orgel.2019.05.030 ↗
27. 10.1016/j.cej.2022.13570210.1016/j.cej.2022.135702 ↗
28. 10.1002/advs.20220045010.1002/advs.202200450 ↗
29. 10.1021/acs.nanolett.4c0072710.1021/acs.nanolett.4c00727 ↗
30. 10.1002/smll.20190011110.1002/smll.201900111 ↗
31. 10.1021/acsami.0c0100110.1021/acsami.0c01001 ↗
32. 10.1002/(SICI)1521-4095(199903)11:3<241::AID-ADMA241>3.0.CO;2-J10.1002/(SICI)1521-4095(199903)11:3<241::AID-ADMA241>3.0.CO;2-J ↗
33. 10.1021/acsenergylett.5c0116910.1021/acsenergylett.5c01169 ↗
34. 10.1002/solr.20220023410.1002/solr.202200234 ↗
35. 10.1007/s42341-023-00499-910.1007/s42341-023-00499-9 ↗
36. 10.1002/adma.20230977910.1002/adma.202309779 ↗
37. 10.1007/s13391-020-00258-510.1007/s13391-020-00258-5 ↗
38. 10.1002/adma.20150563010.1002/adma.201505630 ↗
39. 10.1021/jp903420w10.1021/jp903420w ↗
40. 10.1021/acs.macromol.5b0113710.1021/acs.macromol.5b01137 ↗
41. 10.1002/solr.20190039610.1002/solr.201900396 ↗
42. 10.1039/C7RA08302E10.1039/C7RA08302E ↗
43. 10.1039/C9CC06882A10.1039/C9CC06882A ↗
44. 10.1021/acsami.4c1389910.1021/acsami.4c13899 ↗
45. 10.1007/s12274-022-5268-410.1007/s12274-022-5268-4 ↗