journal article·2021-05-27Open access

Two-dimensional plasmonic polarons in n -doped monolayer MoS2

Fabio Caruso, Patrick Amsalem, Jie Ma, Areej Aljarb, Thorsten Schultz, Marios Zacharias, Vincent Tung, Norbert Koch, Claudia Draxl

Physical Review B· Volume 103· Issue 20

Abstract

We report experimental and theoretical evidence of strong electron-plasmon interaction in $n$-doped single-layer ${\mathrm{MoS}}2$. Angle-resolved photoemission spectroscopy measurements reveal the emergence of distinctive signatures of polaronic coupling in the electron spectral function. Calculations based on many-body perturbation theory illustrate that electronic coupling to two-dimensional carrier plasmons provides an exhaustive explanation of the experimental spectral features and their energies. These results constitute compelling evidence of the formation of plasmon-induced polaronic quasiparticles, suggesting that highly doped transition-metal dichalcogenides may provide a new platform to explore strong-coupling phenomena between electrons and plasmons in two dimensions.
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Research context

OpenAlex topics: 2D Materials and Applications · Chalcogenide Semiconductor Thin Films · Quantum Dots Synthesis And Properties

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