journal article·2023-07-14Open access

Lensfree Air-Quality Monitoring of Fine and Ultrafine Particulate Matter Using Vapor-Condensed Nanolenses

Maryam Baker, Florian Gollier, Jeffrey E. Melzer, Euan McLeod

ACS Applied Nano Materials· Volume 6· Issue 13

Abstract

Current commercial air-quality monitoring devices lack a large dynamic range, especially at the small, ultrafine size scale. Furthermore, there is a low density of air-quality monitoring stations, reducing the precision with which local particulate matter hazards can be tracked. Here, we show a low-cost, lensfree, and portable air-quality monitoring device (LPAQD) that can detect and measure micron-sized particles down to 100 nm-sized particles, with the capability to track and measure particles in real time throughout a day and the ability to accurately measure particulate matter densities as low as 3 μg m –3 . A vapor-condensed film is deposited onto the coverslip used to collect particles before the LPAQD is deployed at outdoor monitoring sites. The vapor-condensed film increases the scattering cross section of particles smaller than the pixel size, enabling the sub-pixel and sub-diffraction-limit-sized particles to be detected. The high dynamic range, low cost, and portability of this device can enable citizens to monitor their own air quality to hopefully impact user decisions that reduce the risk for particulate matter-related diseases.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Air Quality Monitoring and Forecasting · Atmospheric aerosols and clouds · Air Quality and Health Impacts

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

University of Arizona, Wyant College of Optical Sciences, Tucson, Arizona 85721, United States

Funding

University of Arizona

References (52)

Show source-provided references
1. Billions of people still breathe unhealthy air: new WHO data. https://www.who.int/news/item/04-04-2022-billions-of-people-still-breathe-unhealthy-air-new-who-data (accessed Oct 3, 2022).
2. 10.1073/pnas.180947411510.1073/pnas.1809474115 ↗
3. 10.1073/pnas.160594111310.1073/pnas.1605941113 ↗
4. 10.3322/caac.2163210.3322/caac.21632 ↗
5. 10.1289/EHP443810.1289/EHP4438 ↗
6. 10.1038/s41569-020-0371-210.1038/s41569-020-0371-2 ↗
7. Smith, D. The Three Types of Particulate Matter: All About PM10, PM2.5, and PM0.1. https://learn.kaiterra.com/en/resources/three-types-of-particulate-matter (accessed Jully 8, 2022).
8. World Health Organization · 2016
9. Global estimates of mortality associated with long-term exposure to outdoor fine particulate matter | Proceedings of the National Academy of Sciences. PNAS. https://www.pnas.org/doi/abs/10.1073/pnas.1803222115 (accessed July 8, 2022).
10. 10.1038/s12276-020-0405-110.1038/s12276-020-0405-1 ↗
11. 10.1021/acsnano.6b0855110.1021/acsnano.6b08551 ↗
12. Terzano C. · Eur. Rev. Med. Pharmacol. Sci. · 2010 · 14 · 809
13. 10.5194/acp-19-9399-201910.5194/acp-19-9399-2019 ↗
14. 10.1016/j.atmosenv.2016.01.00910.1016/j.atmosenv.2016.01.009 ↗
15. 10.1098/rspa.2018.049210.1098/rspa.2018.0492 ↗
16. 10.1021/acs.est.5b0245510.1021/acs.est.5b02455 ↗
17. project, T. W. A. Q. I. World-wide Air Quality Monitoring Data Coverage. aqicn.org. https://aqicn.org/sources/ (accessed July 8, 2022).
18. 10.1021/acs.est.9b0342510.1021/acs.est.9b03425 ↗
19. Beta Attenuation Technology for Particulate Matter Measurement - US. https://www.thermofisher.com/us/en/home/industrial/environmental/environmental-learning-center/air-quality-analysis-information/beta-attenuation-technology-particulate-matter-measurement.html (accessed July 8, 2022).
20. 10.1016/0021-8502(92)90492-E10.1016/0021-8502(92)90492-E ↗
21. 10.1016/j.envint.2016.12.00710.1016/j.envint.2016.12.007 ↗
22. Scanning Mobility Particle Sizer (Centre for Atmospheric Science - The University of Manchester). http://www.cas.manchester.ac.uk/restools/instruments/aerosol/scanning/ (accessed April 24, 2023).
23. 10.1016/j.envres.2022.11506110.1016/j.envres.2022.115061 ↗
24. ELPI+ - Analyzer for real-time aerosol measurements. Dekati Ltd. https://www.dekati.com/products/elpi/ (accessed April 24, 2023).
25. 10.1016/0021-8502(92)90004-F10.1016/0021-8502(92)90004-F ↗
26. MOUDI-II Impactors 120R, 122R, 125R. TSI.com. https://tsi.com/Products/Cascade-Impactors/MOUDI-II-Rotating-Impactors/MOUDI-II-Impactors-120R,122R,125R (accessed April 24, 2023).
27. Quartz Crystal Microbalance QCM MOUDI Impactor 140. TSI.com. https://tsi.com/Products/Cascade-Impactors/Real-Time-QCM-MOUDI/Quartz-Crystal-Microbalance-QCM-MOUDI-Impactor-140 (accessed April 24, 2023).
28. 10.1021/es402260210.1021/es4022602 ↗
29. 10.1038/s41377-018-0017-x10.1038/s41377-018-0017-x ↗
30. 10.1039/C8AN02157K10.1039/C8AN02157K ↗
31. 10.1109/ACCESS.2019.293077610.1109/ACCESS.2019.2930776 ↗
32. 10.1016/j.jhazmat.2021.12635110.1016/j.jhazmat.2021.126351 ↗
33. 10.1146/annurev-bioeng-092515-01084910.1146/annurev-bioeng-092515-010849 ↗
34. 10.1063/PT.3.369310.1063/PT.3.3693 ↗
35. 10.1038/lsa.2017.4610.1038/lsa.2017.46 ↗
36. 10.1021/acssensors.1c0062810.1021/acssensors.1c00628 ↗
37. 10.1364/OE.43175410.1364/OE.431754 ↗
38. 10.1364/OE.26.02567610.1364/OE.26.025676 ↗
39. 10.1038/srep4415710.1038/srep44157 ↗
40. 10.1021/acsnano.5b0038810.1021/acsnano.5b00388 ↗
41. 10.1038/nphoton.2012.33710.1038/nphoton.2012.337 ↗
42. 10.1038/lsa.2018.310.1038/lsa.2018.3 ↗
43. 10.1364/OE.27.03449610.1364/OE.27.034496 ↗
44. 10.1038/s41467-021-22271-410.1038/s41467-021-22271-4 ↗
45. 10.1021/acssensors.0c0198610.1021/acssensors.0c01986 ↗
46. 10.1016/j.sna.2022.11359110.1016/j.sna.2022.113591 ↗
47. 10.1002/adma.20180026210.1002/adma.201800262 ↗
48. 10.1021/nn502453h10.1021/nn502453h ↗
49. 10.1021/ja01014a01510.1021/ja01014a015 ↗
50. 10.1103/PhysRevLett.106.17550110.1103/PhysRevLett.106.175501 ↗
51. 10.1063/1.505145610.1063/1.5051456 ↗
52. Development, O. of R. & Performance Testing Protocols, Metrics, and Target Values for Fine Particulate Matter Air Sensors: Use in Ambient, Outdoor, Fixed Site, Non-Regulatory Supplemental and Informational Monitoring Applications. https://cfpub.epa.gov/si/si_public_record_Report.cfm?dirEntryId=350785&Lab=CEMM (accessed May 18, 2023).