journal article·2024-03Open access

Enhancing the light emission efficiency of LEDs based on array of Ag nanohollow cylinders and SPR theory

Bolin Zhu, Jun Zun, Liuli Qin

Optical Materials· Volume 149

Abstract

The internal spontaneous emission and external light extraction efficiency have been key issues in the research on LEDs incorporating metal nanoparticles , particularly in terms of transmittance, which presents a series of challenges and less-than-satisfactory outcomes. In this study, we address this issue by proposing a new approach that combines periodic structures with metal surface plasmons . Specifically, we embed an array of Ag nanohollow cylinders above the quantum wells of the LED structure and investigate its impact on the light emission characteristics using the finite-difference time-domain (FDTD) method. By varying the height and radius ratio of the hollow cylinders, the internal spontaneous emission and external light extraction efficiency of the LED can be significantly enhanced. At h = 12 nm, r/R = 1:3, the internal spontaneous emission rate is enhanced by a factor of 3.64. Under the condition of r/R = 1:3, the internal quantum efficiency reaches 90% for h values of 3 nm, 6 nm, 9 nm, 12 nm, and 15 nm. The transmittance increases from 0.26 to 0.44 at h = 3 nm, r/R = 1:3, and the enhancement factor of light extraction efficiency also reaches 1.73. These research findings reveal that embedding a nano Ag hollow cylinder array structure above the active layer can significantly enhance the light emission efficiency of LEDs. The introduction of this structure effectively utilizes the surface plasmon resonance effects of metal nanoparticles and their coupling with the active layer. This provides an important theoretical reference for further improvement and optimization of metal nanostructure designs.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: GaN-based semiconductor devices and materials · ZnO doping and properties · Plasmonic and Surface Plasmon Research

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (39)

Show source-provided references
1. TiO2-C nanocomposite synthesized via facile surfactant-assisted method as a part of less energy-consuming LED-based photocatalytic system for environmental applications10.1016/j.jphotochem.2022.114428 ↗
2. Indoor lighting techniques: an overview of evolution and new trends for energy saving10.1016/j.enbuild.2017.01.028 ↗
3. Efficiently releasing the Trapped energy flow in white organic light‐emitting diodes with Multifunctional Nanofunnel arrays10.1002/adfm.201500310 ↗
4. III-nitride photonic-crystal light-emitting diodes with high extraction efficiency10.1038/nphoton.2009.21 ↗
5. Study on the optical performance of thin-film light-emitting diodes using fractal micro-roughness surface model10.1016/j.apsusc.2017.03.041 ↗
6. Tunable surface plasmon-polariton resonance in organic light-emitting devices based on corrugated alloy electrodes10.29026/oea.2021.200024 ↗
7. Out-of-plane photoconductive and bulk photovoltaic effects in two-dimensional α-In2Se3/Ta2NiS5 ferroelectric heterojunctions
8. Photocatalytic water splitting kinetics of CMV model10.1142/S2010135X23500157 ↗
9. Surface plasmon enhanced blue organic light emitting diode with nearly 100% fluorescence efficiency10.1016/j.orgel.2012.05.018 ↗
10. Enhanced optoelectronic characteristics of MoS 2-based photodetectors through hybridization with CdS0. 42Se0. 58 nanobelt10.1142/S2010135X23450042 ↗
11. Microstructure, domain structure, ferroelectric and piezoelectric properties of textured bismuth-containing ceramics10.1142/S2010135X2350011X ↗
12. Metal nanoclusters/polyvinyl alcohol composite films as the alternatives for fabricating remote-type white light-emitting diodes10.3390/nano12020204 ↗
13. Creation of periodical domain structure by local polarization reversal in planar waveguide produced by soft proton exchange in LiNbO 310.1142/S2010135X23500200 ↗
14. Probing large area surface plasmon interference in thin metal films using photon scanning tunneling microscopy10.1016/j.ultramic.2003.11.018 ↗
15. Coupling localized and extended plasmons to improve the light extraction through metal films10.1364/OE.15.010533 ↗
16. Fabrication of GaN-air channels for embedded photonic structures10.1016/j.mssp.2022.107234 ↗
17. Enhanced surface and optical properties of colloidal silver nano-particles on GaN-based light-emitting diodes by a localized surface plasmon resonance effect using a low-cost metal-assisted chemical etching method10.1016/j.optcom.2019.06.023 ↗
18. Zinc oxide light-emitting diodes: a review10.1117/1.OE.58.1.010901 ↗
19. A novel application of plasmonics: plasmon‐driven surface‐catalyzed reactions10.1002/smll.201200572 ↗
20. Overview of the characteristics of micro-and nano-structured surface plasmon resonance sensors10.3390/s110201565 ↗
21. Recent energy targeted applications of localized surface plasmon resonance semiconductor nanocrystals: a mini-review
22. Toward high efficiency organic light‐emitting diodes: role of nanoparticles10.1002/adom.202001710 ↗
23. Interactions of π-conjugated polymers with inorganic nanocrystals10.1016/j.jphotochemrev.2014.05.001 ↗
24. Localized surface plasmon coupling Nanorods with Graphene as a transparent conductive electrode for micro light-emitting diodes10.1109/LED.2022.3217167 ↗
25. Optical constants of the noble metals10.1103/PhysRevB.6.4370 ↗
26. Enhanced light emission from large-area monolayer MoS2 using plasmonic nanodisc arrays10.1021/acs.nanolett.5b00407 ↗
27. Molecular design strategy for orange red thermally activated delayed fluorescence emitters in organic light‐emitting diodes (OLEDs)
28. Recent advances in OLED optical design10.1002/adfm.201808803 ↗
29. Enhancement in the excitonic spontaneous emission rates for Si nanocrystal multi-layers covered with thin films of Au, Ag, and Al10.1088/0957-4484/26/43/435701 ↗
30. Emergence of fermi's golden rule10.1103/PhysRevLett.129.140402 ↗
31. P-type conduction in Mg-doped GaN treated with low-energy electron beam irradiation (LEEBI)[J]10.1143/JJAP.28.L2112 ↗
32. Following interfacial kinetics in real time using broadband evanescent wave cavity-enhanced absorption spectroscopy: a comparison of light-emitting diodes and supercontinuum sources10.1039/B916712A ↗
33. The effect of sapphire substrates on omni-directional reflector design for flip-chip near-ultraviolet light-emitting diodes
34. Performance analysis of parallelized PSTD-FDTD method for large-scale electromagnetic simulation10.1016/j.cpc.2020.107631 ↗
35. Research on lighting system based on LED current and temperature spectrum model
36. Enhancing light extraction efficiency of GaN-based light-emitting diodes with reticulated photonic crystals10.1117/1.JNP.17.016005 ↗
37. Improved light extraction efficiency of GaN based blue light emitting diode using nano-scaled patterned sapphire substrate10.1166/jno.2019.2669 ↗
38. Titanium oxide nanotube arrays for high light extraction efficiency of GaN-based vertical light-emitting diodes10.1039/C6NR00503A ↗
39. Numerical investigation of light extraction efficiency of GaN-based vertical blue micron-scale light-emitting diode structures10.1166/jnn.2021.18944 ↗