journal article·2024-05-24

Nitrogen-Doped Carbon Dots as Ionizing Radiation Sensors in X-ray Dosimetry

Wandson dos Santos de Almeida, Lucas S. Lima, Luis M. G. Abegão, Fabio Assunção Andrade, Matheus Silveira, Susana Oliveira Souza, Francesco d’Errico, Eliana Midori Sussuchi

ACS Applied Nano Materials· Volume 7· Issue 10
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Abstract

This work explores the synthesis and application of nitrogen-doped carbon dots (N-CDs) obtained by a hydrothermal synthesis route using melamine and citric acid. It also discusses some characterizations and how carbon dots can be introduced into the Fricke solution to potentially serve as an ionizing radiation sensor while maintaining equivalent tissue dosimeter properties. The methodology for synthesis, preparation, and irradiation of the Fricke-N-CD suspensions is described and is simple and safe to execute. The results show that N-CDs have high sensitivity to X-ray radiation, presenting three linear regions with different sensitivity coefficients, −38.6 ± 2.7 Gy –1, −26.0 ± 0.9 Gy –1, and −15.4 ± 0.8 Gy –1, respectively, for the dose range of 0.0 to 100.0 Gy. The Fricke-N-CD suspension has good storage stability under room temperature conditions and a minimum detected dose of 0.25 Gy. Overall, this study provides valuable information about promising applications of carbon dots in X-ray dosimetry and the importance of further research in this area.
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Research context

OpenAlex topics: Carbon and Quantum Dots Applications · Luminescence and Fluorescent Materials · Luminescence Properties of Advanced Materials

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Research Group in Electrochemical Sensors and nano(Materials) - SEnM, Laboratory of Corrosion and Nanotechnology - LCNT, Graduate Program in Chemistry - Department of Chemistry, Federal University of Sergipe (UFS), Av. Marcelo Deda Chagas, 304, Rosa Elze, São Cristóvão/SE, CEP 49107-230, Brazil

Photonics Group, Institute of Physics, Federal University of Goiás (UFG), Av. Esperança, s/n - Campus Samambaia, Goiânia/GO, CEP 74690-900, Brazil

Oncology Center, Radiotherapy Sector, Hospital de Urgência de Sergipe, Av. Presidente Tancredo Neves, 7501, Aracaju/SE, CEP 49000-000, Brazil

Graduate Program in Physics, Federal University of Sergipe (UFS), Av. Marcelo Deda Chagas, 304, Rosa Elze, São Cristóvão/SE, CEP 49107-230, Brazil

Yale University, School of Medicine, 333 Cedar Street, New Haven, Connecticut 06510, United States

Università di Pisa, Scuola di Ingegneria, Via Girolamo Caruso, 16, Pisa, CEP 56122, Italy

Funding

Coordena??o de Aperfei?oamento de Pessoal de N?vel Superior

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