journal article·2019-08-23Open access

Mass fabrication and superior microwave absorption property of multilayer graphene/hexagonal boron nitride nanoparticle hybrids

Yongqing Bai, Bo Zhong, Yuanlie Yu, Meng Wang, Jing Zhang, Bin Zhang, Kaixiong Gao, Aimin Liang, Chunyu Wang, Junyan Zhang

Abstract

Abstract Graphene has been regarded as a promising candidate in microwave absorption field but still faces some major challenges, including the limitation of mass production and poor impedance matching. Here, we demonstrate a simple approach to fabricate multilayer graphene in a kilo-mass/hour (≥2.5 kg/h) scale through an oxidation-thermal expansion-air convection shearing process. The subsequent incorporation of hexagonal boron nitride nanoparticles (h-BNNPs) can effectively tailor the dielectric and magnetic properties of the as-obtained multilayer graphene, which can significantly boost its microwave absorption performance. The as-obtained multilayer graphene/h-BNNP hybrid with 40 wt.% of h-BNNPs, exhibits extremely low reflection loss value of −67.35 dB at 8.04 GHz when the absorber thickness is 3.29 mm, ranking it as one of the most attractive absorbers reported to date. Moreover, the multilayer graphene/h-BNNP hybrids possess low densities less than 0.45 g/cm3, making them very attractive for practical microwave absorption application.
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Research context

OpenAlex topics: Electromagnetic wave absorption materials · Advanced Antenna and Metasurface Technologies · Metamaterials and Metasurfaces Applications

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