journal article·2023-06-09Open access

Interplay of Thermal and Electronic Effects in the Mott Transition of Nanosized VO2 Phase Change Memory Devices

László Pósa, Péter Hornung, Tímea Nóra Török, Sebastian Werner Schmid, Sadaf Arjmandabasi, György Molnár, Zsófia Baji, Goran Dražić, András Halbritter, János Volk

ACS Applied Nano Materials· Volume 6· Issue 11

Abstract

Volatile memory devices relying on the Mott-type insulator-to-metal transition of vanadium oxide (VO 2 ) are widely utilized in the field of neuromorphic computing.Such devices, however, are realized in a nanoscale geometry, where the switching relies on the self-heating of an ultrasmall spot as well as the presence of extremely high electric fields in the active region.In this paper, we investigate the interplay of such nanoscale thermal and nonlinear electronic phenomena by investigating the temperature and voltage dependent conduction properties of our customdesigned VO 2 devices, where a V-shaped electrode focuses the switching to an ultrasmall single-spot active region.This simplified spatial structure of the active volume facilitates the device modeling and the identification of physical mechanisms behind the phase transition.We find that purely thermal or electronic effects fail to describe the device operation, however, according to our finite element simulations, a combined electronic and thermal model provides a precise description of the device characteristics.These results facilitate the understanding as well as the thermal and electronic design of novel VO 2 -based neuronal devices.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Advanced Memory and Neural Computing · Transition Metal Oxide Nanomaterials · Perovskite Materials and Applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Institute of Technical Physics and Materials Science, Centre for Energy Research, Konkoly-Thege M. út 29-33, 1121 Budapest, Hungary

Department of Physics, Institute of Physics, Budapest University of Technology and Economics, Műegyetem rkp. 3., H-1111 Budapest, Hungary

Department of Materials Chemistry, National Institute of Chemistry, Hajdrihova 19, SI-1000 Ljubljana, Slovenia

ELKH-BME Condensed Matter Research Group, Budapest University of Technology and Economics, Műegyetem rkp. 3., H-1111 Budapest, Hungary

Funding

Nemzeti Kutat?si Fejleszt?si ?s Innov?ci?s Hivatal · Innov?ci?s ?s Technol?giai Miniszt?rium · Ministry of Culture and Innovation

References (63)

Show source-provided references
1. 10.1021/acs.nanolett.0c0263810.1021/acs.nanolett.0c02638 ↗
2. 10.1126/sciadv.160269710.1126/sciadv.1602697 ↗
3. 10.1038/s41467-022-29456-510.1038/s41467-022-29456-5 ↗
4. 10.1021/nl900676n10.1021/nl900676n ↗
5. 10.1002/adma.20100286810.1002/adma.201002868 ↗
6. 10.1080/10408436.2012.71913110.1080/10408436.2012.719131 ↗
7. 10.1038/ncomms881210.1038/ncomms8812 ↗
8. 10.1038/ncomms1010410.1038/ncomms10104 ↗
9. 10.1038/s41467-018-07052-w10.1038/s41467-018-07052-w ↗
10. 10.1038/s41586-019-1159-610.1038/s41586-019-1159-6 ↗
11. 10.1021/acs.nanolett.0c0289210.1021/acs.nanolett.0c02892 ↗
12. 10.3389/fnins.2021.62825410.3389/fnins.2021.628254 ↗
13. 10.1016/j.sse.2019.10772910.1016/j.sse.2019.107729 ↗
14. 10.1021/acs.nanolett.9b0155410.1021/acs.nanolett.9b01554 ↗
15. 10.1103/PhysRevApplied.17.02402810.1103/PhysRevApplied.17.024028 ↗
16. 10.1073/pnas.210589511810.1073/pnas.2105895118 ↗
17. 10.1039/C9NR08364B10.1039/C9NR08364B ↗
18. 10.1038/s41467-022-31747-w10.1038/s41467-022-31747-w ↗
19. 10.1038/s41928-022-00812-z10.1038/s41928-022-00812-z ↗
20. 10.1126/science.abd908810.1126/science.abd9088 ↗
21. 10.1103/PhysRevB.104.16514110.1103/PhysRevB.104.165141 ↗
22. 10.1063/5.009324210.1063/5.0093242 ↗
23. 10.1038/s41467-020-16752-110.1038/s41467-020-16752-1 ↗
24. 10.1038/srep3077510.1038/srep30775 ↗
25. 10.3390/nano1101021210.3390/nano11010212 ↗
26. 10.1088/0953-8984/26/1/01560110.1088/0953-8984/26/1/015601 ↗
27. 10.1021/acsami.7b0562010.1021/acsami.7b05620 ↗
28. 10.1021/acsami.8b1787910.1021/acsami.8b17879 ↗
29. 10.1016/j.mee.2019.11105710.1016/j.mee.2019.111057 ↗
30. 10.1039/D0CP01929A10.1039/D0CP01929A ↗
31. 10.1038/s41535-022-00479-x10.1038/s41535-022-00479-x ↗
32. 10.1088/0957-4484/23/20/20520110.1088/0957-4484/23/20/205201 ↗
33. 10.1063/1.325964910.1063/1.3259649 ↗
34. 10.1103/PhysRevLett.110.05660110.1103/PhysRevLett.110.056601 ↗
35. 10.1063/1.343546610.1063/1.3435466 ↗
36. 10.1109/TED.2018.285918010.1109/TED.2018.2859180 ↗
37. 10.1109/TED.2018.285918810.1109/TED.2018.2859188 ↗
38. 10.1021/acsami.6b0350110.1021/acsami.6b03501 ↗
39. 10.1103/PhysRevB.98.19514410.1103/PhysRevB.98.195144 ↗
40. 10.1063/1.490380610.1063/1.4903806 ↗
41. 10.1016/j.jpcs.2010.03.03210.1016/j.jpcs.2010.03.032 ↗
42. 10.1007/s10853-009-3442-710.1007/s10853-009-3442-7 ↗
43. 10.1063/1.481772710.1063/1.4817727 ↗
44. 10.1038/nnano.2014.7110.1038/nnano.2014.71 ↗
45. 10.1063/1.361980610.1063/1.3619806 ↗
46. 10.1063/1.492194910.1063/1.4921949 ↗
47. 10.1063/1.305046410.1063/1.3050464 ↗
48. 10.1063/1.324533810.1063/1.3245338 ↗
49. 10.1063/5.008693210.1063/5.0086932 ↗
50. 10.1103/PhysRevB.61.1036110.1103/PhysRevB.61.10361 ↗
51. 10.1038/nmat496710.1038/nmat4967 ↗
52. 10.1103/PhysRevLett.105.14640410.1103/PhysRevLett.105.146404 ↗
53. 10.1103/PhysRevB.82.20511010.1103/PhysRevB.82.205110 ↗
54. 10.1021/acsnano.9b0339710.1021/acsnano.9b03397 ↗
55. 10.1016/j.sse.2011.04.00310.1016/j.sse.2011.04.003 ↗
56. 10.1039/C7NR05348G10.1039/C7NR05348G ↗
57. 10.1038/s41598-019-45436-010.1038/s41598-019-45436-0 ↗
58. 10.1155/2013/68258610.1155/2013/682586 ↗
59. 10.1063/1.339401610.1063/1.3394016 ↗
60. 10.1016/j.apsusc.2013.06.01610.1016/j.apsusc.2013.06.016 ↗
61. 10.1039/C9NR08803B10.1039/C9NR08803B ↗
62. 10.3938/jkps.62.113410.3938/jkps.62.1134 ↗
63. 10.3390/coatings1005045310.3390/coatings10050453 ↗