Anomalous Nernst effect beyond the magnetization scaling relation in the ferromagnetic Heusler compound Co2MnGa

Abstract Applying a temperature gradient in a magnetic material generates a voltage that is perpendicular to both the heat flow and the magnetization. This phenomenon is the anomalous Nernst effect (ANE), which was long thought to be proportional to the value of the magnetization. However, more generally, the ANE has been predicted to originate from a net Berry curvature of all bands near the Fermi level (E_F). Subsequently, a large anomalous Nernst thermopower ($${\boldsymbol{S}}_{{\boldsymbol{yx}}}^{\boldsymbol{A}}$$) has recently been observed in topological materials with no net magnetization but a large net Berry curvature [Ω_n(k)] around E_F. These experiments clearly fall outside the scope of the conventional magnetization model of the ANE, but a significant question remains. Can the value of the ANE in topological ferromagnets exceed the highest values observed in conventional ferromagnets? Here, we report a remarkably high $${\boldsymbol{S}}_{{\boldsymbol{yx}}}^{\boldsymbol{A}}$$-value of ~6.0 µV K⁻¹ in the ferromagnetic topological Heusler compound Co₂MnGa at room temperature, which is approximately seven times larger than any anomalous Nernst thermopower value ever reported for a conventional ferromagnet. Combined electrical, thermoelectric, and first-principles calculations reveal that this high-value of the ANE arises from a large net Berry curvature near the Fermi level associated with nodal lines and Weyl points.