Detection of cathode agglomerates in batteries applying laser infrared thermography
Source abstract
Abstract
The key to enhancing the cost-effectiveness of the lithium-ion production process is reducing the scrap rate of cells earlier in production. Defective or under-performing cells are detected during the formation or aging steps. The performance of these cells is influenced by earlier production stages, with the coating and calendering processes being crucial steps where quality control is most important. This motivates the use of inline measurement techniques at this stage. Laser thermography is a powerful measurement method that can detect surface and subsurface defects or geometric deviations. This study focuses on the use of a relatively new non-destructive testing technique, named laser infrared thermography (L-IRT), to identify defect types aggregated in cathode electrode sheets. The object movement is simulated using a rotating roll. The data is reconstructed and evaluated using common active thermography evaluation methods, such as the gradient method, thermal signal reconstruction, and pulse phase thermography. The results were analyzed both qualitatively and quantitatively using the signal-to-noise ratio and contrast-to-noise ratio. Here the gradient method showed the highest metrics. Further, in a non-calendered electrode sheet a distinct pattern was made visible using laser infrared thermography, which allows in the future optimisations of the slot die based on laser infrared thermography measurements.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Advanced Battery Technologies Research · Thermography and Photoacoustic Techniques · Molten salt chemistry and electrochemical processes
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
References (56)
Show source-provided references
1. A review of current automotive battery technology and future prospects10.1177/0954407013485567 ↗
2. Electrochemical performance of lini0.5mn1.5o4 cathode material for lithium-ion batteries10.1149/1.1652053 ↗
3. Acoustic emission technique for battery health monitoring: Comprehensive literature review10.3390/batteries11010014 ↗
4. Review on surface engineering of NMC for high performance of lithium-ion batteries10.55713/jmmm.v35i2.2338 ↗
5. Research progress on cathode materials for lithium-ion batteries10.1007/s10008-025-06293-2 ↗
6. Enhancing the electrochemical performance of nickel-rich layered cathode material (NMC622) for lithium-ion batteries by ultrathin conductive ceria-surface coatig10.1002/ejic.202400689 ↗
7. 3D lithium-metal anode for high-energy lithium-metal batteries
8. Lithium-based batteries, history, current status, challanges, and future perspectives10.1002/bte2.20230030 ↗
9. Pushing the energy-lifetime frontier of li-ion batteries: Study of Ni-rich, co-free NMAW cathode material
10. Reichweite, Sicherheit, Lebensdauer—Batterierohstoffe und ihre technische Relevanz10.1007/s35658-022-1418-4 ↗
11. Produktionsprozess einer Lithium-Ionen-Batteriezelle
12. Dahmen · 2024
13. Tracking flows of end-of-life battery materials and manufacturing scrap10.3390/batteries9070360 ↗
14. Effect of electrode manufacturing defects on electrochemical performance of lithium-ion batteries: Cognizance of the battery failure sources10.1016/j.jpowsour.2016.02.007 ↗
15. Coating defects of lithium-ion battery electrodes and their inline detection and tracking10.3390/batteries9020111 ↗
16. Influence of metallic contaminants on the electrochemical and thermal behavior of Li-ion electrodes10.1016/j.jpowsour.2021.230760 ↗
17. Challenges in lithium-ion battery slurry preparation and potential of modifying electrode structures by different mixing processes10.1002/ente.201402218 ↗
18. Electrode manufacturing for lithium-ion batteries—Analysis of current and next generation processing10.1016/j.est.2019.100862 ↗
19. Kampker · 2014
20. Identifying degradation mechanisms in lithium-ion batteries with coating defects at the cathode10.1016/j.apenergy.2018.09.073 ↗
21. Significant agglomeration of conductive materials and the dispersion state change of the Ni-rich NMC-based cathode slurry during storage10.1021/acs.iecr.1c04205 ↗
22. Thermographic detection of surface breaking defects using a laser scanner source10.1016/j.ndteint.2011.06.001 ↗
23. Use of line laser scanning thermography for the defect detection and evaluation of composite material10.1515/secm-2022-0007 ↗
24. Active thermography for in-situ defect detection in laser powder bed fusion of metal10.1016/j.jmapro.2024.09.085 ↗
25. Lithium-ion battery electrode inspection using pulse thermography10.1016/j.ndteint.2014.02.006 ↗
26. Non-destructive evaluation of slot-die-coated lithium secondary battery electrodes by in-line laser caliper and IR thermography methods10.1039/C3AY41140K ↗
27. Partikeldetektion auf Elektroden für Lithium-Ionen-Batterien mit laserangeregter Thermografie
28. Detection of anode coating defects in batteries electrode production and their effect on cell performance10.1007/s10921-025-01208-7 ↗
29. Gradient-based image generation for thermographic material inspection10.1016/j.applthermaleng.2025.125900 ↗
30. Linear laser fast scanning thermography NDT for artificial disbond defects in thermal barrier coatings10.1364/OE.25.031789 ↗
31. Infrared thermography
32. Active thermography
33. Aktuelle Anwendungen der Laser-Thermografie
34. A pilot study using flying spot laser thermography and signal reconstruction10.1016/j.optlaseng.2025.108901 ↗
35. Zerstörungsfreie Prüfung durch aktive Thermografie im kontinuierlichen Bauteildurchlauf
36. Thiemann · 2015
37. Defect detection in ceramic materials by quantitative infrared thermography
38. Ibarra-Castanedo C, Bendada A, Maldague X. Thermographic Image Processing for NDT. In: Asociación Argentina de Ensayos No Destructivos y Estructurales. Buenos Aires; 2007, p. 1–12.
39. Ibarra-Castanedo C, et al. Thermographic nondestructive evaluation: overview of recent progress. In: AeroSense 2003. Orlando, FL; 2003, p. 450–9. http://dx.doi.org/10.1117/12.485699.10.1117/12.485699 ↗
40. A brief review and advances of thermographic image-processing methods for IRT inspection: A case study on GFRP plate10.1007/s40799-020-00414-4 ↗
41. Popow V, Budesheim L, Gurka M. Zerstörungsfreie Prüfung von faserverstärkten Kunststoffen mittels Impuls-Thermographie – Gegenüberstellung und Bewertung verschiedener Auswertealgorithmen, booktitle=Thermografie-Kolloquium. Berlin; 2017.
42. Active thermography data-processing algorithm for nondestructive testing of materials10.1109/ACCESS.2020.3025329 ↗
43. Olafsson G. Pulsethermography. GitHub Repository, [Accessed 26 December 2024].
44. Latest advances in common signal processing of pulsed thermography for enhanced detectability: A review10.3390/app112412168 ↗
45. Recent advances in active infrared thermography for non-destructive testing of aerospace components10.3390/s18020609 ↗
46. Improving the probing depth of thermographic inspections of polymer composite materials10.1088/1361-6501/aaed15 ↗
47. Improvement of the detection of defects by pulse thermography thanks to the TSR approach in the case of a smart composite repair patch10.3166/qirt.7.167-187 ↗
48. Development and application of infrared thermography non-destructive testing techniques10.3390/s20143851 ↗
49. Conduction of heat in solids
50. S. Pham Tu Quoc · 2014
51. Thermal failure analysis by IR lock-in thermography
52. Fertigungsverfahren von Lithium-Ionen-Zellen und -Batterien
53. Pulvertechnisch hergestellte werkstoffe fuer die elektromobilitaet — Teil 1: Batterien
54. Separatoren
55. Investigating the moisture sensitivity of nickel-rich cathodes in lithium-ion battery production: Implications for production atmospheres and cost reduction
56. Identification of critical moisture exposure for nickel-rich cathode active materials in lithium-ion battery production10.1016/j.jpowsour.2024.235661 ↗