journal article·2023-11-10

Fe-Doped SnS2 Nanoflowers for Magnetically-Tunable Photoelectrocatalytic Hydrogen Evolution Reaction

Yugao Hu, Tingting Bo, Ruixin Xu, Nan Mu, Yanyu Liu, Wei Zhou

ACS Applied Nano Materials· Volume 6· Issue 21
Publisher page

Abstract

Because of its excellent optical and electrical properties, SnS 2 has been widely used in solar cells, photocatalysis, and other fields. Here, a Fe-doped SnS 2 nanoflower with room temperature ferromagnetism was constructed to investigate the effect of Fe doping and an external magnetic field on the photoelectric catalytic hydrogen production of water splitting. Enhanced visible-light absorption and electrical conductivity were observed in Fe-doped SnS 2, thereby enhancing its photoelectrocatalytic hydrogen production performance. Moreover, the application of an external magnetic field leads to a negative potential shift, resulting in a decreased photocurrent response for Fe-doped SnS 2 . In addition, the first-principles calculations also indicate the origin of the magnetic properties and improved catalytic activity of a SnS 2 nanoflower with Fe doping.
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Research context

OpenAlex topics: Advanced Photocatalysis Techniques · Copper-based nanomaterials and applications · Quantum Dots Synthesis And Properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Applied Physics, Tianjin Key Laboratory of Low Dimensional Materials Physics and Preparing Technology, School of Science, Tianjin University, Tianjin 300072, P. R. China

College of Physics and Materials Science, Tianjin Normal University, Tianjin 300387, P. R. China

Funding

National Natural Science Foundation of China

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