journal article·2026-04-20Open access

Sub-wavelength extreme ultraviolet microscopy reveals domain-wall stability during ultrafast demagnetization

Hung-Tzu Chang, Sergey Zayko, Timo Schmidt, Ofer Kfir, Murat Sivis, Johan H. Mentink, Manfred Albrecht, Claus Ropers

Abstract

Abstract Ultrafast control of magnetic textures relies on understanding how domain walls respond to femtosecond laser excitation. Previous X-ray scattering studies suggested transient domain-wall broadening and motion during reversible demagnetization. Yet such dynamics have never been observed directly, owing to insufficient spatiotemporal resolution in existing techniques. Here we introduce femtosecond extreme ultraviolet microscopy with sub-wavelength 13.5-nm spatial resolution, enabling direct real-space imaging of domains in ferri- and ferromagnetic thin films during laser-induced demagnetization. Within an experimental precision better than 2 nm, domain-wall positions and widths remain unchanged up to the onset of irreversible magnetic switching at 50%–80% demagnetization. These findings establish quantitative limits for reversible domain-wall motion and spin transport upon ultrafast demagnetization, while implying that irreversible reconfiguration underlies characteristic changes in diffraction signatures at high fluence. The approach expands time-resolved microscopy into the nanometre and femtosecond regime, enabling element-specific studies of coupled spin, charge and lattice dynamics in quantum and functional materials.
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Magnetic properties of thin films · Advanced X-ray Imaging Techniques · Chemical and Physical Properties of Materials

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (68)

Show source-provided references
1. Beaurepaire, E., Merle, J.-C., Daunois, A. & Bigot, J.-Y. Ultrafast spin dynamics in ferromagnetic nickel. Phys. Rev. Lett. 76, 4250–4253 (1996).10.1103/PhysRevLett.76.4250 ↗
2. Kirilyuk, A., Kimel, A. V. & Rasing, T. Ultrafast optical manipulation of magnetic order. Rev. Mod. Phys. 82, 2731–2784 (2010).10.1103/RevModPhys.82.2731 ↗
3. Parkin, S. S. P., Hayashi, M. & Thomas, L. Magnetic domain-wall racetrack memory. Science 320, 190–194 (2008).10.1126/science.1145799 ↗
4. Fert, A., Reyren, N. & Cros, V. Magnetic skyrmions: advances in physics and potential applications. Nat. Rev. Mater. 2, 17031 (2017).10.1038/natrevmats.2017.31 ↗
5. Kimel, A. V. & Li, M. Writing magnetic memory with ultrashort light pulses. Nat. Rev. Mater. 4, 189–200 (2019).10.1038/s41578-019-0086-3 ↗
6. Koopmans, B. et al. Explaining the paradoxical diversity of ultrafast laser-induced demagnetization. Nat. Mater. 9, 259–265 (2010).10.1038/nmat2593 ↗
7. Dornes, C. et al. The ultrafast Einstein–de Haas effect. Nature 565, 209–212 (2019).10.1038/s41586-018-0822-7 ↗
8. Tauchert, S. R. et al. Polarized phonons carry angular momentum in ultrafast demagnetization. Nature 602, 73–77 (2022).10.1038/s41586-021-04306-4 ↗
9. Battiato, M., Carva, K. & Oppeneer, P. M. Superdiffusive spin transport as a mechanism of ultrafast demagnetization. Phys. Rev. Lett. 105, 027203 (2010).10.1103/PhysRevLett.105.027203 ↗
10. Melnikov, A. et al. Ultrafast transport of laser-excited spin-polarized carriers in Au/Fe/MgO (001). Phys. Rev. Lett. 107, 076601 (2011).10.1103/PhysRevLett.107.076601 ↗
11. Suturin, S. M. et al. Short nanometer range optically induced magnetic fluctuations accompanying ultrafast demagnetization of nanoscale ferromagnetic domains. Phys. Rev. B 108, 174444 (2023).10.1103/PhysRevB.108.174444 ↗
12. Pfau, B. et al. Ultrafast optical demagnetization manipulates nanoscale spin structure in domain walls. Nat. Commun. 3, 1100 (2012).10.1038/ncomms2108 ↗
13. Zusin, D. et al. Ultrafast perturbation of magnetic domains by optical pumping in a ferromagnetic multilayer. Phys. Rev. B 106, 144422 (2022).10.1103/PhysRevB.106.144422 ↗
14. Hennes, M. et al. Laser-induced ultrafast demagnetization and perpendicular magnetic anisotropy reduction in a Co88Tb12 thin film with stripe domains. Phys. Rev. B 102, 174437 (2020).10.1103/PhysRevB.102.174437 ↗
15. Fan, G. et al. Ultrafast magnetic scattering on ferrimagnets enabled by a bright Yb-based soft X-ray source. Optica 9, 399–407 (2022).10.1364/OPTICA.443440 ↗
16. Zhou Hagström, N. et al. Symmetry-dependent ultrafast manipulation of nanoscale magnetic domains. Phys. Rev. B 106, 224424 (2022).10.1103/PhysRevB.106.224424 ↗
17. Jangid, R. et al. Extreme domain wall speeds under ultrafast optical excitation. Phys. Rev. Lett. 131, 256702 (2023).10.1103/PhysRevLett.131.256702 ↗
18. Schryer, N. L. & Walker, L. R. The motion of 180° domain walls in uniform d.c. magnetic fields. J. Appl. Phys. 45, 5406–5421 (1974).10.1063/1.1663252 ↗
19. Baláž, P., Carva, K., Ritzmann, U., Maldonado, P. & Oppeneer, P. M. Domain wall dynamics due to femtosecond laser-induced superdiffusive spin transport. Phys. Rev. B 101, 174418 (2020).10.1103/PhysRevB.101.174418 ↗
20. Weder, D. et al. Transient magnetic gratings on the nanometer scale. Struct. Dyn. 7, 054501 (2020).10.1063/4.0000017 ↗
21. Kerber, N. et al. Faster chiral versus collinear magnetic order recovery after optical excitation revealed by femtosecond XUV scattering. Nat. Commun. 11, 6304 (2020).10.1038/s41467-020-19613-z ↗
22. Léveillé, C. et al. Ultrafast time-evolution of chiral Néel magnetic domain walls probed by circular dichroism in X-ray resonant magnetic scattering. Nat. Commun. 13, 1412 (2022).10.1038/s41467-022-28899-0 ↗
23. Girardi, D. et al. Three-dimensional spin-wave dynamics, localization and interference in a synthetic antiferromagnet. Nat. Commun. 15, 3057 (2024).10.1038/s41467-024-47339-9 ↗
24. Butcher, T. A. et al. Nanoscale domain-wall dynamics in micromagnetic structures with weak perpendicular anisotropy. Phys. Rev. B 111, L220409 (2024).10.1103/2y4r-my27 ↗
25. Donnelly, C. et al. Time-resolved imaging of three-dimensional nanoscale magnetization dynamics. Nat. Nanotechnol. 15, 356–360 (2020).10.1038/s41565-020-0649-x ↗
26. Weigand, M. et al. TimeMaxyne: a shot-noise limited, time-resolved pump-and-probe acquisition system capable of 50 GHz frequencies for synchrotron-based X-ray microscopy. Crystals 12, 1029 (2022).10.3390/cryst12081029 ↗
27. Büttner, F. et al. Dynamics and inertia of skyrmionic spin structures. Nat. Phys. 11, 225–228 (2015).10.1038/nphys3234 ↗
28. Baumgartner, M. et al. Spatially and time-resolved magnetization dynamics driven by spin–orbit torques. Nat. Nanotechnol. 12, 980–986 (2017).10.1038/nnano.2017.151 ↗
29. Battistelli, R. et al. Coherent X-ray magnetic imaging with 5 nm resolution. Optica 11, 234–237 (2024).10.1364/OPTICA.505999 ↗
30. Butcher, T. A. et al. Ptychographic nanoscale imaging of the magnetoelectric coupling in freestanding BiFeO3. Adv. Mater. 36, 2311157 (2024).10.1002/adma.202311157 ↗
31. Rana, A. et al. Three-dimensional topological magnetic monopoles and their interactions in a ferromagnetic meta-lattice. Nat. Nanotechnol. 18, 227–232 (2023).10.1038/s41565-022-01311-0 ↗
32. Mayr, S. et al. Time-resolved X-ray imaging of nanoscale spin-wave dynamics at multi-GHz frequencies using low-alpha synchrotron operation. Appl. Phys. Rev. 11, 041411 (2024).10.1063/5.0206576 ↗
33. Rubiano da Silva, N. et al. Nanoscale mapping of ultrafast magnetization dynamics with femtosecond Lorentz microscopy. Phys. Rev. X 8, 031052 (2018).
34. Möller, M., Gaida, J. H., Schäfer, S. & Ropers, C. Few-nm tracking of current-driven magnetic vortex orbits using ultrafast Lorentz microscopy. Commun. Phys. 3, 36 (2020).10.1038/s42005-020-0301-y ↗
35. Harvey, T. R. et al. Ultrafast electron microscopy for probing magnetic dynamics. MRS Bull. 46, 711–719 (2021).10.1557/s43577-021-00166-5 ↗
36. Miyamachi, T., Sürgers, C. & Wulfhekel, W. Resolving the spin polarization and magnetic domain wall width of (Nd,Dy)2Fe14B with spin-polarized scanning tunneling microscopy. Appl. Phys. Express 14, 115504 (2021).10.35848/1882-0786/ac2a56 ↗
37. Liang, K., Bi, L., Zhu, Q., Zhou, H. & Li, S. Ultrafast dynamics revealed with time-resolved scanning tunneling microscopy: a review. ACS Appl. Opt. Mater. 1, 924–938 (2023).10.1021/acsaom.2c00169 ↗
38. Liu, C. et al. Correlated spin-wave generation and domain-wall oscillation in a topologically textured magnetic film. Nat. Mater. 24, 406–413 (2025).10.1038/s41563-024-02085-7 ↗
39. von Korff Schmising, C. et al. Imaging ultrafast demagnetization dynamics after a spatially localized optical excitation. Phys. Rev. Lett. 112, 217203 (2014).10.1103/PhysRevLett.112.217203 ↗
40. Kfir, O. et al. Nanoscale magnetic imaging using circularly polarized high-harmonic radiation. Sci. Adv. 3, eaao4641 (2017).10.1126/sciadv.aao4641 ↗
41. Zayko, S. et al. Ultrafast high-harmonic nanoscopy of magnetization dynamics. Nat. Commun. 12, 6337 (2021).10.1038/s41467-021-26594-0 ↗
42. Zayko, S. et al. A dynamical symmetry triad in high-harmonic generation revealed by attosecond recollision control. New J. Phys. 22, 053017 (2020).10.1088/1367-2630/ab82bd ↗
43. Siddiqui, S. A., Han, J., Finley, J. T., Ross, C. A. & Liu, L. Current-induced domain wall motion in a compensated ferrimagnet. Phys. Rev. Lett. 121, 057701 (2018).10.1103/PhysRevLett.121.057701 ↗
44. Hubert, A. & Schäfer, R. Magnetic Domains: The Analysis of Magnetic Microstructures (Springer Science & Business Media, 1998).
45. Lemesh, I., Büttner, F. & Beach, G. S. D. Accurate model of the stripe domain phase of perpendicularly magnetized multilayers. Phys. Rev. B 95, 174423 (2017).10.1103/PhysRevB.95.174423 ↗
46. Birch, M. T. et al. History-dependent domain and skyrmion formation in 2D van der Waals magnet Fe3GeTe2. Nat. Commun. 13, 3035 (2022).10.1038/s41467-022-30740-7 ↗
47. Albisetti, E. & Petti, D. Domain wall engineering through exchange bias. J. Magn. Magn. Mater. 400, 230–235 (2016).10.1016/j.jmmm.2015.07.009 ↗
48. Graves, C. E. et al. Nanoscale spin reversal by non-local angular momentum transfer following ultrafast laser excitation in ferrimagnetic GdFeCo. Nat. Mater. 12, 293–298 (2013).10.1038/nmat3597 ↗
49. Seifert, T. S., Cheng, L., Wei, Z., Kampfrath, T. & Qi, J. Spintronic sources of ultrashort terahertz electromagnetic pulses. Appl. Phys. Lett. 120, 180401 (2022).10.1063/5.0080357 ↗
50. Medapalli, R. et al. Multiscale dynamics of helicity-dependent all-optical magnetization reversal in ferromagnetic Co/Pt multilayers. Phys. Rev. B 96, 224421 (2017).10.1103/PhysRevB.96.224421 ↗
51. Quessab, Y. et al. Helicity-dependent all-optical domain wall motion in ferromagnetic thin films. Phys. Rev. B 97, 054419 (2018).10.1103/PhysRevB.97.054419 ↗
52. Prabhakara, K. H. et al. Study of domain wall dynamics in GdFeCo using double high-speed photography. Phys. Solid State 64, 547–553 (2022).10.1134/S1063783422110105 ↗
53. Khusyainov, D. et al. Texture-dependent all-optical switching in ferromagnetic films via stochastic nucleation of nanoscale domains. Nat. Mater. https://doi.org/10.1038/s41563-026-02515-8 (2026).10.1038/s41563-026-02515-8 ↗
54. Metternich, D. et al. Picosecond localization dynamics following ultrafast nanoscale magnetic switching. Preprint at https://arxiv.org/abs/2512.17643 (2025).
55. Koshibae, W. & Nagaosa, N. Creation of skyrmions and antiskyrmions by local heating. Nat. Commun. 5, 5148 (2014).10.1038/ncomms6148 ↗
56. Je, S.-G. et al. Creation of magnetic skyrmion bubble lattices by ultrafast laser in ultrathin films. Nano Lett. 18, 7362–7371 (2018).10.1021/acs.nanolett.8b03653 ↗
57. Büttner, F. et al. Observation of fluctuation-mediated picosecond nucleation of a topological phase. Nat. Mater. 20, 30–37 (2021).10.1038/s41563-020-00807-1 ↗
58. Juge, R. et al. Skyrmions in synthetic antiferromagnets and their nucleation via electrical current and ultra-fast laser illumination. Nat. Commun. 13, 4807 (2022).10.1038/s41467-022-32525-4 ↗
59. Steinbach, F. et al. Exploring the fundamental spatial limits of magnetic all-optical switching. Nano Lett. 24, 6865–6871 (2024).10.1021/acs.nanolett.4c00129 ↗
60. Hariki, A. et al. X-ray magnetic circular dichroism in altermagnetic α-MnTe. Phys. Rev. Lett. 132, 176701 (2024).10.1103/PhysRevLett.132.176701 ↗
61. Stinson, H. T. et al. Imaging the nanoscale phase separation in vanadium dioxide thin films at terahertz frequencies. Nat. Commun. 9, 3604 (2018).10.1038/s41467-018-05998-5 ↗
62. Johnson, A. S. et al. Ultrafast X-ray imaging of the light-induced phase transition in VO2. Nat. Phys. 19, 215–220 (2023).
63. Heinrich, T. et al. Electronic and structural fingerprints of charge-density-wave excitations in extreme ultraviolet transient absorption spectroscopy. Phys. Rev. X 13, 021033 (2023).
64. Domröse, T. & Ropers, C. Femtosecond trimer quench in the unconventional charge-density-wave material $$1{{\rm{T}}}^{{\prime} }-{\mathrm{TaTe}}2$$. Phys. Rev. B 110, 085155 (2024).10.1103/PhysRevB.110.085155 ↗
65. Raines, K. S. et al. Three-dimensional structure determination from a single view. Nature 463, 214–217 (2010).10.1038/nature08705 ↗
66. Luke, D. R. Relaxed averaged alternating reflections for diffraction imaging. Inverse Probl. 21, 37–50 (2005).10.1088/0266-5611/21/1/004 ↗
67. Fienup, J. R. Reconstruction of an object from the modulus of its Fourier transform. Opt. Lett. 3, 27–29 (1978).10.1364/OL.3.000027 ↗
68. Clark, J. N., Huang, X., Harder, R. & Robinson, I. K. High-resolution three-dimensional partially coherent diffraction imaging. Nat. Commun. 3, 993 (2012).10.1038/ncomms1994 ↗