journal article·2026-04

Nonlinear phase-matched van der Waals crystals integrated on optical fibres

Kaifeng Lin, Guangjie Yao, Jiahui Shao, Yilong You, Jiajie Qi, Daopeng Yuan, Yijun Wang, Muhong Wu, Lingjun Kong, Xiangdong Zhang, Enge Wang, Zhipei Sun, Hao Hong, Kaihui Liu

Nature Materials· Volume 25· Issue 4
Publisher page

Abstract

High optical nonlinearity can enable classical and quantum functionalities in all-fibre laser systems. However, despite long-standing efforts to exploit second-order optical nonlinearity in conventional all-fibre systems, nonlinear optical conversion efficiencies remain modest. Here we demonstrate all-fibre integration of twist-phase-matched rhombohedral boron nitride (rBN) flakes on the end facet of optical fibres for second-harmonic generation (SHG) and spontaneous parametric downconversion (SPDC). We provide local and global optimization of the interflake twist angles for phase-matching design, achieving an SHG conversion efficiency of ~4.1% and an SPDC coincidence rate of ~90 in van der Waals crystals integrated on optical fibre devices. Finally, we design an all-fibre frequency-doubling ultrafast laser by integrating a multifunctional nonlinear crystal of a graphene/rBN heterostructure to simultaneously generate mode-locked pulses and intracavity SHG emission. This work establishes a route for developing high-efficiency, second-order nonlinear functionalities, such as optical parametric oscillators, optical modulators and entangled photon sources, in all-fibre lasers.
Source: europepmc · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Advanced Fiber Laser Technologies · Photonic Crystal and Fiber Optics · Photorefractive and Nonlinear Optics

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

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