journal article·2023-07Open access

Picophotonic localization metrology beyond thermal fluctuations

Tongjun Liu, Cheng-Hung Chi, Jun-Yu Ou, Jie Xu, Eng Aik Chan, Kevin F. MacDonald, Nikolay I. Zheludev

Nature Materials· Volume 22· Issue 7

Abstract

Abstract Despite recent tremendous progress in optical imaging and metrology1–6, there remains a substantial resolution gap between atomic-scale transmission electron microscopy and optical techniques. Is optical imaging and metrology of nanostructures exhibiting Brownian motion possible with such resolution, beyond thermal fluctuations? Here we report on an experiment in which the average position of a nanowire with a thermal oscillation amplitude of ∼150 pm is resolved in single-shot measurements with subatomic precision of 92 pm, using light at a wavelength of λ = 488 nm, providing an example of such sub-Brownian metrology with ∼λ/5,300 precision. To localize the nanowire, we employ a deep-learning analysis of the scattering of topologically structured light, which is highly sensitive to the nanowire’s position. This non-invasive metrology with absolute errors down to a fraction of the typical size of an atom, opens a range of opportunities to study picometre-scale phenomena with light.
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Research context

OpenAlex topics: Advanced Fluorescence Microscopy Techniques · Near-Field Optical Microscopy · Advanced Electron Microscopy Techniques and Applications

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