journal article·2018-07

Terahertz-light quantum tuning of a metastable emergent phase hidden by superconductivity

X. Yang, C. Vaswani, C. Sundahl, M. Mootz, P. Gagel, L. Luo, J. H. Kang, P. P. Orth, I. E. Perakis, C. B. Eom, J. Wang

Nature Materials· Volume 17· Issue 7
Publisher page

Abstract

'Sudden' quantum quench and prethermalization have become a cross-cutting theme for discovering emergent states of matter1-4. Yet this remains challenging in electron matter5-9, especially superconductors10-14. The grand question of what is hidden underneath superconductivity (SC) 15 appears universal, but poorly understood. Here we reveal a long-lived gapless quantum phase of prethermalized quasiparticles (QPs) after a single-cycle terahertz (THz) quench of a Nb3Sn SC gap. Its conductivity spectra is characterized by a sharp coherent peak and a vanishing scattering rate that decreases almost linearly towards zero frequency, which is most pronounced around the full depletion of the condensate and absent for a high-frequency pump. Above a critical pump threshold, such a QP phase with coherent transport and memory persists as an unusual prethermalization plateau, without relaxation to normal and SC thermal states for an order of magnitude longer than the QP recombination and thermalization times. Switching to this metastable 'quantum QP fluid' signals non-thermal quench of coupled SC and charge-density-wave (CDW)-like orders and hints quantum control beneath the SC.
Source: europepmc · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Physics of Superconductivity and Magnetism · Magnetic and transport properties of perovskites and related materials · Quantum and electron transport phenomena

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (34)

Show source-provided references
1. Aoki, H. et al. Nonequilibrium dynamical mean-field theory and its applications. Rev. Mod. Phys. 86, 779–837 (2014).10.1103/RevModPhys.86.779 ↗
2. Langen, T. et al. Experimental observation of a generalized Gibbs ensemble. Science 348, 207–211 (2015).10.1126/science.1257026 ↗
3. Barankov, R. A. & Levitov, L. S. Synchronization in the BCS pairing dynamics as a critical phenomenon. Phys. Rev. Lett. 96, 230403 (2006).10.1103/PhysRevLett.96.230403 ↗
4. Yuzbashyan, E. A. & Dzero, M. Dynamical vanishing of the order parameter in a fermionic condensate. Phys. Rev. Let. 96, 230404 (2006).10.1103/PhysRevLett.96.230404 ↗
5. Torchinsky, D. H. et al. Fluctuating charge-density waves in a cuprate superconductor. Nat. Mater. 12, 387–391 (2013).10.1038/nmat3571 ↗
6. Li, T. et al. Femtosecond switching of magnetism via strongly correlated spin charge quantum excitations. Nature 496, 69–73 (2013).10.1038/nature11934 ↗
7. Patz, A. et al. Ultrafast observation of critical nematic fluctuations and giant magnetoelastic coupling in iron pnictides. Nat. Commun. 5, 3229 (2014).10.1038/ncomms4229 ↗
8. Porer, M. et al. Non-thermal separation of electronic and structural orders in a persisting charge density wave. Nat. Mater. 13, 857–861 (2014).10.1038/nmat4042 ↗
9. Zhang, J. et al. Cooperative photoinduced metastable phase control in strained manganite films. Nat. Mater. 15, 956–960 (2016).10.1038/nmat4695 ↗
10. Matsunaga, R. & Shimano, R. Nonequilibrium BCS state dynamics induced by intense terahertz pulses in a superconducting NbN film. Phys. Rev. Lett. 109, 187002 (2012).10.1103/PhysRevLett.109.187002 ↗
11. Matsunaga, R. et al. Higgs amplitude mode in the BCS superconductors Nb 1−x Ti x N induced by terahertz pulse excitation. Phys. Rev. Lett. 111, 057002 (2013).10.1103/PhysRevLett.111.057002 ↗
12. Matsunaga, R. et al. Light-induced collective pseudospin precession resonating with Higgs mode in a superconductor. Science 345, 1145–1149 (2014).10.1126/science.1254697 ↗
13. Dienst, A. et al. Bi-directional ultrafast electric-field gating of interlayer charge transport in a cuprate superconductor. Nat. Photon. 5, 485–488 (2011).10.1038/nphoton.2011.124 ↗
14. Fausti, D. et al. Light-induced superconductivity in a stripe-ordered cuprate. Science 331, 189–192 (2011).10.1126/science.1197294 ↗
15. Broun, D. M. What lies beneath the dome? Nat. Phys. 4, 170–172 (2008).10.1038/nphys909 ↗
16. Kampfrath, T., Tanaka, K. & Nelson, K. A. Resonant and nonresonant control over matter and light by intense terahertz transients. Nat. Photon. 7, 680–690 (2013).10.1038/nphoton.2013.184 ↗
17. Liu, M. et al. Terahertz-field-induced insulator-to-metal transition in vanadium dioxide metamaterial. Nature 487, 345–348 (2012).10.1038/nature11231 ↗
18. Beck, M. et al. Transient increase of the energy gap of superconducting NbN thin films excited by resonant narrow-band terahertz pulses. Phys. Rev. Lett. 110, 267003 (2013).10.1103/PhysRevLett.110.267003 ↗
19. Shirane, G. & Axe, J. D. Neutron scattering study of the lattice-dynamical phase transition in Nb3Sn. Phys. Rev. B 4, 2957–2963 (1971).10.1103/PhysRevB.4.2957 ↗
20. Bilbro, G. & McMillan, W. L. Theoretical model of superconductivity and the martensitic transformation in A15 compounds. Phys. Rev. B 14, 1887–1892 (1976).10.1103/PhysRevB.14.1887 ↗
21. Markiewicz, R. S. A survey of the Van Hove scenario for high Tc superconductivity with special emphasis on pseudogaps and striped phases. J. Phys. Chem. Solids 58, 1179–1310 (1997).10.1016/S0022-3697(97)00025-5 ↗
22. Escudero, R. & Morale, F. Point contact spectroscopy of Nb3Sn crystals: evidence of a CDW gap related to the martensitic transition. Solid State Commun. 150, 715–719 (2010).10.1016/j.ssc.2010.01.038 ↗
23. Bhatt, R. N. Microscopic theory of the martensitic transition in A-15 compounds based on a three-dimensional band structure. Phys. Rev. B 16, 1915–1932 (1977).10.1103/PhysRevB.16.1915 ↗
24. Bhatt, R. N. & Lee, P. A. Theory of coherence length and phonon softening in A-15 compounds. Phys. Rev. B 16, 4288–4301 (1977).10.1103/PhysRevB.16.4288 ↗
25. Weber, W. & Mattheiss, L. F. Electronic structure of tetragonal Nb3Sn. Phys. Rev. B 25, 2270–2284 (1982).10.1103/PhysRevB.25.2270 ↗
26. Sadigh, B. & Ozolins, V. Structural instability and electronic excitations in Nb3Sn. Phys. Rev. B 57, 2793–2800 (1997).10.1103/PhysRevB.57.2793 ↗
27. Owen, C. S. & Scalapino, D. J. Superconducting state under the influence of external dynamic pair breaking. Phys. Rev. Lett. 28, 1559–1561 (1972).10.1103/PhysRevLett.28.1559 ↗
28. Chou, Y. Z. et al. Twisting Anderson pseudospins with light: quench dynamics in terahertz-pumped BCS superconductors. Phys. Rev. B 95, 104507 (2017).10.1103/PhysRevB.95.104507 ↗
29. Stojchevska, L. et al. Ultrafast switching to a stable hidden topologically protected quantum state in an electronic crystal. Science 344, 177–180 (2014).10.1126/science.1241591 ↗
30. Lingos, P. C., Wang, J. & Perakis, I. E. Manipulating femtosecond spin-orbit torques with laser pulse sequences to control magnetic memory states and ringing. Phys. Rev. B 91, 195203 (2015).10.1103/PhysRevB.91.195203 ↗
31. Yang, X. et al. Non-equilibrium pair breaking in Ba(Fe1−xCo x )2As2 superconductors: evidence for formation of photo-induced excitonic spin-density-wave state. Preprint at https://arxiv.org/abs/1804.04987 (2018).
32. Papenkort, T., Axt, V. M. & Kuhn, T. Coherent dynamics and pump-probe spectra of BCS superconductors. Phys. Rev. B 76, 224522 (2007).10.1103/PhysRevB.76.224522 ↗
33. Schnyder, A. P., Manske, D. & Avella, A. Resonant generation of coherent phonons in a superconductor by ultrafast optical pump pulses. Phys. Rev. B 84, 214513 (2011).10.1103/PhysRevB.84.214513 ↗
34. Fernandes, R. M. & Schmalian, J. Transfer of optical spectral weight in magnetically ordered superconductors. Phys. Rev. B 82, 014520 (2010).10.1103/PhysRevB.82.014520 ↗