journal article·2024-06Open access

Field-free switching of perpendicular magnetization by two-dimensional PtTe2/WTe2 van der Waals heterostructures with high spin Hall conductivity

Fei Wang, Guoyi Shi, Kyoung-Whan Kim, Hyeon-Jong Park, Jae Gwang Jang, Hui Ru Tan, Ming Lin, Yakun Liu, Taeheon Kim, Dongsheng Yang, Shishun Zhao, Kyusup Lee, Shuhan Yang, Anjan Soumyanarayanan, Kyung-Jin Lee, Hyunsoo Yang

Nature Materials· Volume 23· Issue 6

Abstract

The key challenge of spin-orbit torque applications lies in exploring an excellent spin source capable of generating out-of-plane spins while exhibiting high spin Hall conductivity. Here we combine PtTe2 for high spin conductivity and WTe2 for low crystal symmetry to satisfy the above requirements. The PtTe2/WTe2 bilayers exhibit a high in-plane spin Hall conductivity σs,y ≈ 2.32 × 105 × ħ/2e Ω-1 m-1 and out-of-plane spin Hall conductivity σs,z ≈ 0.25 × 105 × ħ/2e Ω-1 m-1, where ħ is the reduced Planck's constant and e is the value of the elementary charge. The out-of-plane spins in PtTe2/WTe2 bilayers enable the deterministic switching of perpendicular magnetization at room temperature without magnetic fields, and the power consumption is 67 times smaller than that of the Pt control case. The high out-of-plane spin Hall conductivity is attributed to the conversion from in-plane spin to out-of-plane spin, induced by the crystal asymmetry of WTe2. Our work establishes a low-power perpendicular magnetization manipulation based on wafer-scale two-dimensional van der Waals heterostructures.
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Research context

OpenAlex topics: 2D Materials and Applications · Graphene research and applications · Quantum and electron transport phenomena

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References (40)

Show source-provided references
1. Liu, L., Lee, O. J., Gudmundsen, T. J., Ralph, D. C. & Buhrman, R. A. Current-induced switching of perpendicularly magnetized magnetic layers using spin torque from the spin Hall effect. Phys. Rev. Lett. 109, 096602 (2012).10.1103/PhysRevLett.109.096602 ↗
2. Emori, S., Bauer, U., Ahn, S. M., Martinez, E. & Beach, G. S. Current-driven dynamics of chiral ferromagnetic domain walls. Nat. Mater. 12, 611–616 (2013).10.1038/nmat3675 ↗
3. Haazen, P. P. et al. Domain wall depinning governed by the spin Hall effect. Nat. Mater. 12, 299–303 (2013).10.1038/nmat3553 ↗
4. Miron, I. M. et al. Perpendicular switching of a single ferromagnetic layer induced by in-plane current injection. Nature 476, 189–193 (2011).10.1038/nature10309 ↗
5. Baek, S. C. et al. Spin currents and spin–orbit torques in ferromagnetic trilayers. Nat. Mater. 17, 509–513 (2018).10.1038/s41563-018-0041-5 ↗
6. Liu, Y. & Shao, Q. Two-dimensional materials for energy-efficient spin–orbit torque devices. ACS Nano 14, 9389–9407 (2020).10.1021/acsnano.0c04403 ↗
7. Stiehl, G. M. et al. Layer-dependent spin-orbit torques generated by the centrosymmetric transition metal dichalcogenide β−MoTe2. Phys. Rev. B 100, 184402 (2019).10.1103/PhysRevB.100.184402 ↗
8. Song, P. et al. Coexistence of large conventional and planar spin Hall effect with long spin diffusion length in a low-symmetry semimetal at room temperature. Nat. Mater. 19, 292–298 (2020).10.1038/s41563-019-0600-4 ↗
9. Liu, L. et al. Symmetry-dependent field-free switching of perpendicular magnetization. Nat. Nanotechnol. 16, 277–282 (2021).10.1038/s41565-020-00826-8 ↗
10. Stiehl, G. M. et al. Current-induced torques with Dresselhaus symmetry due to resistance anisotropy in 2D materials. ACS Nano 13, 2599–2605 (2019).
11. MacNeill, D. et al. Control of spin–orbit torques through crystal symmetry in WTe2/ferromagnet bilayers. Nat. Phys. 13, 300–305 (2017).10.1038/nphys3933 ↗
12. MacNeill, D. et al. Thickness dependence of spin-orbit torques generated by WTe2. Phys. Rev. B 96, 054450 (2017).10.1103/PhysRevB.96.054450 ↗
13. Shi, S. et al. All-electric magnetization switching and Dzyaloshinskii–Moriya interaction in WTe2/ferromagnet heterostructures. Nat. Nanotechnol. 14, 945–949 (2019).10.1038/s41565-019-0525-8 ↗
14. Shi, S. et al. Observation of the out‐of‐plane polarized spin current from CVD grown WTe2. Adv. Quantum Technol. 4, 2100038 (2021).10.1002/qute.202100038 ↗
15. Xie, Q. et al. Field-free magnetization switching induced by the unconventional spin–orbit torque from WTe2. APL Mater. 9, 051114 (2021).10.1063/5.0048926 ↗
16. Kao, I. H. et al. Deterministic switching of a perpendicularly polarized magnet using unconventional spin–orbit torques in WTe2. Nat. Mater. 21, 1029–1034 (2022).10.1038/s41563-022-01275-5 ↗
17. Mellnik, A. R. et al. Spin-transfer torque generated by a topological insulator. Nature 511, 449–451 (2014).10.1038/nature13534 ↗
18. DC, M. et al. Room-temperature high spin–orbit torque due to quantum confinement in sputtered BixSe(1–x) films. Nat. Mater. 17, 800–807 (2018).10.1038/s41563-018-0136-z ↗
19. Liu, L., Moriyama, T., Ralph, D. C. & Buhrman, R. A. Spin-torque ferromagnetic resonance induced by the spin Hall effect. Phys. Rev. Lett. 106, 036601 (2011).10.1103/PhysRevLett.106.036601 ↗
20. Liu, L. et al. Spin-torque switching with the giant spin Hall effect of tantalum. Science 336, 555–558 (2012).10.1126/science.1218197 ↗
21. Geim, A. K. & Grigorieva, I. V. Van der Waals heterostructures. Nature 499, 419–425 (2013).10.1038/nature12385 ↗
22. Novoselov, K. S., Mishchenko, A., Carvalho, A. & Castro Neto, A. H. 2D materials and van der Waals heterostructures. Science 353, aac9439 (2016).10.1126/science.aac9439 ↗
23. Sierra, J. F., Fabian, J., Kawakami, R. K., Roche, S. & Valenzuela, S. O. Van der Waals heterostructures for spintronics and opto-spintronics. Nat. Nanotechnol. 16, 856–868 (2021).10.1038/s41565-021-00936-x ↗
24. Yang, H. et al. Two-dimensional materials prospects for non-volatile spintronic memories. Nature 606, 663–673 (2022).10.1038/s41586-022-04768-0 ↗
25. Fang, D. et al. Spin–orbit-driven ferromagnetic resonance. Nat. Nanotechnol. 6, 413–417 (2011).10.1038/nnano.2011.68 ↗
26. Chen, X. et al. Observation of the antiferromagnetic spin Hall effect. Nat. Mater. 20, 800–804 (2021).10.1038/s41563-021-00946-z ↗
27. Xu, H. et al. High spin Hall conductivity in large-area type-II Dirac semimetal PtTe2. Adv. Mater. 32, e2000513 (2020).10.1002/adma.202000513 ↗
28. Zhu, L. et al. Strong damping‐like spin‐orbit torque and tunable Dzyaloshinskii–Moriya interaction generated by low‐resistivity Pd1−xPtx alloys. Adv. Funct. Mater. 29, 1805822 (2019).10.1002/adfm.201805822 ↗
29. Lifshits, M. B. & Dyakonov, M. I. Swapping spin currents: interchanging spin and flow directions. Phys. Rev. Lett. 103, 186601 (2009).10.1103/PhysRevLett.103.186601 ↗
30. Saidaoui, H. B. & Manchon, A. Spin-swapping transport and torques in ultrathin magnetic bilayers. Phys. Rev. Lett. 117, 036601 (2016).10.1103/PhysRevLett.117.036601 ↗
31. Park, H. J. et al. Spin swapping effect of band structure origin in centrosymmetric ferromagnets. Phys. Rev. Lett. 129, 037202 (2022).10.1103/PhysRevLett.129.037202 ↗
32. Lin, W. et al. Evidence for spin swapping in an antiferromagnet. Nat. Phys. 18, 800–805 (2022).10.1038/s41567-022-01608-w ↗
33. Valet, T. & Fert, A. Theory of the perpendicular magnetoresistance in magnetic multilayers. Phys. Rev. B 48, 7099–7113 (1993).10.1103/PhysRevB.48.7099 ↗
34. Haney, P. M., Lee, H.-W., Lee, K.-J., Manchon, A. & Stiles, M. D. Current induced torques and interfacial spin-orbit coupling: semiclassical modeling. Phys. Rev. B 87, 174411 (2013).10.1103/PhysRevB.87.174411 ↗
35. Wang, Y., Deorani, P., Qiu, X., Kwon, J. H. & Yang, H. Determination of intrinsic spin Hall angle in Pt. Appl. Phys. Lett. 105, 152412 (2014).10.1063/1.4898593 ↗
36. Shao, Q. et al. Roadmap of spin–orbit torques. IEEE Trans. Magn. 57, 800439 (2021).10.1109/TMAG.2021.3078583 ↗
37. Guimaraes, M. H. D., Stiehl, G. M., MacNeill, D., Reynolds, N. D. & Ralph, D. C. Spin–orbit torques in NbSe2/permalloy bilayers. Nano Lett. 18, 1311–1316 (2018).10.1021/acs.nanolett.7b04993 ↗
38. Liang, S. et al. Spin-orbit torque magnetization switching in MoTe2/permalloy heterostructures. Adv. Mater. 32, e2002799 (2020).10.1002/adma.202002799 ↗
39. Nan, T. et al. Controlling spin current polarization through non-collinear antiferromagnetism. Nat. Commun. 11, 4671 (2020).10.1038/s41467-020-17999-4 ↗
40. Bose, A. et al. Tilted spin current generated by the collinear antiferromagnet ruthenium dioxide. Nat. Electron. 5, 267–274 (2022).10.1038/s41928-022-00744-8 ↗