Room-temperature antiskyrmions and sawtooth surface textures in a non-centrosymmetric magnet with S4 symmetry
Source abstract
Abstract
Topological spin textures have attracted much attention both for fundamental physics and spintronics applications. Among them, antiskyrmions possess a unique spin configuration with Bloch-type and Néel-type domain walls owing to anisotropic Dzyaloshinskii-Moriya interaction in the non-centrosymmetric crystal structure. However, antiskyrmions have thus far only been observed in a few Heusler compounds with D2d symmetry. Here we report a new material, Fe1.9Ni0.9Pd0.2P, in a different symmetry class (S4), in which antiskyrmions exist over a wide temperature range that includes room temperature, and transform into skyrmions on changing magnetic field and lamella thickness. The periodicity of magnetic textures greatly depends on the crystal thickness, and domains with anisotropic sawtooth fractals were observed at the surface of thick crystals and attributed to the interplay between the dipolar interaction and the Dzyaloshinskii-Moriya interaction as governed by crystal symmetry. Our findings provide an arena in which to study antiskyrmions, and should stimulate further research on topological spin textures and their applications.
Source: europepmc · Quality: candidate unverified · Source record ↗
Research context
OpenAlex topics: Magnetic properties of thin films · Heusler alloys: electronic and magnetic properties · Topological Materials and Phenomena
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
References (43)
Show source-provided references
1. Nagaosa, N. & Tokura, Y. Topological properties and dynamics of magnetic skyrmions. Nat. Nanotechnol. 8, 899–911 (2013).10.1038/nnano.2013.243 ↗
2. Bogdanov, A. N. & Yablonskii, D. A. Thermodynamically stable ‘vortices’ in magnetically ordered crystals. The mixed state of magnets. Sov. Phys. JETP 68, 101–103 (1989).
3. Leonov, A. O. et al. The properties of isolated chiral skyrmions in thin magnetic films. New J. Phys. 18, 065003 (2016).10.1088/1367-2630/18/6/065003 ↗
4. Mühlbauer, S. et al. Skyrmion lattice in a chiral magnet. Science 323, 915–919 (2009).10.1126/science.1166767 ↗
5. Yu, X. Z. et al. Real-space observation of a two-dimensional skyrmion crystal. Nature 465, 901–904 (2010).10.1038/nature09124 ↗
6. Seki, S., Yu, X. Z., Ishiwata, S. & Tokura, Y. Observation of skyrmions in a multiferroic material. Science 336, 198–201 (2012).10.1126/science.1214143 ↗
7. Tokunaga, Y. et al. A new class of chiral materials hosting magnetic skyrmions beyond room temperature. Nat. Commun. 6, 7638–7644 (2015).10.1038/ncomms8638 ↗
8. Heinze, S. et al. Spontaneous atomic-scale magnetic skyrmion lattice in two dimensions. Nat. Phys. 7, 713–718 (2011).10.1038/nphys2045 ↗
9. Woo, S. et al. Observation of room-temperature magnetic skyrmions and their current-driven dynamics in ultrathin metallic ferromagnets. Nat. Mater. 15, 501–506 (2016).10.1038/nmat4593 ↗
10. Pollard, S. D. et al. Observation of stable Néel skyrmions in cobalt/palladium multilayers with Lorentz transmission electron microscopy. Nat. Commun. 8, 14761 (2017).10.1038/ncomms14761 ↗
11. Kézsmárki, I. et al. Néel-type skyrmion lattice with confined orientation in the polar magnetic semiconductor GaV4S8. Nat. Mater. 14, 1116–1122 (2015).10.1038/nmat4402 ↗
12. Kurumaji, T. et al. Néel-type skyrmion lattice in the tetragonal polar magnet VOSe2O5. Phys. Rev. Lett. 119, 237201 (2017).10.1103/PhysRevLett.119.237201 ↗
13. Srivastava, A. K. et al. Observation of robust Néel skyrmions in metallic PtMnGa. Adv. Mater. 32, 1904327 (2020).10.1002/adma.201904327 ↗
14. Hoffmann, M. et al. Antiskyrmions stabilized at interfaces by anisotropic Dzyaloshinskii–Moriya interactions. Nat. Commun. 8, 308 (2017).10.1038/s41467-017-00313-0 ↗
15. Camosi, L., Rougemaille, N., Fruchart, O., Vogel, J. & Rohart, S. Micromagnetics of antiskyrmions in ultrathin films. Phys. Rev. B 97, 134404 (2018).10.1103/PhysRevB.97.134404 ↗
16. Nayak, A. K. et al. Magnetic antiskyrmions above room temperature in tetragonal Heusler materials. Nature 548, 561–566 (2017).10.1038/nature23466 ↗
17. Jena, J. et al. Observation of magnetic antiskyrmions in the low magnetization ferrimagnet Mn2Rh0.95Ir0.05Sn. Nano Lett. 20, 59–65 (2020).10.1021/acs.nanolett.9b02973 ↗
18. Gambino, R. J., McGuire, T. R. & Nakamura, Y. Magnetic properties of the iron-group metal phosphides. J. Appl. Phys. 38, 1253–1255 (1967).10.1063/1.1709566 ↗
19. Goto, M., Tange, H., Tokunaga, T., Fujii, H. & Okamoto, T. Magnetic properties of the (Fe1−xMx)3P compounds. Jpn J. Appl. Phys. 16, 2175–2179 (1977).10.1143/JJAP.16.2175 ↗
20. Koshibae, W. & Nagaosa, N. Theory of antiskyrmions in magnets. Nat. Commun. 7, 10542 (2016).10.1038/ncomms10542 ↗
21. Vir, P. et al. Tetragonal superstructure of the antiskyrmion hosting Heusler compound Mn1.4PtSn. Chem. Mater. 31, 5876–5880 (2019).10.1021/acs.chemmater.9b02013 ↗
22. Peng, L. C. et al. Controlled transformation of skyrmions and antiskyrmions in a non-centrosymmetric magnet. Nat. Nanotech. 15, 181–186 (2020).10.1038/s41565-019-0616-6 ↗
23. Jena, J. et al. Elliptical Bloch skyrmion chiral twins in an antiskyrmion system. Nat. Commun. 11, 1115 (2020).10.1038/s41467-020-14925-6 ↗
24. Kittel, C. Theory of the structure of ferromagnetic domains in films and small particles. Phys. Rev. 70, 965–971 (1946).10.1103/PhysRev.70.965 ↗
25. Malozemoff, A. P. & Slonczewski, J. C. Magnetic Domain Walls in Bubble Materials (Academic, 1979).
26. Hubert, A. & Schäfer, R. Magnetic Domains: The Analysis of Magnetic Microstructures (Springer, 1998).
27. Szymczak, R. A modification of the Kittel open structure. J. Appl. Phys. 39, 875–876 (1968).10.1063/1.2163656 ↗
28. Kaczér, J. On the domain structure of uniaxial ferromagnets. Sov. Phys. JETP 19, 1204–1208 (1964).
29. Gemperle, R., Murtinová, L. & Kamberský, V. Experimental verification of theoretical relations for the domain structure of uniaxial ferromagnets. Phys. Stat. Sol. A 158, 229 (1996).10.1002/pssa.2211580125 ↗
30. Szmaja, W. Investigations of the domain structure of anisotropic sintered Nd–Fe–B-based permanent magnets. J. Mag. Mag. Mater. 301, 546–561 (2006).10.1016/j.jmmm.2005.09.039 ↗
31. Kreyssig, A. et al. Probing fractal magnetic domains on multiple length scales in Nd2Fe14B. Phys. Rev. Lett. 102, 047204 (2009).10.1103/PhysRevLett.102.047204 ↗
32. Jalli, J. et al. MFM studies of magnetic domain patterns in bulk barium ferrite (BaFe12O19) single crystals. J. Mag. Mag. Mater. 323, 2627–2631 (2011).10.1016/j.jmmm.2011.05.046 ↗
33. Vansteenkiste, A. et al. The design and verification of MuMax3. AIP Adv. 4, 107133 (2014).10.1063/1.4899186 ↗
34. Ma, T. et al. Tunable magnetic antiskyrmion size and helical period from nanometers to micrometers in a D2d Heusler compound. Adv. Mater. 32, 2002043 (2020).10.1002/adma.202002043 ↗
35. Ishizuka, K. & Allman, B. Phase measurement of atomic resolution image using transport of intensity equation. J. Electron Microsc. 54, 191–197 (2005).
36. Chapman, J. N., Batson, P. E., Waddell, E. M. & Ferrier, R. P. The direct determination of magnetic domain wall profiles by differential phase contrast electron microscopy. Ultramicroscopy 3, 203–214 (1978).10.1016/S0304-3991(78)80027-8 ↗
37. Sandweg, C. W. et al. Direct observation of domain wall structures in curved permalloy wires containing an antinotch. J. Appl. Phys. 103, 093906 (2008).10.1063/1.2913318 ↗
38. McGrouther, D. et al. Internal structure of hexagonal skyrmion lattices in cubic helimagnets. New J. Phys. 18, 095004 (2016).10.1088/1367-2630/18/9/095004 ↗
39. Shibata, N. et al. Direct visualization of local electromagnetic field structures by scanning transmission electron microscopy. Acc. Chem. Res. 50, 1502–1512 (2017).10.1021/acs.accounts.7b00123 ↗
40. Matsumoto, T., So, Y. G., Kohno, Y., Ikuhara, Y. & Shibata, N. Stable magnetic skyrmion states at room temperature confined to corrals of artificial surface pits fabricated by a focused electron beam. Nano Lett. 18, 754–762 (2018).10.1021/acs.nanolett.7b03967 ↗
41. Pöllath, S. et al. Spin structure relation to phase contrast imaging of isolated magnetic Bloch and Néel skyrmions. Ultramicroscopy 212, 112973 (2020).10.1016/j.ultramic.2020.112973 ↗
42. Yasin, F. S. et al. Bloch lines constituting antiskyrmions captured via differential phase contrast. Adv. Mater. 32, 2004206 (2020).10.1002/adma.202004206 ↗
43. Ishizuka, A., Oka, M., Seki, T., Shibata, N. & Ishizuka, K. Boundary-artifact-free determination of potential distribution from differential phase contrast signals. Microscopy 66, 397 (2017).10.1093/jmicro/dfx032 ↗