journal article·2019-09Open access

Spatially dispersive circular photogalvanic effect in a Weyl semimetal

Zhurun Ji, Gerui Liu, Zachariah Addison, Wenjing Liu, Peng Yu, Heng Gao, Zheng Liu, Andrew M. Rappe, Charles L. Kane, Eugene J. Mele, Ritesh Agarwal

Nature Materials· Volume 18· Issue 9

Abstract

Weyl semimetals (WSMs) are gapless topological states of matter with broken inversion and/or time reversal symmetry. WSMs can support a circulating photocurrent when illuminated by circularly polarized light at normal incidence. Here, we report a spatially dispersive circular photogalvanic effect (s-CPGE) in a WSM that occurs with a spatially varying beam profile. Our analysis shows that the s-CPGE is controlled by a symmetry selection rule combined with asymmetric carrier excitation and relaxation dynamics. By evaluating the s-CPGE for a minimal model of a WSM, a frequency-dependent scaling behaviour of the photocurrent is obtained. Wavelength-dependent measurements from the visible to mid-infrared range show evidence of Berry curvature singularities and band inversion in the s-CPGE response. We present the s-CPGE as a promising spectroscopic probe for topological band properties, with the potential for controlling photoresponse by patterning optical fields on topological materials to store, manipulate and transmit information.
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Research context

OpenAlex topics: Topological Materials and Phenomena · Quantum Mechanics and Non-Hermitian Physics · Metamaterials and Metasurfaces Applications

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