journal article·2023-01Open access

Planar thermal Hall effect of topological bosons in the Kitaev magnet α-RuCl3

Peter Czajka, Tong Gao, Max Hirschberger, Paula Lampen-Kelley, Arnab Banerjee, Nicholas Quirk, David G. Mandrus, Stephen E. Nagler, N. P. Ong

Nature Materials· Volume 22· Issue 1

Abstract

The honeycomb magnet α-RuCl3 has attracted considerable interest because it is proximate to the Kitaev Hamiltonian whose excitations are Majoranas and vortices. The thermal Hall conductivity κxy of Majorana fermions is predicted to be half-quantized. Half-quantization of κxy/T (T, temperature) was recently reported, but this observation has proven difficult to reproduce. Here, we report detailed measurements of κxy on α-RuCl3 with the magnetic field B ∥ a (zigzag axis). In our experiment, κxy/T is observed to be strongly temperature dependent between 0.5 and 10 K. We show that its temperature profile matches the distinct form expected for topological bosonic modes in a Chern-insulator-like model. Our analysis yields magnon band energies in agreement with spectroscopic experiments. At high B, the spin excitations evolve into magnon-like modes with a Chern number of ~1. The bosonic character is incompatible with half-quantization of κxy/T.
Source: europepmc · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Advanced Condensed Matter Physics · Magnetic and transport properties of perovskites and related materials · Topological Materials and Phenomena

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (30)

Show source-provided references
1. Kitaev, A. Anyons in an exactly solved model and beyond. Ann. Phys. 321, 2–111 (2006).10.1016/j.aop.2005.10.005 ↗
2. Jackeli, G. & Khaliullin, G. Mott insulators in the strong spin-orbit coupling limit: from Heisenberg to a quantum compass and Kitaev models. Phys. Rev. Lett. 102, 017205 (2009).10.1103/PhysRevLett.102.017205 ↗
3. Plumb, K. W. et al. α–RuCl3 : a spin-orbit assisted Mott insulator on a honeycomb lattice. Phys. Rev. B 90, 041112 (2014).10.1103/PhysRevB.90.041112 ↗
4. Banerjee, A. et al. Proximate Kitaev quantum spin liquid behavior in a honeycomb magnet. Nat. Mater. 15, 733–740 (2016).10.1038/nmat4604 ↗
5. Leahy, I. A. et al. Anomalous thermal conductivity and magnetic torque response in the honeycomb magnet α–RuCl3. Phys. Rev. Lett. 118, 187203 (2017).10.1103/PhysRevLett.118.187203 ↗
6. Banerjee, A. et al. Excitations in the field-induced quantum spin liquid state of α-RuCl3. npj Quantum Mater. 3, 8 (2018).10.1038/s41535-018-0079-2 ↗
7. Hentrich, R. et al. Unusual phonon heat transport in α–RuCl3: strong spin-phonon scattering and field-induced spin gap. Phys. Rev. Lett. 120, 117204 (2018).10.1103/PhysRevLett.120.117204 ↗
8. McClarty, P. A. et al. Topological magnons in Kitaev magnets at high fields. Phys. Rev. B 98, 060404 (2018).10.1103/PhysRevB.98.060404 ↗
9. Joshi, D. G. Topological excitations in the ferromagnetic Kitaev-Heisenberg model. Phys. Rev. B 98, 060405 (2018).10.1103/PhysRevB.98.060405 ↗
10. Gordon, J. S., Catuneanu, A., Sørensen, E. S. & Kee, H.-Y. Theory of the field-revealed Kitaev spin liquid. Nat. Commun. 10, 2470 (2019).10.1038/s41467-019-10405-8 ↗
11. Hickey, C. & Trebst, S. Emergence of a field-driven U(1) spin liquid in the Kitaev honeycomb model. Nat. Commun. 10, 530 (2019).10.1038/s41467-019-08459-9 ↗
12. Savary, L. & Balents, L. Quantum spin liquids: a review. Rep. Prog. Phys. 80, 106502 (2017).10.1088/0034-4885/80/1/016502 ↗
13. Kasahara, Y. et al. Majorana quantization and half-integer thermal quantum Hall effect in a Kitaev spin liquid. Nature 559, 227–231 (2018).10.1038/s41586-018-0274-0 ↗
14. Yokoi, T. et al. Half-integer quantized anomalous thermal Hall effect in the Kitaev candidate α-RuCl3. Science 373, 568–572 (2021).10.1126/science.aay5551 ↗
15. Czajka, P. et al. Oscillations of the thermal conductivity in the spin-liquid state of α-RuCl3. Nat. Phys. 17, 915–919 (2021).10.1038/s41567-021-01243-x ↗
16. Bruin, J. A. N. et al. Robustness of the thermal Hall effect close to half-quantization in α-RuCl3. Nat. Phys. 18, 401–405 (2022).10.1038/s41567-021-01501-y ↗
17. Onose, Y. et al. Observation of the magnon Hall effect. Science 329, 297–299 (2011).10.1126/science.1188260 ↗
18. Hirschberger, M., Krizan, J. W., Cava, R. J. & Ong, N. P. Large thermal Hall conductivity of neutral spin excitations in a frustrated quantum magnet. Science 348, 106–109 (2015).10.1126/science.1257340 ↗
19. Liang, T. et al. Anomalous Hall effect in ZrTe5. Nat. Phys. 14, 451–455 (2018).10.1038/s41567-018-0078-z ↗
20. Chern, L. E., Zhang, E. Z. & Kim, Y. B. Sign structure of thermal Hall conductivity and topological magnons for in-plane field polarized Kitaev magnets. Phys. Rev. Lett. 126, 147201 (2021).10.1103/PhysRevLett.126.147201 ↗
21. Zhang, E. Z., Chern, L. E. & Kim, Y. B. Topological magnons for thermal Hall transport in frustrated magnets with bond-dependent interactions. Phys. Rev. B 103, 174402 (2021).10.1103/PhysRevB.103.174402 ↗
22. Utermohlen, F. G. & Trivedi, N. Symmetry analysis of tensors in the honeycomb lattice of edge-sharing octahedra. Phys. Rev. B 103, 155124 (2021).10.1103/PhysRevB.103.155124 ↗
23. Matsumoto, R. & Murakami, S. Rotational motion of magnons and the thermal Hall effect. Phys. Rev. B 84, 184406 (2011).10.1103/PhysRevB.84.184406 ↗
24. Kane, C. L. & Fisher, M. P. A. Quantized thermal transport in the fractional quantum Hall effect. Phys. Rev. B 55, 15832 (1997).10.1103/PhysRevB.55.15832 ↗
25. Ponomaryov, A. N. et al. Unconventional spin dynamics in the honeycomb-lattice material α–RuCl3: high-field electron spin resonance studies. Phys. Rev. B 96, 241107(R) (2017).10.1103/PhysRevB.96.241107 ↗
26. Ponomaryov, A. N. et al. Nature of magnetic excitations in the high-field phase of α–RuCl3. Phys. Rev. Lett. 125, 037202 (2020).10.1103/PhysRevLett.125.037202 ↗
27. Wellm, C. et al. Signatures of low-energy fractionalized excitations in α–RuCl3 from field-dependent microwave absorption. Phys. Rev. B 98, 184408 (2018).10.1103/PhysRevB.98.184408 ↗
28. Balz, C. et al. Finite field regime for a quantum spin liquid in α–RuCl3. Phys. Rev. B 100, 060405(R) (2019).10.1103/PhysRevB.100.060405 ↗
29. Winter, S. M., Riedl, K., Kaib, D., Coldea, R. & Valenti, R. Probing α–RuCl3 beyond magnetic order: effects of temperature and magnetic field. Phys. Rev. Lett. 120, 077203 (2018).10.1103/PhysRevLett.120.077203 ↗
30. Villadiego, I. S. Pseudoscalar U(1) spin liquids in α–RuCl3. Phys. Rev. B 104, 195149 (2021).10.1103/PhysRevB.104.195149 ↗