journal article·2005-04-01Open access

Spin chirality on a two-dimensional frustrated lattice

Daniel Grohol, Kittiwit Matan, Jin-Hyung Cho, Seung-Hun Lee, Jeffrey W. Lynn, Daniel G. Nocera, Young S. Lee

Nature Materials· Volume 4· Issue 4

Abstract

The collective behaviour of interacting magnetic moments can be strongly influenced by the topology of the underlying lattice. In geometrically frustrated spin systems, interesting chiral correlations may develop that are related to the spin arrangement on triangular plaquettes. We report a study of the spin chirality on a two-dimensional geometrically frustrated lattice. Our new chemical synthesis methods allow us to produce large single-crystal samples of KFe3(OH)6(SO4)2, an ideal Kagomé lattice antiferromagnet. Combined thermodynamic and neutron scattering measurements reveal that the phase transition to the ordered ground-state is unusual. At low temperatures, application of a magnetic field induces a transition between states with different non-trivial spin-textures.
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Research context

OpenAlex topics: Advanced Condensed Matter Physics · Physics of Superconductivity and Magnetism · Magnetic and transport properties of perovskites and related materials

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