Engineering relaxors by entropy for high energy storage performance
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OpenAlex topics: Ferroelectric and Piezoelectric Materials · Multiferroics and related materials · Dielectric properties of ceramics
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References (50)
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1. Chu, B. et al. A dielectric polymer with high-electric-energy density and fast discharge speed. Science 313, 334–336 (2006).10.1126/science.1127798 ↗
2. Wang, G. et al. Electroceramics for high-energy density capacitors: current status and future perspectives. Chem. Rev. 121, 6124–6172 (2021).10.1021/acs.chemrev.0c01264 ↗
3. Li, J. et al. Grain-orientation-engineered multilayer ceramic capacitors for energy storage applications. Nat. Mater. 19, 999–1005 (2020).10.1038/s41563-020-0704-x ↗
4. Yang, L. et al. Perovskite lead-free dielectrics for energy storage applications. Prog. Mater. Sci. 102, 72–108 (2019).10.1016/j.pmatsci.2018.12.005 ↗
5. Pan, H. et al. Ultrahigh energy storage in superparaelectric relaxor ferroelectrics. Science 374, 100–104 (2021).10.1126/science.abi7687 ↗
6. Kim, J. et al. Ultrahigh-capacitive energy density in ion-bombarded relaxor ferroelectric films. Science 369, 81–84 (2020).10.1126/science.abb0631 ↗
7. Jayakrishnan, A. R. et al. Are lead-free relaxor ferroelectric materials the most promising candidates for energy storage capacitors? Prog. Mater. Sci. 132, 101046 (2023).10.1016/j.pmatsci.2022.101046 ↗
8. Li, F., Zhang, S., Damjanovic, D., Chen, L.-Q. & Shrout, T. R. Local structural heterogeneity and electromechanical responses of ferroelectrics: learning from relaxor ferroelectrics. Adv. Funct. Mater. 28, 1801504 (2018).10.1002/adfm.201801504 ↗
9. Pan, H. et al. Giant energy density and high efficiency achieved in bismuth ferrite-based film capacitors via domain engineering. Nat. Commun. 9, 1813 (2018).10.1038/s41467-018-04189-6 ↗
10. Shetty, S. et al. Relaxor behavior in ordered lead magnesium niobate (PbMg1/3Nb2/3O3) thin films. Adv. Funct. Mater. 29, 1804258 (2019).10.1002/adfm.201804258 ↗
11. Yang, C. et al. Fatigue-free and bending-endurable flexible Mn-doped Na0.5Bi0.5TiO3-BaTiO3-BiFeO3 film capacitor with an ultrahigh energy storage performance. Adv. Energy Mater. 9, 1803949 (2019).10.1002/aenm.201803949 ↗
12. Chen, J., Qi, H. & Zuo, R. Realizing stable relaxor antiferroelectric and superior energy storage properties in (Na1−x/2Lax/2)(Nb1−xTix)O3 lead-free ceramics through A/6-site complex substitution. ACS Appl. Mater. Interfaces 12, 32871–32879 (2020).10.1021/acsami.0c09876 ↗
13. Cantor, B., Chang, I. T. H., Knight, P. & Vincent, A. J. B. Microstructural development in equiatomic multicomponent alloys. Mater. Sci. Eng. A 375, 213–218 (2004).10.1016/j.msea.2003.10.257 ↗
14. Rost, C. M. et al. Entropy-stabilized oxides. Nat. Commun. 6, 8485 (2015).10.1038/ncomms9485 ↗
15. Yang, B. et al. High-entropy enhanced capacitive energy storage. Nat. Mater. 21, 1074–1080 (2022).10.1038/s41563-022-01274-6 ↗
16. Sarkar, A. et al. High-entropy oxides for reversible energy storage. Nat. Commun. 9, 3400 (2018).10.1038/s41467-018-05774-5 ↗
17. Bérardan, D., Franger, S., Dragoe, D., Meena, A. K. & Dragoe, N. Colossal dielectric constant in high-entropy oxides. Phys. Status Solidi Rapid Res. Lett. 10, 328–333 (2016).10.1002/pssr.201600043 ↗
18. Jiang, S. et al. A new class of high-entropy perovskite oxides. Scr. Mater. 142, 116–120 (2018).10.1016/j.scriptamat.2017.08.040 ↗
19. Braun, J. L. et al. Charge-induced disorder controls the thermal conductivity of entropy-stabilized oxides. Adv. Mater. 30, 1805004 (2018).10.1002/adma.201805004 ↗
20. Berardan, D., Franger, S., Meena, A. K. & Dragoe, N. Room temperature lithium superionic conductivity in high-entropy oxides. J. Mater. Chem. A 4, 9536–9541 (2016).10.1039/C6TA03249D ↗
21. Sarkar, A. et al. High-entropy oxides: fundamental aspects and electrochemical properties. Adv. Mater. 31, 1806236 (2019).10.1002/adma.201806236 ↗
22. Chen, L. et al. Giant energy-storage density with ultrahigh efficiency in lead-free relaxors via high-entropy design. Nat. Commun. 13, 3089 (2022).10.1038/s41467-022-30821-7 ↗
23. Pu, Y. et al. Dielectric properties and electrocaloric effect of high-entropy (Na0.2Bi0.2Ba0.2Sr0.2Ca0.2)TiO3 ceramic. Appl. Phys. Lett. 115, 223901 (2019).10.1063/1.5126652 ↗
24. Yan, B., Chen, K. & An, L. Design and preparation of lead-free (Bi0.4Na0.2K0.2Ba0.2)TiO3-Sr(Mg1/3Nb2/3)O3 high-entropy relaxor ceramics for dielectric energy storage. Chem. Eng. J. 453, 139921 (2023).10.1016/j.cej.2022.139921 ↗
25. Hong, Z. et al. Role of point defects in the formation of relaxor ferroelectrics. Acta Mater. 225, 117558 (2022).10.1016/j.actamat.2021.117558 ↗
26. Cummins, S. E. & Cross, L. E. Electrical and optical properties of ferroelectric Bi4Ti3O12 single crystals. J. Appl. Phys. 39, 2268–2274 (1968).10.1063/1.1656542 ↗
27. Chon, U., Jang, H. M., Kim, M. G. & Chang, C. H. Layered perovskites with giant spontaneous polarizations for non-volatile memories. Phys. Rev. Lett. 89, 087601 (2002).10.1103/PhysRevLett.89.087601 ↗
28. Kim, J. et al. Utilization of high-entropy alloy characteristics in Er-Gd-Y-Al-Co high entropy bulk metallic glass. Acta Mater. 155, 350–361 (2018).10.1016/j.actamat.2018.06.024 ↗
29. Kim, S. J. et al. Direct observation of oxygen stabilization in layered ferroelectric Bi3.25La0.75Ti3O12. Appl. Phys. Lett. 91, 062913 (2007).10.1063/1.2768906 ↗
30. Shannon, R. D. Revised effective ionic radii and systematic studies of interatomic distances in halides and chalcogenides. Acta Cryst. 32, 751–767 (1976).10.1107/S0567739476001551 ↗
31. Jiang, B. et al. High-entropy-stabilized chalcogenides with high thermoelectric performance. Science 371, 830–834 (2021).10.1126/science.abe1292 ↗
32. Su, L. et al. Direct observation of elemental fluctuation and oxygen octahedral distortion-dependent charge distribution in high-entropy oxides. Nat. Commun. 13, 2358 (2022).10.1038/s41467-022-30018-y ↗
33. Li, F. et al. Giant piezoelectricity of Sm-doped Pb(Mg1/3Nb2/3)O3-PbTiO3 single crystals. Science 364, 264–268 (2019).10.1126/science.aaw2781 ↗
34. Wright, A. J. et al. Size disorder as a descriptor for predicting reduced thermal conductivity in medium- and high-entropy pyrochlore oxides. Scr. Mater. 181, 76–81 (2020).10.1016/j.scriptamat.2020.02.011 ↗
35. Ma, Z. et al. High thermoelectric performance and low lattice thermal conductivity in lattice-distorted high-entropy semiconductors AgMnSn1−xPbxSbTe4. Chem. Mater. 34, 8959–8967 (2022).10.1021/acs.chemmater.2c02344 ↗
36. Xiong, W. et al. Low-loss high entropy relaxor-like ferroelectrics with A-site disorder. J. Eur. Ceram. Soc. 41, 2979–2985 (2021).10.1016/j.jeurceramsoc.2020.11.030 ↗
37. Pan, H. et al. Ultrahigh-energy density lead-free dielectric films via polymorphic nanodomain design. Science 365, 578–582 (2019).10.1126/science.aaw8109 ↗
38. Kim, C., Pilania, G. & Ramprasad, R. Machine learning assisted predictions of intrinsic dielectric breakdown strength of ABX3 perovskites. J. Phys. Chem. C 120, 14575–14580 (2016).10.1021/acs.jpcc.6b05068 ↗
39. Yeh J.-W., Chen S.-K., Shih H. C., Zhang Y. & Zuo T. T. in High-Entropy Alloys: Fundamentals and Applications (eds Gao, M. C. et al.) 238–240 (Springer, 2016).
40. Mu, S. et al. Uncovering electron scattering mechanisms in NiFeCoCrMn derived concentrated solid solution and high-entropy alloys. npj Comput. Mater. 4, 47–54 (2020).10.1038/s41524-018-0138-z ↗
41. Jin, L. et al. BiFeO3(00l)/LaNiO3/Si thin films with enhanced polarization: an all-solution approach. RSC Adv. 6, 78629–78635 (2016).10.1039/C6RA16388B ↗
42. Li, M. et al. A family of oxide ion conductors based on the ferroelectric perovskite Na0.5Bi0.5TiO3. Nat. Mater. 13, 31–35 (2014).10.1038/nmat3782 ↗
43. Sun Y. et al. Ultrahigh energy storage density in glassy ferroelectric thin films under low electric field. Adv. Sci. https://doi.org/10.1002/advs.202203926 (2022).10.1002/advs.202203926 ↗
44. Wang, K. et al. Superparaelectric (Ba0.95,Sr0.05)(Zr0.2,Ti0.8)O3 ultracapacitors. Adv. Energy Mater. 10, 2001778 (2020).10.1002/aenm.202001778 ↗
45. Bin, C. et al. Flexible lead-free film capacitor based on BiMg0.5Ti0.5O3-SrTiO3 for high-performance energy storage. Chem. Eng. J. 445, 136728 (2022).10.1016/j.cej.2022.136728 ↗
46. Yang, S., Kim, T., Yoon, J.-G. & Noh, T. Nanoscale observation of time-dependent domain wall pinning as the origin of polarization fatigue. Adv. Funct. Mater. 22, 2310–2317 (2012).10.1002/adfm.201102685 ↗
47. Glaum, J. & Hoffman, M. Electric fatigue of lead-free piezoelectric materials. J. Am. Ceram. Soc. 97, 665–680 (2014).10.1111/jace.12811 ↗
48. Chen, X., Huang, B., Liu, Y., Wang, W. & Yu, P. High energy density and high efficiency achieved in the Ca0.74Sr0.26Zr0.7Ti0.3O3 linear dielectric thin films on the silicon substrates. Appl. Phys. Lett. 117, 112902 (2020).10.1063/5.0024307 ↗
49. Shvartsman, V. V. & Lupascu, D. C. Lead-free relaxor ferroelectrics. J. Am. Ceram. Soc. 95, 1–26 (2012).10.1111/j.1551-2916.2011.04952.x ↗
50. Hong, K., Lee, T. H., Suh, J. M., Yoon, S.-H. & Jang, H. W. Perspectives and challenges in multilayer ceramic capacitors for next generation electronics. J. Mater. Chem. C 7, 9782–9802 (2019).10.1039/C9TC02921D ↗