Pressure-induced disorder and nanosizing inhibits superconductivity in In2Te3
Source abstract
Abstract
Abstract The generation of disorder often gives rise to profound and irreversible physical phenomena. Here, we explore the influence of disorder on the superconducting properties of In2Te3 through comprehensive high-pressure investigations. Building upon previous findings, we investigated the progressive suppression of superconductivity in In2Te3 during the depressurization process: the increased disorder that ultimately leads to the complete disappearance of the superconducting state. Simultaneously, our high-pressure x-ray diffraction analysis reveals an irreversible structural phase transition. Furthermore, microstructure analysis using transmission electron microscopy clearly demonstrates both grain refinement and a substantial enhancement of disorder. These findings not only provide valuable insights into the mechanism by which disorder suppresses superconductivity, but also offer guidance for future advancements in the fabrication of atmospheric-pressure superconductors.
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Research context
OpenAlex topics: Electronic and Structural Properties of Oxides · Machine Learning in Materials Science · Chalcogenide Semiconductor Thin Films
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References (35)
Show source-provided references
1. Quantum breakdown of superconductivity in low-dimensional materials10.1038/s41567-020-0905-x ↗
2. Superconducting phase induced by a local structure transition in amorphous Sb2Se3 under high pressure10.1103/PhysRevLett.127.127002 ↗
3. Pair-breaking model for disorder in two-dimensional superconductors10.1103/PhysRevB.30.4063 ↗
4. Suppression of superconductivity by crystallographic defects in epitaxial Sr2RuO4 films10.1063/1.1364659 ↗
5. Theory of dirty superconductors10.1016/0022-3697(59)90036-8 ↗
6. A disorder-enhanced Quasi-one-dimensional Superconductor10.1038/ncomms12262 ↗
7. Disorder Enhanced Superconductivity toward TaS2 Monolayer10.1021/acsnano.8b04718 ↗
8. Localized superconductors10.1103/PhysRevB.32.5658 ↗
9. Nature of the superconductor–insulator transition in disordered superconductors10.1038/nature06180 ↗
10. Pressure-quenched superconductivity in Weyl semimetal NbP induced by electronic phase transitions under pressure10.1021/acs.jpclett.2c01266 ↗
11. Phase transition mechanism and bandgap engineering of Sb2S3 at gigapascal pressures10.1038/s42004-021-00565-4 ↗
12. Pressure-induced order-disorder transitions in beta-In2S3: an experimental and theoretical study of structural and vibrational properties10.1039/D1CP02969J ↗
13. High-pressure phase diagrams of FeSe1–xTex: correlation between suppressed nematicity and enhanced superconductivity10.1038/s41467-020-20621-2 ↗
14. La2Rh3+δ Sb4: a new ternary superconducting rhodium-antimonide10.1088/2752-5724/ac972f ↗
15. Tailoring the oxygen concentration in Ge–Sb–O alloys to enable femtojoule-level phase-change memory operations10.1088/2752-5724/aca07b ↗
16. Passivation of layered gallium telluride by double encapsulation with graphene10.1021/acsomega.9b01752 ↗
17. Effects of interlayer interactions on the nanoindentation response of freely suspended multilayer gallium telluride10.1088/1361-6528/ab668b ↗
18. Unusual deformation and fracture in gallium telluride multilayers10.1021/acs.jpclett.2c00411 ↗
19. Migration of Te inclusions in CdZnTe single crystals under the temperature gradient annealing10.1016/j.jcrysgro.2014.04.004 ↗
20. Dislocation-mediated coupling mechanism between the microstructural defects and Te inclusions in CdZnTe single crystals10.1016/j.scriptamat.2014.03.007 ↗
21. Interlayer investigations of GaN heterostructures integrated into silicon substrates by surface activated bonding10.3390/cryst13020217 ↗
22. Superconductivity in In2Te3 under compression induced by electronic and structural phase transitions10.1021/acs.jpclett.1c04124 ↗
23. Decompression-driven superconductivity enhancement in In2Se310.1002/adma.201701983 ↗
24. Resistivity studies on Ga2Te3 and In2Te3 under high pressures10.1016/0167-577X(82)90007-6 ↗
25. Electrical properties of the high-pressure phases of gallium and indium tellurides10.1134/1.1131343 ↗
26. Thermal conductivity of materials under pressure10.1038/s42254-022-00423-9 ↗
27. Metallization and superconductivity in the van der Waals compound CuP2Se through pressure-tuning of the interlayer coupling10.1021/jacs.1c09735 ↗
28. Large area growth of fewlayer In2Te3 films by chemical vapor deposition and its magnetoresistance properties10.1038/s41598-019-47520-x ↗
29. Tinkham · 1975 · 281
30. Onset of superconductivity in the two-dimensional limit10.1103/PhysRevLett.62.2180 ↗
31. Superconducting-insulating transition in two-dimensional a-MoGe thin films10.1103/PhysRevLett.74.3037 ↗
32. Highly crystalline 2D superconductors10.1038/natrevmats.2016.94 ↗
33. Local disorder effects on the pressure dependence of the metal–insulator transition in manganese perovskites10.1063/1.121432 ↗
34. Structural disordering process of an amorphous alloy driven by the elastostatic compression at room temperature10.1063/1.2908218 ↗
35. Bandgap widening by pressure-induced disorder in two-dimensional lead halide perovskite10.1063/1.5143795 ↗