journal article·2025

Optical spin polarization by coherent magnetoabsorption generation

Gabriel M. Jacobsen, Vinicius A. Oliveira, Baolai Liang, André Pelais, Hryhorii V. Stanchu, Morgan E. Ware, Gregory J. Salamo, Yuriy I. Mazur, Gilmar. E. Marques, Victor Lopez-Richard, Marcio D. Teodoro

Nanoscale· Volume 17· Issue 29
Publisher page

Abstract

/GaAs quantum wells (QWs) is investigated through magneto-photoluminescence measurements. Notably, spin-dependent intensity oscillations emerge in high magnetic fields, originating from interband transitions between Landau levels in the GaAs barriers and described by the magnetoabsorption effect. These spin-resolved absorption resonances, when coupled with coherent relaxation toward the ground-state optical transition in the type-II QWs lead to pronounced spin polarization peaks. A theoretical framework based on rate equations for spin-split states demonstrates that such polarization is only achieved when spin-flip times are comparable to or exceed the optical recombination time, ensuring that spin orientation is maintained from carrier excitation to optical recombination. This prediction is experimentally validated though time-resolved measurements with circularly polarized excitation, where a spin lifetime of 3.5 ns is determined, confirming the role of magnetoabsorption in sustaining spin coherence.
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Research context

OpenAlex topics: Quantum and electron transport phenomena · Quantum Information and Cryptography · Semiconductor Quantum Structures and Devices

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Physics, Federal University of São Carlos, 13565-905, São Carlos, São Paulo, Brazil

Institute for Nanoscience and Engineering, University of Arkansas, 72701, Fayetteville, Arkansas, USA

Department of Electrical and Computer Engineering, California NanoSystems Institute, University of California – Los Angeles, 90095, Los Angeles, California, USA

Funding

Fundação de Amparo à Pesquisa do Estado de São Paulo · Conselho Nacional de Desenvolvimento Científico e Tecnológico

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