journal article·2025Open access

Controlled bioorthogonal catalyst self-assembly and activity using rationally designed polymer scaffolds

Rui Huang, Cristina-Maria Hirschbiegel, David C. Luther, Cheng-Hsuan Li, Ahmed Nabawy, Jungmi Park, Alexander Ribbe, Yisheng Xu, Vincent M. Rotello

Nanoscale· Volume 17· Issue 1

Abstract

Polymer-based nanocatalysts have been extensively utilized in advanced drug delivery due to their versatility and high reactivity. Incorporating bioorthogonal transition metal catalysts (TMCs) into polymers generates bioorthogonal nanocatalysts capable of producing therapeutic agents in situ, minimizing off-target effects. The supramolecular interactions within the polymer matrix, including hydrophobic interactions and aromatic stacking, play a crucial role in catalytic properties. Our study focuses on co-engineering the host polymer structure and the catalyst encapsulation process to achieve precise control over the supramolecular interactions within the nanoenvironment. By carefully engineering these interactions, we successfully generate thermo-responsive nanocatalysts with a resolution of 6 °C. These nanocatalysts demonstrate thermal activation of the catalytic deprotection of a pro-antibiotic, with concomitant external control of bacterial biofilm eradication.
Source: europepmc · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Advanced Nanomaterials in Catalysis · Supramolecular Self-Assembly in Materials · Advanced biosensing and bioanalysis techniques

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Chemistry, University of Massachusetts Amherst, 710 North Pleasant Street, Amherst, Massachusetts 01003, USA

Department of Polymer Science and Engineering, University of Massachusetts Amherst, 120 Governors Dr, Amherst, MA 01003, USA

State Key Laboratory of Chemical Engineering, East China University of Science and Technology, Shanghai, 200237, P. R. China

Funding

National Institutes of Health · National Basic Research Program of China · University of Massachusetts

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