journal article·2022

Inert metal induces the modulation of unsaturated aldehyde absorption mode for enhanced selective hydrogenation

Qinglin Liu, Jiayi Wu, Jiawei Kang, Qian Liu, Peisen Liao, Guangqin Li

Nanoscale· Volume 14· Issue 41
Publisher page

Abstract

Selective hydrogenation of α,β-unsaturated aldehydes to obtain a high yield of unsaturated alcohols is important in industrial production. This is still a great challenge because it is thermally more favorable for the hydrogenation of CC than for the CO bond. Various strategies have been developed to optimize the catalysts for improving selectivity but are usually accompanied by the sacrifice of catalytic activity. Herein, we adopt the inert metal inducement strategy to synthesize a series of Ir-M alloy nanoparticle catalysts. The optimal catalyst IrCd5 exhibits impressive catalytic performance in the selective hydrogenation of cinnamaldehyde, achieving 96.7% conversion with 94.3% selectivity for cinnamal alcohol, which is far superior to that of the Ir counterpart. Furthermore, the H2 temperature-programmed desorption (H2-TPD) test, styrene-TPD test, surface valence band test and density functional theory calculations demonstrate that the adsorption mode of cinnamaldehyde shifted from parallel to vertical configurations after introducing an inert metal. Compared to Ir, the weaker adsorption of alkene and stronger adsorption of the substrate for IrCd5 lead to the prior adsorption and hydrogenation of the CO bond, thus elevating the selectivity of the cinnamal alcohol. This strategy disperses precious metal nanoparticles effectively, maximizes atomic utilization, and improves the selectivity, which provides a new avenue to design bimetal alloy catalysts for the selective hydrogenation of α,β-unsaturated aldehydes.
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Research context

OpenAlex topics: Nanomaterials for catalytic reactions · Catalysis and Hydrodesulfurization Studies · Asymmetric Hydrogenation and Catalysis

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou 510006, P. R. China

Funding

National Key Research and Development Program of China · Fundamental Research Funds for the Central Universities · Sun Yat-sen University · Guangdong Innovative and Entrepreneurial Research Team Program · National Natural Science Foundation of China

References (57)

Show source-provided references
1. Zhao · Nature · 2016 · 539 · 7610.1038/nature19763 ↗
2. Kuai · Nat. Commun. · 2020 · 11 · 4810.1038/s41467-019-13941-5 ↗
3. Bakuru · Chem. – Eur. J. · 2017 · 23 · 1645610.1002/chem.201704119 ↗
4. Long · ACS Catal. · 2018 · 8 · 850610.1021/acscatal.8b01851 ↗
5. Liu · J. Mater. Chem. A · 2020 · 8 · 1144210.1039/D0TA01845G ↗
6. Liu · Chin. Chem. Lett. · 2021 · 33 · 37410.1016/j.cclet.2021.06.047 ↗
7. Wang · ACS Catal. · 2018 · 9 · 15410.1021/acscatal.8b03471 ↗
8. Bai · J. Am. Chem. Soc. · 2018 · 140 · 838410.1021/jacs.8b03862 ↗
9. Wang · Adv. Funct. Mater. · 2018 · 28 · 170591810.1002/adfm.201705918 ↗
10. Wu · ACS Catal. · 2019 · 9 · 642510.1021/acscatal.9b00917 ↗
11. Mitsudome · Chem. – Eur. J. · 2013 · 19 · 525510.1002/chem.201204160 ↗
12. Li · Mater. Horiz. · 2017 · 4 · 58410.1039/C6MH00478D ↗
13. Zhang · Chem. Commun. · 2019 · 55 · 498910.1039/C9CC01572H ↗
14. Harada · Adv. Funct. Mater. · 2008 · 18 · 219010.1002/adfm.200701442 ↗
15. Guo · ACS Catal. · 2018 · 8 · 1138610.1021/acscatal.8b02103 ↗
16. Ju · ACS Sustainable Chem. Eng. · 2017 · 5 · 251610.1021/acssuschemeng.6b02865 ↗
17. Lan · ACS Catal. · 2020 · 10 · 276410.1021/acscatal.9b04331 ↗
18. Liu · ChemCatChem · 2016 · 8 · 94610.1002/cctc.201501256 ↗
19. Liu · Ind. Eng. Chem. Res. · 2015 · 54 · 148710.1021/ie504357r ↗
20. Gu · Chem. Sci. · 2019 · 10 · 211110.1039/C8SC05450A ↗
21. Yu · Appl. Catal., B · 2020 · 277 · 11927310.1016/j.apcatb.2020.119273 ↗
22. Zhang · Small · 2018 · 14 · 170431810.1002/smll.201704318 ↗
23. Dai · J. Catal. · 2018 · 364 · 19210.1016/j.jcat.2018.05.008 ↗
24. Yang · ACS Catal. · 2018 · 8 · 1174910.1021/acscatal.8b02755 ↗
25. Zhou · J. Mater. Chem. A · 2016 · 4 · 1282510.1039/C6TA04542A ↗
26. Taylor · Appl. Catal., B · 2021 · 284 · 11973710.1016/j.apcatb.2020.119737 ↗
27. Pi · Adv. Funct. Mater. · 2017 · 27 · 170088610.1002/adfm.201700886 ↗
28. Wang · Inorg. Chem. · 2020 · 59 · 569410.1021/acs.inorgchem.0c00458 ↗
29. Lyu · J. Am. Chem. Soc. · 2021 · 143 · 14910.1021/jacs.0c05408 ↗
30. Chen · ACS Catal. · 2015 · 5 · 206210.1021/cs501953d ↗
31. Li · Angew. Chem., Int. Ed. · 2017 · 56 · 1637110.1002/anie.201710164 ↗
32. Chen · ACS Cent. Sci. · 2019 · 5 · 17610.1021/acscentsci.8b00805 ↗
33. Feng · J. Am. Chem. Soc. · 2020 · 142 · 96210.1021/jacs.9b10816 ↗
34. Li · Nano Lett. · 2020 · 20 · 140310.1021/acs.nanolett.9b05024 ↗
35. Yuan · Angew. Chem., Int. Ed. · 2018 · 57 · 570810.1002/anie.201801289 ↗
36. Tamura · ACS Catal. · 2016 · 6 · 360010.1021/acscatal.6b00400 ↗
37. Wang · Angew. Chem., Int. Ed. · 2020 · 59 · 1273610.1002/anie.202003651 ↗
38. Wei · Chem. Sci. · 2017 · 8 · 512610.1039/C7SC00568G ↗
39. Han · Nat. Commun. · 2019 · 10 · 378710.1038/s41467-019-11794-6 ↗
40. Ren · Nat. Commun. · 2019 · 10 · 450010.1038/s41467-019-12459-0 ↗
41. Tamura · ACS Catal. · 2017 · 7 · 510310.1021/acscatal.7b01055 ↗
42. Tamura · ACS Sustainable Chem. Eng. · 2017 · 5 · 368510.1021/acssuschemeng.6b03060 ↗
43. Chang · Mol. Catal. · 2017 · 433 · 7710.1016/j.mcat.2017.01.009 ↗
44. Deng · J. Am. Chem. Soc. · 2021 · 143 · 2089810.1021/jacs.1c09535 ↗
45. Wang · Angew. Chem., Int. Ed. · 2019 · 58 · 766810.1002/anie.201903827 ↗
46. Ling · Angew. Chem., Int. Ed. · 2021 · 61 · e20211639610.1002/anie.202116396 ↗
47. Lv · Angew. Chem., Int. Ed. · 2020 · 59 · 2352110.1002/anie.202009913 ↗
48. Shen · ACS Catal. · 2021 · 11 · 523110.1021/acscatal.1c00200 ↗
49. Lv · Angew. Chem., Int. Ed. · 2022 · 61 · e20211453910.1002/anie.202114539 ↗
50. Jin · Angew. Chem., Int. Ed. · 2021 · 60 · 1743010.1002/anie.202106459 ↗
51. Xu · Angew. Chem., Int. Ed. · 2020 · 59 · 351110.1002/anie.201914335 ↗
52. Kharas · J. Macromol. Sci., Part A · 2007 · 43 · 3910.1080/10601320500405851 ↗
53. Li · Chem · 2021 · 7 · 68610.1016/j.chempr.2020.11.023 ↗
54. Choe · Angew. Chem., Int. Ed. · 2020 · 59 · 365010.1002/anie.201913453 ↗
55. Han · Angew. Chem., Int. Ed. · 2020 · 59 · 1182410.1002/anie.202003208 ↗
56. Yang · CCS Chem. · 2021 · 3 · 2631
57. Liu · CCS Chem. · 2022 · 4 · 327510.31635/ccschem.022.202201801 ↗