journal article·2023

Strong gate-tunability of flat bands in bilayer graphene due to moiré encapsulation between hBN monolayers

Robin Smeyers, Milorad V. Milošević, Lucian Covaci

Nanoscale· Volume 15· Issue 9
Publisher page

Abstract

When using hexagonal boron-nitride (hBN) as a substrate for graphene, the resulting moiré pattern creates secondary Dirac points. By encapsulating a multilayer graphene within aligned hBN sheets the controlled moiré stacking may offer even richer benefits. Using advanced tight-binding simulations on atomistically-relaxed heterostructures, here we show that the gap at the secondary Dirac point can be opened in selected moiré-stacking configurations, and is independent of any additional vertical gating of the heterostructure. On the other hand, gating can broadly tune the gap at the principal Dirac point, and may thereby strongly compress the first moiré mini-band in width against the moiré-induced gap at the secondary Dirac point. We reveal that in hBN-encapsulated bilayer graphene this novel mechanism can lead to isolated bands flatter than 10 meV under moderate gating, hence presenting a convenient pathway towards electronically-controlled strongly-correlated states on demand.
Source: openalex_inverted_index · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Graphene research and applications · Diamond and Carbon-based Materials Research · Advancements in Semiconductor Devices and Circuit Design

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Physics and NANOlab Center of Excellence, University of Antwerp, Groenenborgerlaan 171, 2020 Antwerp, Belgium

Instituto de Física, Universidade Federal de Mato Grosso, Cuiabá, Mato Grosso 78060-900, Brazil

Funding

Fonds Wetenschappelijk Onderzoek

References (47)

Show source-provided references
1. Bolotin · Solid State Commun. · 2008 · 146 · 35110.1016/j.ssc.2008.02.024 ↗
2. Decker · Nano Lett. · 2011 · 11 · 229110.1021/nl2005115 ↗
3. Dean · Nat. Nanotechnol. · 2010 · 5 · 72210.1038/nnano.2010.172 ↗
4. Xue · Nat. Mater. · 2011 · 10 · 28210.1038/nmat2968 ↗
5. Chen · Nat. Nanotechnol. · 2008 · 3 · 20610.1038/nnano.2008.58 ↗
6. Park · Phys. Rev. Lett. · 2008 · 101 · 12680410.1103/PhysRevLett.101.126804 ↗
7. Yankowitz · Nat. Phys. · 2012 · 8 · 38210.1038/nphys2272 ↗
8. Wallbank · Phys. Rev. B: Condens. Matter Mater. Phys. · 2013 · 87 · 24540810.1103/PhysRevB.87.245408 ↗
9. Wallbank · Ann. Phys. · 2015 · 527 · 35910.1002/andp.201400204 ↗
10. Moon · Phys. Rev. B: Condens. Matter Mater. Phys. · 2014 · 90 · 15540610.1103/PhysRevB.90.155406 ↗
11. Cea · Phys. Rev. B · 2020 · 102 · 15513610.1103/PhysRevB.102.155136 ↗
12. Jung · Phys. Rev. B · 2017 · 96 · 08544210.1103/PhysRevB.96.085442 ↗
13. Cao · Nature · 2018 · 556 · 4310.1038/nature26160 ↗
14. Cao · Nature · 2018 · 556 · 8010.1038/nature26154 ↗
15. Chittari · Phys. Rev. Lett. · 2019 · 122 · 01640110.1103/PhysRevLett.122.016401 ↗
16. Chen · Nat. Phys. · 2019 · 15 · 23710.1038/s41567-018-0387-2 ↗
17. Zhang · Phys. Rev. Lett. · 2021 · 127 · 16680210.1103/PhysRevLett.127.166802 ↗
18. Suárez Morell · Phys. Rev. B: Condens. Matter Mater. Phys. · 2010 · 82 · 12140710.1103/PhysRevB.82.121407 ↗
19. Zhu · Phys. Rev. Lett. · 2020 · 125 · 11640410.1103/PhysRevLett.125.116404 ↗
20. Wu · Sci. China: Phys., Mech. Astron. · 2021 · 64 · 267811
21. Marchenko · Sci. Adv. · 2018 · 4 · eaau005910.1126/sciadv.aau0059 ↗
22. Mayorov · Nano Lett. · 2011 · 11 · 239610.1021/nl200758b ↗
23. Kretinin · Nano Lett. · 2014 · 14 · 327010.1021/nl5006542 ↗
24. Oka · Phys. Rev. B · 2021 · 104 · 03530610.1103/PhysRevB.104.035306 ↗
25. Anđelković · Nano Lett. · 2020 · 20 · 97910.1021/acs.nanolett.9b04058 ↗
26. Wang · Nano Lett. · 2019 · 19 · 237110.1021/acs.nanolett.8b05061 ↗
27. Long · npj Comput Mater · 2021 · 8 · 7310.1038/s41524-022-00763-1 ↗
28. Kuiri · Phys. Rev. B · 2021 · 103 · 11541910.1103/PhysRevB.103.115419 ↗
29. Jung · Nat. Commun. · 2015 · 6 · 630810.1038/ncomms7308 ↗
30. McCann · Rep. Prog. Phys. · 2013 · 76 · 05650310.1088/0034-4885/76/5/056503 ↗
31. Zhang · Phys. Rev. B: Condens. Matter Mater. Phys. · 2010 · 82 · 03540910.1103/PhysRevB.82.035409 ↗
32. Chen · Nature · 2019 · 572 · 21510.1038/s41586-019-1393-y ↗
33. Kim · Nano Lett. · 2018 · 18 · 773210.1021/acs.nanolett.8b03423 ↗
34. Zheng · Nature · 2020 · 588 · 7110.1038/s41586-020-2970-9 ↗
35. Zhu · Phys. Rev. B · 2022 · 106 · 20513410.1103/PhysRevB.106.205134 ↗
36. Domaretskiy · Nat. Nanotechnol. · 2022 · 1
37. Weintrub · Nat. Commun. · 2022 · 13 · 660110.1038/s41467-022-34158-z ↗
38. Argentero · Nano Lett. · 2017 · 17 · 140910.1021/acs.nanolett.6b04360 ↗
39. Woods · Nat. Phys. · 2014 · 10 · 45110.1038/nphys2954 ↗
40. Slater · Phys. Rev. · 1954 · 94 · 149810.1103/PhysRev.94.1498 ↗
41. Menezes · Phys. Rev. B: Condens. Matter Mater. Phys. · 2014 · 89 · 03543110.1103/PhysRevB.89.035431 ↗
42. Weiße · Rev. Mod. Phys. · 2006 · 78 · 27510.1103/RevModPhys.78.275 ↗
43. Plimpton · J. Comput. Phys. · 1995 · 117 · 110.1006/jcph.1995.1039 ↗
44. Plimpton · MRS Bull. · 2012 · 37 · 51310.1557/mrs.2012.96 ↗
45. Brenner · J. Phys.: Condens. Matter · 2002 · 14 · 783
46. Kolmogorov · Phys. Rev. Lett. · 2000 · 85 · 472710.1103/PhysRevLett.85.4727 ↗
47. Tersoff · Phys. Rev. B: Condens. Matter Mater. Phys. · 1988 · 37 · 699110.1103/PhysRevB.37.6991 ↗