Boosting nanoparticle yield: enhanced atom-to-nanoparticle conversion in gas aggregation
Source abstract
Abstract
Nanoparticles are atomic aggregates with diameters around 10 nm and are highly valued for their unique properties and broad technological applications. Their synthesis via physical methods offers key advantages over chemical methods, including high purity, precise size control, and material versatility, whilst also being environmentally friendly. A current disadvantage of physical synthesis is that they typically suffer from low production yields and inefficient atom-to-nanoparticle conversion. This paper describes the mechanisms of nanoparticle growth and presents a strategy to enhance their production in gas-aggregation systems. The approach leverages pulsed magnetron sputtering, where atoms serve as building blocks for nanoparticle formation. By optimizing pulse duration and repetition frequency, this paper shows significant improvement in atom-to-nanoparticle conversion demonstrating improved nanoparticle production by an order of magnitude without increasing the amount of sputtered material or overall energy consumption. This advancement paves the way for more cost-effective and scalable nanoparticle manufacturing.
Source: europepmc · Quality: candidate unverified · Source record ↗
Research context
OpenAlex topics: Catalytic Processes in Materials Science · Coagulation and Flocculation Studies
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
University of South Bohemia, Faculty of Science, Branisovska 1760, 37005 Ceske Budejovice, Czech Republic
Warsaw University of Technology, Institute of Microelectronics and Optoelectronics, Koszykowa 75, 00-662 Warsaw, Poland
Funding
Technology Agency of the Czech Republic · North Atlantic Treaty Organization · Politechnika Warszawska
References (60)
Show source-provided references
1. Haviar · Int. J. Hydrogen Energy · 2018 · 43 · 2275610.1016/j.ijhydene.2018.10.127 ↗
2. Kumar · Nanomaterials · 2021 · 11 · 345610.3390/nano11123456 ↗
3. Sato · Biomaterials · 2005 · 26 · 134910.1016/j.biomaterials.2004.04.044 ↗
4. Lin · J. Nanopart. Res. · 2019 · 21 · 13710.1007/s11051-019-4581-7 ↗
5. Podestà · J. Phys. Chem. C · 2009 · 113 · 1826410.1021/jp905930r ↗
6. Wei · J. Appl. Phys. · 2009 · 105 · 07C51710.1063/1.3074509 ↗
7. Tiwari · Chem. Commun. · 2008 · 651610.1039/b813935k ↗
8. Khomiakova · Vacuum · 2023 · 217 · 11258610.1016/j.vacuum.2023.112586 ↗
9. Linic · Nat. Mater. · 2011 · 10 · 91110.1038/nmat3151 ↗
10. Coronado · Nanoscale · 2011 · 3 · 404210.1039/c1nr10788g ↗
11. Chen · Chem. Rev. · 2010 · 110 · 376710.1021/cr9003902 ↗
12. Wang · Chem. Commun. · 2008 · 501010.1039/b807660j ↗
13. Hong · Curr. Appl. Phys. · 2009 · 9 · 17210.1016/j.cap.2008.01.010 ↗
14. Yi · J. Electroanal. Chem. · 2008 · 619–620 · 19710.1016/j.jelechem.2008.03.012 ↗
15. Lepró · Chem. Phys. Lett. · 2008 · 463 · 12410.1016/j.cplett.2008.08.001 ↗
16. Wang · Electrochim. Acta · 2008 · 53 · 694410.1016/j.electacta.2008.02.028 ↗
17. Hou · Small · 2006 · 2 · 23510.1002/smll.200500328 ↗
18. Bass · Ind. Eng. Chem. Res. · 2008 · 47 · 718410.1021/ie8007506 ↗
19. Taguchi · Vacuum · 2008 · 83 · 57510.1016/j.vacuum.2008.04.023 ↗
20. Bommersbach · J. Phys. Chem. C · 2008 · 112 · 1467210.1021/jp801143a ↗
21. Grammatikopoulos · Adv. Phys.:X · 2016 · 1 · 8110.1080/23746149.2016.1142829 ↗
22. Kashtanov · Phys.-Usp. · 2007 · 50 · 45510.1070/PU2007v050n05ABEH006138 ↗
23. R.Hippler , H.Kersten , M.Schmidt and K. H.Schoenbach , Low temperature plasmas: Fundamentals, Technologies and Techniques , Wiley-VCH , 2008
24. Haberland · Z. Phys. D: At., Mol. Clusters · 1991 · 20 · 41310.1007/BF01544025 ↗
25. Haberland · Phys. Rev. B: Condens. Matter Mater. Phys. · 1995 · 51 · 1106110.1103/PhysRevB.51.11061 ↗
26. Mayoral · Nanotechnology · 2019 · 30 · 06560610.1088/1361-6528/aaf1fa ↗
27. Pilch · Appl. Phys. Lett. · 2013 · 102 · 03310810.1063/1.4788739 ↗
28. Pleskunov · Appl. Surf. Sci. · 2023 · 639 · 15823510.1016/j.apsusc.2023.158235 ↗
29. M. C. M.Ramos and M. d. M.Sanz Lluch , High–Flux DC Magnetron Sputtering , in Gas–Phase Synthesis of Nanoparticles , 2017 , pp. 137–154 . 10.1002/9783527698417.ch810.1002/9783527698417.ch8 ↗
30. Shelemin · Vacuum · 2015 · 120 · 16210.1016/j.vacuum.2015.07.008 ↗
31. Nikitin · Plasma Processes Polym. · 2021 · 18 · 210006810.1002/ppap.202100068 ↗
32. Drache · Phys. Status Solidi A · 2014 · 211 · 118910.1002/PSSA.201330399 ↗
33. Coroa · Surf. Coat. Technol. · 2025 · 500 · 13189210.1016/j.surfcoat.2025.131892 ↗
34. Knabl · Vacuum · 2024 · 230 · 11372410.1016/j.vacuum.2024.113724 ↗
35. Smirnov · Phys. Rev. E: Stat., Nonlinear, Soft Matter Phys. · 2007 · 75 · 06640210.1103/PhysRevE.75.066402 ↗
36. Haberland · Phys. Rev. Lett. · 1991 · 67 · 329010.1103/PhysRevLett.67.3290 ↗
37. Bogaerts · J. Appl. Phys. · 1999 · 86 · 412410.1063/1.371337 ↗
38. Hippler · Plasma Sources Sci. Technol. · 2018 · 27 · 06501010.1088/1361-6595/aacb5c ↗
39. H.Haberland , History, some basics, and an outlook , in Gas–Phase Synthesis of Nanoparticles , 2017 , pp. 1–21 . 10.1002/9783527698417.ch110.1002/9783527698417.ch1 ↗
40. Gerhard · Z. Phys. B: Condens. Matter · 1975 · 22 · 4110.1007/BF01325458 ↗
41. Stranak · Contrib. Plasma Phys. · 2011 · 51 · 23710.1002/ctpp.201000065 ↗
42. Samuelsson · Surf. Coat. Technol. · 2010 · 205 · 59110.1016/j.surfcoat.2010.07.041 ↗
43. Sader · Rev. Sci. Instrum. · 1999 · 70 · 396710.1063/1.1150021 ↗
44. Batková · Surf. Coat. Technol. · 2021 · 417 · 12719610.1016/j.surfcoat.2021.127196 ↗
45. Davis · Phys. Rev. · 1963 · 131 · 21910.1103/PhysRev.131.219 ↗
46. Britun · J. Appl. Phys. · 2015 · 117 · 16330210.1063/1.4919006 ↗
47. Ran · J. Phys. Chem · 1993 · 97 · 853510.1063/1.481343 ↗
48. Signorell · J. Chem. Phys. · 1997 · 107 · 1081910.1063/1.474199 ↗
49. Sanzone · Rev. Sci. Instrum. · 2021 · 92 · 03390110.1063/5.0028854 ↗
50. Zhang · Vacuum · 2016 · 128 · 13710.1016/j.vacuum.2016.03.011 ↗
51. Ali-Ogly · J. Phys. D: Appl. Phys. · 2022 · 55 · 44520310.1088/1361-6463/ac8c4e ↗
52. Curda · Surf. Coat. Technol. · 2023 · 473 · 13004510.1016/j.surfcoat.2023.130045 ↗
53. Kousal · Nanoscale · 2018 · 10 · 1827510.1039/C8NR06155F ↗
54. Drewes · Plasma Processes Polym. · 2022 · 19 · 210012510.1002/PPAP.202100125 ↗
55. Drewes · Part. Part. Syst. Charact. · 2022 · 39 · 220011210.1002/PPSC.202200112 ↗
56. Smirnov · Phys.-Usp. · 2011 · 54 · 69110.3367/UFNE.0181.201107B.0713 ↗
57. Stranak · Contrib. Plasma Phys. · 2011 · 51 · 23710.1002/ctpp.201000065 ↗
58. Ayesh · J. Mater. Res. · 2013 · 28 · 262210.1557/jmr.2013.246 ↗
59. Anders · Appl. Phys. Rev. · 2024 · 1 · 03131010.1063/5.0205274 ↗
60. Ganeva · Surf. Coat. Technol. · 2012 · 213 · 4110.1016/j.surfcoat.2012.10.012 ↗