journal article·2023

Reflective dielectric cavity enhanced emission from hexagonal boron nitride spin defect arrays

Xiao-Dong Zeng, Yuan-Ze Yang, Nai-Jie Guo, Zhi-Peng Li, Zhao-An Wang, Lin-Ke Xie, Shang Yu, Yu Meng, Qiang Li, Jin-Shi Xu, Wei Liu, Yi-Tao Wang, Jian-Shun Tang, Chuan-Feng Li, Guang-Can Guo

Nanoscale· Volume 15· Issue 36
Publisher page

Abstract

Among the various kinds of spin defects in hexagonal boron nitride (hBN), the negatively charged boron vacancy (VB-) spin defect that can be site-specifically generated is undoubtedly a potential candidate for quantum sensing, but its low quantum efficiency restricts its practical applications. Here, we demonstrate a robust enhancement structure called reflective dielectric cavity (RDC) with advantages including easy on-chip integration, convenient processing, low cost and suitable broad-spectrum enhancement for VB- defects. In the experiment, we used a metal reflective layer under the hBN flakes, filled with a transition dielectric layer in the middle, and adjusted the thickness of the dielectric layer to achieve the best coupling between RDC and spin defects in hBN. A remarkable 11-fold enhancement in the fluorescence intensity of VB- spin defects in hBN flakes can be achieved. By designing the metal layer into a waveguide structure, high-contrast optically detected magnetic resonance (ODMR) signal (∼21%) can be obtained. The oxide layer of the RDC can be used as the integrated material to implement secondary processing of micro-nano photonic devices, which means that it can be combined with other enhancement structures to achieve stronger enhancement. This work has guiding significance for realizing the on-chip integration of spin defects in two-dimensional materials.
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Research context

OpenAlex topics: Diamond and Carbon-based Materials Research · Graphene research and applications · Semiconductor materials and devices

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui 230026, China

CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui 230026, China

Institute of Advanced Semiconductors and Zhejiang Provincial Key Laboratory of Power Semiconductor Materials and Devices, ZJU-Hangzhou Global Scientific and Technological Innovation Center, Hangzhou, Zhejiang 311200, China

State Key Laboratory of Silicon Materials and Advanced Semiconductors and School of Materials Science and Engineering, Zhejiang University, Hangzhou 310027, China

Hefei National Laboratory, University of Science and Technology of China, Hefei, Anhui 230088, China

Funding

Fok Ying Tong Education Foundation · Youth Innovation Promotion Association of the Chinese Academy of Sciences · National Natural Science Foundation of China

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