journal article·2020

Monolayer 2D ZrTe 2 transition metal dichalcogenide as nanoscatter for random laser action

Pablo I. R. Pincheira, Manoel L. da Silva Neto, Melissa Maldonado, Cid B. de Araújo, Ali M. Jawaid, Robert Busch, Allyson J. Ritter, Richard A. Vaia, Anderson S. L. Gomes

Nanoscale· Volume 12· Issue 29
Publisher page

Abstract

We demonstrate random laser emission from Rhodamine 6G with ZrTe2 transition metal dichalcogenide (TMD) as nanoscatters, both in powder and 2D nanoflakes liquid suspension. The 2D semimetal ZrTe2 was synthesized by a modified redox exfoliation method to provide single layer TMD, which was employed for the first time as the scatter medium to provide feedback in an organic gain medium random laser. In order to exploit random laser emission and its threshold value, replica symmetry breaking leading to a photonic paramagnetic to photonic spin glass transition in both 2D and 3D (powder) ZrTe2 was demonstrated. One important aspect of mixing organic dyes with ZrTe2 is that there is no chemical reaction leading to dye degradation, demonstrated by operating over more than 2 hours of pulsed (5 Hz) random laser emission.
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Research context

OpenAlex topics: Random lasers and scattering media · Orbital Angular Momentum in Optics · Photonic Crystals and Applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Departamento de Ciencias Fisicas

Universidad de La Frontera

Temuco

Chile

Graduate Program in materials Science

Universidade Federal de Pernambuco

Recife-PE

Brazil

Departamento de Física

Recife

Materials and Manofacturing Directorate

Air Force Research Laboratories

USA

Funding

Conselho Nacional de Desenvolvimento Científico e Tecnológico · Fundação de Amparo à Ciência e Tecnologia do Estado de Pernambuco · Coordenação de Aperfeiçoamento de Pessoal de Nível Superior · Air Force Office of Scientific Research · Air Force Research Laboratory · Fondo Nacional de Desarrollo Científico y Tecnológico

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