journal article·2020Open access

Optically detected magnetic resonance in CdSe/CdMnS nanoplatelets

Danil O. Tolmachev, Vitalii Yu. Ivanov, Dmitri R. Yakovlev, Elena V. Shornikova, Bartłomiej Witkowski, Sushant Shendre, Furkan Isik, Savas Delikani, Hilmi Volkan Demir, Manfred Bayer

Nanoscale· Volume 12· Issue 42

Abstract

Core/shell CdSe/(Cd,Mn)S colloidal nanoplatelets containing magnetic Mn2+ ions are investigated by the optically detected magnetic resonance technique, combining 60 GHz microwave excitation and photoluminescence detection. Resonant heating of the Mn spin system is observed. We identify two mechanisms of optical detection, via variation of either the photoluminescence polarization or its intensity in an external magnetic field. The spin-lattice relaxation dynamics of the Mn spin system is measured and used for evaluation of the Mn concentration. In CdSe/(Cd,Zn,Mn)S nanoplatelets the addition of Zn in the shells significantly broadens the magnetic resonance, evidencing local strain.
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Research context

OpenAlex topics: Quantum Dots Synthesis And Properties · Chalcogenide Semiconductor Thin Films · Semiconductor Quantum Structures and Devices

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Experimentelle Physik 2

Technische Universität Dortmund

44227 Dortmund

Germany

Ioffe Institute

Institute of Physics

Polish Academy of Sciences

PL-02-668 Warsaw

Poland

LUMINOUS! Center of Excellence for Semiconductor Lighting and Displays

School of Electrical and Electronic Engineering

School of Physical and Materials Sciences

Nanyang Technological University

639798 Singapore

Department of Electrical and Electronics Engineering

Department of Physics

UNAM – Institute of Materials Science and Nanotechnology

Bilkent University

06800 Ankara

Funding

Deutsche Forschungsgemeinschaft · Russian Science Foundation · Narodowe Centrum Nauki · National Research Foundation Singapore · Türkiye Bilimler Akademisi

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