journal article·2025-04-01Open access

Surface magnetism in Fe3GeTe2 van der Waals ferromagnet

Trevor A Tyson, Sandun Amarasinghe, A M Milinda Abeykoon, Roger Lalancette, Kai Du, Xiaochen Fang, Sang-W Cheong, Abdullah Al-Mahboob, Jerzy T Sadowski

2D Materials· Volume 12· Issue 2

Abstract

Abstract The surface magnetization of Fe3GeTe2 was examined by low-energy electron microscopy (LEEM) using an off-normal incidence electron beam. We found that the 180° domain walls are of Bloch type. Temperature-dependent LEEM measurements yield a surface magnetization with a surface critical exponent β1 = 0.79 ± 0.02. This result is consistent with surface magnetism in the 3D semi-infinite Heisenberg (β1 = 0.84 ± 0.01) or Ising (β1 = 0.78 ± 0.02) models, which is distinctly different from the bulk exponent (β = 0.34 ± 0.07). The measurements reveal the power of LEEM with a tilted beam to determine magnetic domain structure in quantum materials without the need for the use of spin-polarized electrons. Single crystal diffraction measurements reveal inversion symmetry-breaking weak peaks and yield space group P-6m2. This Fe site defect-derived loss of inversion symmetry enables the formation of skyrmions in this Fe3GeTe2 crystal.
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Research context

OpenAlex topics: 2D Materials and Applications · Iron-based superconductors research · Chalcogenide Semiconductor Thin Films

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

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