journal article·2019-04

TiO2/MoS2 heterojunctions-decorated carbon fibers with broad-spectrum response as weaveable photocatalyst/photoelectrode

Zhun Shi, Pengfei Xu, Xiaofeng Shen, Yan Zhang, Li Luo, Gumila Duoerkun, Lisha Zhang

Publisher page

Abstract

Abstract The development of efficient and recyclable photocatalysts with wide spectrum response has drawn much attention. Herein, we prepared TiO2/MoS2 heterostructures on carbon fibers (CFs) by a two-step hydrothermal method. CFs/TiO2/MoS2 exhibits a strong and wide absorption spectrum from ultraviolet to near-infrared region (>1200 nm). Under the irradiation of visible-light, CFs/TiO2/MoS2 could degrade 97.6% Rhodamine B (RhB) after 100 min, 94.2% Acid Orange 7 (AO7) or 93.4% tetracycline hydrochloride (TC) after 60 min, and 88.7% 4-chlorophenol (4-CP) after 180 min. Moreover, CFs/TiO2/MoS2 bundles can be further weaved into a cloth (area: 4 × 4 cm2). CFs/TiO2/MoS2 cloth as a working electrode exhibits significant photocurrent (7.53 × 10−6 A/cm2) and enhanced photoelectrocatalytic efficiency (100% TC) comparing with only photocatalysis (90.7% TC) or electrocatalysis (47% TC). In particular, CFs/TiO2/MoS2 cloth shows excellent stability. Therefore, CFs/TiO2/MoS2 cloth has great potential to be used as flexible and weaveable photocatalyst/photoelectrode for degrading various pollutants.
Source: openaire · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Advanced Photocatalysis Techniques · TiO2 Photocatalysis and Solar Cells · Carbon and Quantum Dots Applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (44)

Show source-provided references
1. Recent developments in photocatalytic water treatment technology: a review10.1016/j.watres.2010.02.039 ↗
2. Nano-photocatalytic materials: possibilities and challenges10.1002/adma.201102752 ↗
3. Titanium dioxide-based nanomaterials for photocatalytic fuel generations10.1021/cr500008u ↗
4. Photocatalytic oxidation of organic dyes and pollutants in wastewater using different modified titanium dioxides: a comparative review10.1016/j.jiec.2014.10.043 ↗
5. One-dimensional TiO2Nanotube photocatalysts for solar water splitting10.1002/advs.201600152 ↗
6. Preparation of TiO2/C3N4 heterojunctions on carbon-fiber cloth as efficient filter-membrane-shaped photocatalyst for removing various pollutants from the flowing wastewater10.1016/j.jcis.2018.08.028 ↗
7. Synthesis of Au-decorated V2O5@ZnO heteronanostructures and enhanced plasmonic photocatalytic activity10.1021/am501549n ↗
8. Hierarchical assembly of graphene-bridged Ag3PO4 /Ag/BiVO4(040) Z-scheme photocatalyst: An efficient, sustainable and heterogeneous catalyst with enhanced visible-light photoactivity towards tetracycline degradation under visible light irradiation10.1016/j.apcatb.2016.07.021 ↗
9. Enhanced photocatalytic performance of morphologically tuned Bi2S3 NPs in the degradation of organic pollutants under visible light irradiation10.1016/j.jcis.2016.08.023 ↗
10. Wafer-level artificial photosynthesis for CO2 reduction into CH4and CO using GaN nanowires10.1021/acscatal.5b00776 ↗
11. MoS2/graphene cocatalyst for efficient photocatalytic H2 evolution under visible light irradiation10.1021/nn5019945 ↗
12. Single-layer MoS2 as an efficient photocatalyst10.1039/c3cy00207a ↗
13. Recent development on MoS2-based photocatalysis: a review10.1016/j.jphotochemrev.2017.12.002 ↗
14. Semiconductor heterojunction photocatalysts: design, construction, and photocatalytic performances10.1039/C4CS00126E ↗
15. MoS2/CdS nanosheets-on-nanorod heterostructure for highly efficient photocatalytic H2 generation under visible light irradiation10.1021/acsami.6b02687 ↗
16. Fabrication of a novel p–n heterojunction photocatalyst n-BiVO4@p-MoS2 with core–shell structure and its excellent visible-light photocatalytic reduction and oxidation activities10.1016/j.apcatb.2015.12.023 ↗
17. highly efficient visible-light-induced photoactivity of Z-scheme g-C3N4/Ag/MoS2 ternary photocatalysts for organic pollutant degradation and production of hydrogen10.1021/acssuschemeng.6b02010 ↗
18. In situ light-assisted preparation of MoS2 on graphitic C3N4 nanosheets for enhanced photocatalytic H2 production from water10.1039/C5TA00402K ↗
19. Application of carbon fibers to biomaterials: a new era of nano-level control of carbon fibers after 30-years of development10.1039/c0cs00120a ↗
20. Growth of C3N4 nanosheets on carbon-fiber cloth as flexible and macroscale filter-membrane-shaped photocatalyst for degrading the flowing wastewater10.1016/j.apcatb.2017.07.059 ↗
21. Growth of TiO2 nanorod bundles on carbon fibers as flexible and weaveable photocatalyst/photoelectrode10.1039/C5RA21344D ↗
22. Preparation of TiO2/Bi2WO6 nanostructured heterojunctions on carbon fibers as a weaveable visible-light photocatalyst/photoelectrode10.1039/C7EN00822H ↗
23. Bactericidal activity of photocatalytic TiO2 reaction: toward an understanding of its killing mechanism10.1128/AEM.65.9.4094-4098.1999 ↗
24. Glucose-assisted synthesis of the hierarchical TiO2 nanowire@MoS2 nanosheet nanocomposite and its synergistic lithium storage performance10.1039/C4TA05249H ↗
25. Hierarchical porous carbon nanofibers as binder-free electrode for high-performance supercapacitor10.1016/j.electacta.2016.02.050 ↗
26. Preparation, characterization and photocatalytic activities of holmium-doped titanium dioxide nanoparticles10.1016/j.jhazmat.2008.03.114 ↗
27. Graphene-like MoS2/amorphous carbon composites with high capacity and excellent stability as anode materials for lithium ion batteries10.1039/c1jm10174a ↗
28. Interface band engineering charge transfer for 3D MoS2 photoanode to boost photoelectrochemical water splitting10.1021/acssuschemeng.6b02883 ↗
29. Construction of N-doped TiO2/MoS2 heterojunction with synergistic effect for enhanced visible photodegradation activity10.1016/j.materresbull.2018.04.046 ↗
30. Hierarchical MoS2 Nanosheet@TiO2 nanotube array composites with enhanced photocatalytic and photocurrent performances10.1002/smll.201503441 ↗
31. Vertical single or few-layer MoS2 nanosheets rooting into TiO2 nanofibers for highly efficient photocatalytic hydrogen evolution10.1016/j.apcatb.2014.08.046 ↗
32. Interface engineering of few-layered MoS2 nanosheets with ultrafine TiO2 nanoparticles for ultrastable Li-ion batteries10.1016/j.cej.2018.03.166 ↗
33. Self-supported nanotube arrays of sulfur-doped TiO2 enabling ultrastable and robust sodium storage10.1002/adma.201504412 ↗
34. Fabrication of 3D flower-like black N-TiO2-x@MoS2 for unprecedented-high visible-light-driven photocatalytic performance10.1016/j.apcatb.2016.08.031 ↗
35. The fabrication, microstructure, photo-catalysis and piezo-catalysis of layered TiO2-MoS2
36. 2D co-catalytic MoS2 nanosheets embedded with 1D TiO2 nanoparticles for enhancing photocatalytic activity10.1088/0022-3727/49/31/315304 ↗
37. Dependence of the absorption and optical surface plasmon scattering of MoS2 nanoparticles on aspect ratio, size, and media10.1021/nn5000354 ↗
38. Constructing 2D porous graphitic C3N4 nanosheets/nitrogen-doped graphene/layered MoS2 ternary nanojunction with enhanced photoelectrochemical activity10.1002/adma.201303116 ↗
39. Heterogeneous degradation of tetracycline by magnetic Ag/AgCl/modified zeolite X–persulfate system under visible light10.1039/C6RA00695G ↗
40. Synthesis of BiOBr/WO3 p–n heterojunctions with enhanced visible light photocatalytic activity10.1039/C6CE00824K ↗
41. Synthesis of Ta3N5/Bi2MoO6 core–shell fiber-shaped heterojunctions as efficient and easily recyclable photocatalysts10.1039/C6EN00706F ↗
42. Synthesis of Au nanoparticle-decorated carbon nitride nanorods with plasmon-enhanced photoabsorption and photocatalytic activity for removing various pollutants from water10.1016/j.jhazmat.2017.10.040 ↗
43. Efficient hydrogen evolution and rapid degradation of organic pollutants by robust catalysts of MoS2/TNT@CNTs10.1016/j.ijhydene.2018.07.051 ↗
44. Molybdenum disulphide/titanium dioxide nanocomposite-poly 3-hexylthiophene bulk heterojunction solar cell10.1063/1.3703602 ↗